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S型异质结In2O3/ZnIn2S4光催化5-羟甲基糠醛选择性氧化耦合产氢

骆泽 ,  朱玉坤 ,  罗雅丹 ,  任广敏 ,  王永红 ,  唐华

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引用本文: 骆泽, 朱玉坤, 罗雅丹, 任广敏, 王永红, 唐华. S型异质结In2O3/ZnIn2S4光催化5-羟甲基糠醛选择性氧化耦合产氢[J]. 物理化学学报, 2026, 42(3): 100166. doi: 10.1016/j.actphy.2025.100166 shu
Citation:  Ze Luo,  Yukun Zhu,  Yadan Luo,  Guangmin Ren,  Yonghong Wang,  Hua Tang. Photocatalytic selective oxidation of 5-hydroxymethylfurfural coupled with H2 evolution over In2O3/ZnIn2S4 S-scheme heterojunction[J]. Acta Physico-Chimica Sinica, 2026, 42(3): 100166. doi: 10.1016/j.actphy.2025.100166 shu

S型异质结In2O3/ZnIn2S4光催化5-羟甲基糠醛选择性氧化耦合产氢

  • 1.

    青岛大学, 环境与地理科学学院, 材料科学与工程学院, 山东 青岛 266071;

  • 2.

    青岛科技大学, 化工学院, 山东 青岛 266042

    • 通讯作者: 唐华,Email:huatang79@163.com
  • 基金项目:

    本研究部分得到国家自然科学基金(22378219)资助

摘要: 发展可持续的光催化技术，以实现生物质向高附加值化学品和清洁燃料的高效转化，是应对全球能源与环境危机有效途径。本研究通过原位生长法构建了一种新型一维/二维(1D/2D)In2O3/ZnIn2S4 S型异质结光催化剂。该设计巧妙结合棒状In2O3与片状ZnIn2S4，促进定向电荷传输并提供高密度活性位点。因此，优化后的In2O3/ZnIn2S4异质结在420 nm LED光照下对5-羟甲基糠醛(HMF)转化率达81.6%，且对2,5-二甲酰基呋喃(DFF)和2,5-呋喃二甲酸(FDCA)的选择性高达78.2%。同时，该异质结表现出257.69 μmol g-1 h-1的产氢(H2)速率。这些结果表明，S型异质结能有效实现空间电荷分离并提升光催化活性，为太阳能驱动的生物质增值与可持续产氢提供了可行策略。

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