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离子热法合成沸石咪唑骨架材料及其溶解-结晶机理研究

王亚松 ,  徐云鹏 ,  李大伟 ,  刘浩 ,  厉晓蕾 ,  陶硕 ,  田志坚

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引用本文: 王亚松, 徐云鹏, 李大伟, 刘浩, 厉晓蕾, 陶硕, 田志坚. 离子热法合成沸石咪唑骨架材料及其溶解-结晶机理研究[J]. 催化学报, 2015, 36(6): 855-865. doi: 10.1016/S1872-2067(14)60278-3 shu
Citation:  Yasong Wang, Yunpeng Xu, Dawei Li, Hao Liu, Xiaolei Li, Shuo Tao, Zhijian Tian. Ionothermal synthesis of zeolitic imidazolate frameworks and the synthesis dissolution-crystallization mechanism[J]. Chinese Journal of Catalysis, 2015, 36(6): 855-865. doi: 10.1016/S1872-2067(14)60278-3 shu

离子热法合成沸石咪唑骨架材料及其溶解-结晶机理研究

    通讯作者: 田志坚,电话/传真: (0411)84379151; 电子信箱: tianz@dicp.ac.cn
  • 基金项目:

    国家自然科学基金(21001102, 21373214). (21001102, 21373214)

摘要: 基于沸石咪唑骨架材料在离子液体和低共熔溶剂中冷却结晶的析出方式, 开发了一种离子热法合成沸石咪唑骨架材料的新途径, 采用X射线衍射、扫描电镜、核磁共振光谱、红外光谱以及热重分析等方法对制备的产物进行了表征, 研究了合成条件对产物结晶度、尺寸和形貌的影响, 探讨了沸石咪唑骨架材料在离子热合成体系中的溶解-结晶析出机理. 研究发现, 冷却速率能够影响产物形貌, 急速冷却时, sod (RCSR代码)型产物的形貌为球形, zni (RCSR代码)型产物为棒状或平板状; 程序控制冷却时, sod型产物的形貌为多面体, zni型产物呈团簇状.

English

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  • 发布日期:  2015-06-20
  • 收稿日期:  2014-11-14
  • 网络出版日期:  2014-12-14
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