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石墨烯量子点介导的肖特基结光疗：卓越抗菌性能与快速伤口愈合

李江婷 ,  欧阳峰 ,  王强 ,  周尚 ,  包锡旭 ,  程雅琪 ,  杨一菲 ,  陈沛 ,  陈伊鹏 ,  张继业 ,  王亮 ,  钟海舰

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引用本文: 李江婷, 欧阳峰, 王强, 周尚, 包锡旭, 程雅琪, 杨一菲, 陈沛, 陈伊鹏, 张继业, 王亮, 钟海舰. 石墨烯量子点介导的肖特基结光疗：卓越抗菌性能与快速伤口愈合[J]. 物理化学学报, 2026, 42(7): 100223. doi: 10.1016/j.actphy.2025.100223 shu
Citation:  Jiangting Li,  Feng Ouyang,  Qiang Wang,  Shang Zhou,  Xixu Bao,  Yaqi Cheng,  Yifei Yang,  Pei Chen,  Yipeng Chen,  Jiye Zhang,  Liang Wang,  Haijian Zhong. Schottky junction phototherapy mediated by graphene quantum dots for superior antibacterial performance and rapid wound healing[J]. Acta Physico-Chimica Sinica, 2026, 42(7): 100223. doi: 10.1016/j.actphy.2025.100223 shu

石墨烯量子点介导的肖特基结光疗：卓越抗菌性能与快速伤口愈合

  • 1.

    赣南医科大学组织工程江西省重点实验室, 江西 赣州 341000;

  • 2.

    赣南医科大学医学信息工程学院, 江西 赣州 341000;

  • 3.

    赣南医科大学心脑血管疾病防治教育部重点实验室, 江西 赣州 341000;

  • 4.

    赣南医科大学基础医学院, 江西 赣州 341000;

  • 5.

    上海大学材料科学与工程学院, 上海 200444;

  • 6.

    上海大学环境与化学工程学院纳米化学与生物学研究所, 上海 200444

    • 通讯作者: 王亮,E-mail:wangl@shu.edu.cn; 钟海舰,E-mail:Hjzhong2007@gmu.edu.cn
  • 基金项目:

    本研究获国家自然科学基金(61674164，62164001和62571141)、心脑血管疾病防治教育部重点实验室开放课题(XN201903)资助。江西省职业早期青年科技人才项目(20244BCE52228和20244BCE52225)以及赣南医科大学博士启动基金(QD202403和QD202402)对本研究提供支持。

摘要: 抗生素耐药性感染日益严重的威胁亟需发展先进的非侵入性治疗策略。本文构建了一种基于肖特基结的金纳米粒子(AuNPs)与氧化石墨烯量子点(GOQDs)纳米复合材料，其中GOQDs作为多功能构建单元，在460 nm LED照射下协同增强光动力治疗(PDT)和光热治疗(PTT)。GOQDs不仅能促进电荷分离与转移以产生活性氧(ROS)，其宽光谱吸收特性与高电子迁移率还可提升光热转换效率。此外，其丰富的表面官能团可增强分散性、生物相容性及组织亲和力。所制备的AuNPs/GOQDs纳米复合材料展现出优异的分散稳定性、增强的光热与ROS输出性能以及卓越的生物相容性。体外抗菌实验表明其对革兰氏阳性菌和阴性菌的杀灭效率均> 97%。更重要的是，在小鼠伤口感染模型中，该纳米复合材料能在9天内实现约99%的伤口愈合率，显著优于对照组治疗。组织学分析进一步证实其能减轻炎症并加速组织再生。本研究揭示了GOQDs在增强光触发抗菌活性和促进伤口愈合中的关键作用，为临床治疗多重耐药病原体提供了有前景的光疗策略。

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