尿素对土壤中碳钢微生物腐蚀的影响

引用本文: 孙成, 李喜明, 许进, 闫茂成, 王福会, 王振尧. 尿素对土壤中碳钢微生物腐蚀的影响[J]. 物理化学学报, doi: 10.3866/PKU.WHXB201208243 shu

Citation: SUN Cheng, LI Xi-Ming, XU Jin, YAN Mao-Cheng, WANG Fu-Hui, WANG Zhen-Yao. Effect of Urea on Microbiologically Induced Corrosion of Carbon Steel in Soil[J]. Acta Physico-Chimica Sinica, doi: 10.3866/PKU.WHXB201208243 shu

尿素对土壤中碳钢微生物腐蚀的影响

基金项目:
国家自然科学基金(50971128, 51161001) (50971128, 51161001)

国家科技基础条件平台建设项目(2005DKA10400-CT-2-02)资助 (2005DKA10400-CT-2-02)

摘要:

采用失重、极化曲线和阻抗谱等方法研究了尿素对土壤中微生物腐蚀(MIC)的影响. 研究结果表明, 在接菌土壤中尿素加速碳钢的腐蚀, 而在灭菌土壤中抑制其腐蚀. 接菌土壤中由于硫酸盐还原菌(SRB)的存在,腐蚀产物中检测到FeS₂. 电化学阻抗谱(EIS)的结果表明, 在实验后期腐蚀过程由浓差极化控制.

关键词:

English

Effect of Urea on Microbiologically Induced Corrosion of Carbon Steel in Soil

1.
State Key Laboratory for Corrosion and Protection, Institute of Metals Research, Chinese Academy of Sciences, Shenyang 110016, P. R. China
Received Date: 12 June 2012
Available Online: 17 October 2012
Fund Project:
国家自然科学基金(50971128, 51161001)

国家科技基础条件平台建设项目(2005DKA10400-CT-2-02)资助

Abstract:

The effect of urea on microbiologically induced corrosion (MIC) of carbon steel in soil was investigated using weight-loss measurement, electrochemical polarization, and electrochemical impedance spectroscopy (EIS). Urea tends to accelerate corrosion of carbon steel in inoculated soils and inhibit corrosion in sterile soils. In inoculated soils, FeS₂ was detected in corrosion products because of the presence of sulfate-reducing bacteria (SRB). The EIS results showed that the process was controlled by concentration polarization in the later stages.

Key words:

Sulphate-reducing bacteria
/ Carbon steel
/ Urea
/ Electrochemical impedance spectroscopy
/ Weight loss

1. [1]
  
  (1) Chaker, V.; Palmer, J. D. Effects of Soil Characteristics on Corrosion, ASTM STP 1013, American Society of Testing andMaterials ( ASTM) International,West Conshohocken,Pennsylvania, 1989; p 37.
  (1) Chaker, V.; Palmer, J. D. Effects of Soil Characteristics on Corrosion, ASTM STP 1013, American Society of Testing andMaterials ( ASTM) International,West Conshohocken,Pennsylvania, 1989; p 37.
2. [2]
  (2) Benmoussa, A.; Hadjel, M.; Traisnel, M. Materials and Corrosion-Werkstoffe Und Korrosion 2006, 57 (10), 771. doi: 10.1002/(ISSN)1521-4176(2) Benmoussa, A.; Hadjel, M.; Traisnel, M. Materials and Corrosion-Werkstoffe Und Korrosion 2006, 57 (10), 771. doi: 10.1002/(ISSN)1521-4176
3. [3]
  (3) Ismail, A. I. M.; El-Shamy, A. M. Applied Clay Science 2009,42 (3-4), 356. doi: 10.1016/j.clay.2008.03.003(3) Ismail, A. I. M.; El-Shamy, A. M. Applied Clay Science 2009,42 (3-4), 356. doi: 10.1016/j.clay.2008.03.003
4. [4]
  (4) Liu, T. M.;Wu, Y. H.; Luo, S. X.; Sun, C.Materialwissenschaft und Werkstofftechnik 2010, 41 (4), 228.doi: 10.1002/(ISSN)1521-4052(4) Liu, T. M.;Wu, Y. H.; Luo, S. X.; Sun, C.Materialwissenschaft und Werkstofftechnik 2010, 41 (4), 228.doi: 10.1002/(ISSN)1521-4052
5. [5]
  (5) Pope, D. H.; Duquette, D. J.; Johannes, A. H.;Wayner, P. C.Materials Performance 1984, 23 (4), 14.(5) Pope, D. H.; Duquette, D. J.; Johannes, A. H.;Wayner, P. C.Materials Performance 1984, 23 (4), 14.
6. [6]
  (6) Little., B.;Wagner, P.; Mansfeld, F. Electrochimica Acta 1992,37 (12), 9.(6) Little., B.;Wagner, P.; Mansfeld, F. Electrochimica Acta 1992,37 (12), 9.
7. [7]
  (7) Wagner, P.; Little, B. Materials Performance 1993, 32 (9), 65.(7) Wagner, P.; Little, B. Materials Performance 1993, 32 (9), 65.
8. [8]
  (8) Hernandez, G.; Kucera, V.; Thierry, D.; Pedersen, A.;Hermansson, M. Corrosion 1994, 50, 603. doi: 10.5006/1.3293532(8) Hernandez, G.; Kucera, V.; Thierry, D.; Pedersen, A.;Hermansson, M. Corrosion 1994, 50, 603. doi: 10.5006/1.3293532
9. [9]
  (9) Pikas, J. L. Corrosion 1996, 96, 7.(9) Pikas, J. L. Corrosion 1996, 96, 7.
10. [10]
  (10) Li, S. Y.; Kim, Y. G.; Jeon, K. S.; Kho, Y. T.; Kang, T. Corrosion2001, 57, 815. doi: 10.5006/1.3280616(10) Li, S. Y.; Kim, Y. G.; Jeon, K. S.; Kho, Y. T.; Kang, T. Corrosion2001, 57, 815. doi: 10.5006/1.3280616
11. [11]
  (11) Rao, T. S. Corrosion Reviews 2009, 333.(11) Rao, T. S. Corrosion Reviews 2009, 333.
12. [12]
  (12) Hamilton,W. A. Annual Review of Microbiology 1985, 39, 195.doi: 10.1146/annurev.mi.39.100185.001211(12) Hamilton,W. A. Annual Review of Microbiology 1985, 39, 195.doi: 10.1146/annurev.mi.39.100185.001211
13. [13]
  (13) Lee,W.; Lewandowski, Z.; Nielsen, P. H.; Hamilton,W. A.Biofouling 1995, 8 (3), 165. doi: 10.1080/08927019509378271(13) Lee,W.; Lewandowski, Z.; Nielsen, P. H.; Hamilton,W. A.Biofouling 1995, 8 (3), 165. doi: 10.1080/08927019509378271
14. [14]
  (14) Rao, T. S.; Sairam, T. N.; Viswanathan, B.; Nair, K. V. K.Corrosion Science 2000, 42 (8), 1417. doi: 10.1016/S0010-938X(99)00141-9(14) Rao, T. S.; Sairam, T. N.; Viswanathan, B.; Nair, K. V. K.Corrosion Science 2000, 42 (8), 1417. doi: 10.1016/S0010-938X(99)00141-9
15. [15]
  (15) Videla, H. A. Biofouling 2000, 15 (1-3), 37. doi: 10.1080/08927010009386296(15) Videla, H. A. Biofouling 2000, 15 (1-3), 37. doi: 10.1080/08927010009386296
16. [16]
  (16) Liu, T.; Liu, H.; Hu, Y.; Zhou, L.; Zheng, I. Materials and Corrosion-Werkstoffe Und Korrosion 2009, 60 (3), 218. doi: 10.1002/maco.v60:3(16) Liu, T.; Liu, H.; Hu, Y.; Zhou, L.; Zheng, I. Materials and Corrosion-Werkstoffe Und Korrosion 2009, 60 (3), 218. doi: 10.1002/maco.v60:3
17. [17]
  (17) Booth, G. H.; Tiller, A. K. Transactions of the Faraday Society1960, 56, 1689. doi: 10.1039/tf9605601689(17) Booth, G. H.; Tiller, A. K. Transactions of the Faraday Society1960, 56, 1689. doi: 10.1039/tf9605601689
18. [18]
  (18) Booth, G. H.; Tiller, A. K. Corrosion Science 1968, 8 (8), 583.doi: 10.1016/S0010-938X(68)80094-0(18) Booth, G. H.; Tiller, A. K. Corrosion Science 1968, 8 (8), 583.doi: 10.1016/S0010-938X(68)80094-0
19. [19]
  (19) Javaherdashti, R. Applied Microbiology and Biotechnology2011, 91 (6), 1507. doi: 10.1007/s00253-011-3455-4(19) Javaherdashti, R. Applied Microbiology and Biotechnology2011, 91 (6), 1507. doi: 10.1007/s00253-011-3455-4
20. [20]
  (20) Li, Y.; Zhang, T.;Wang, F. H. Journal of Chinese Society for Corrosion and Protection 2004, 24, 334 [李瑛, 张涛,王福会. 中国腐蚀与防护学报, 2004, 24, 334.](20) Li, Y.; Zhang, T.;Wang, F. H. Journal of Chinese Society for Corrosion and Protection 2004, 24, 334 [李瑛, 张涛,王福会. 中国腐蚀与防护学报, 2004, 24, 334.]
21. [21]
  (21) Mozheiko, F. F.; Potkina, T. N.; ncharik, I. I. Russian Journal of Applied Chemistry 2008, 81 (9), 1705. doi: 10.1134/S1070427208090437(21) Mozheiko, F. F.; Potkina, T. N.; ncharik, I. I. Russian Journal of Applied Chemistry 2008, 81 (9), 1705. doi: 10.1134/S1070427208090437
22. [22]
  (22) Booth, G. H.; Cooper, A.W.; Cooper, P. M.;Wakerley, D. S.British Corrosion Journal 1967, 2, 104. doi: 10.1179/000705967798326957(22) Booth, G. H.; Cooper, A.W.; Cooper, P. M.;Wakerley, D. S.British Corrosion Journal 1967, 2, 104. doi: 10.1179/000705967798326957
23. [23]
  (23) Stations National Soil Corrosion Test Networks. Test Methods of Soil Corrosion of Materials; Science Press: Beijing, 1990. [全国土壤腐蚀试验网站编. 材料土壤腐蚀试验方法. 北京: 科学出版社, 1990.](23) Stations National Soil Corrosion Test Networks. Test Methods of Soil Corrosion of Materials; Science Press: Beijing, 1990. [全国土壤腐蚀试验网站编. 材料土壤腐蚀试验方法. 北京: 科学出版社, 1990.]
24. [24]
  (24) Wei, B. M. The Corrosion Theory and Application of Metals;Chemical Industry Press: Beijing, 2004. [魏宝明. 金属腐蚀理论及应用. 北京: 化学工业出版社, 2004.](24) Wei, B. M. The Corrosion Theory and Application of Metals;Chemical Industry Press: Beijing, 2004. [魏宝明. 金属腐蚀理论及应用. 北京: 化学工业出版社, 2004.]
25. [25]
  (25) Li, M. C.; Lin, H. C.; Cao, C. N. Journal of Chinese Society for Corrosion and Protection 2000, 20, 111. [李谋成,林海潮, 曹楚南. 中国腐蚀与防护学报, 2000, 20, 111.](25) Li, M. C.; Lin, H. C.; Cao, C. N. Journal of Chinese Society for Corrosion and Protection 2000, 20, 111. [李谋成,林海潮, 曹楚南. 中国腐蚀与防护学报, 2000, 20, 111.]
26. [26]
  (26) Xu, J.;Wang, K.; Sun, C.;Wang, F.; Li, X.; Yang, J.; Yu, C.Corrosion Science 2011, 53 (4), 1554. doi: 10.1016/j.corsci.2011.01.037(26) Xu, J.;Wang, K.; Sun, C.;Wang, F.; Li, X.; Yang, J.; Yu, C.Corrosion Science 2011, 53 (4), 1554. doi: 10.1016/j.corsci.2011.01.037
27. [27]
  (27) Castaneda, H.; Benetton, X. D. Corrosion Science 2008, 50 (4),1169. doi: 10.1016/j.corsci.2007.11.032(27) Castaneda, H.; Benetton, X. D. Corrosion Science 2008, 50 (4),1169. doi: 10.1016/j.corsci.2007.11.032
28. [28]
  (28) Cao, C. N. Principles of Electrochemistry of Corrosion, 3rd ed.;Chemical Industry Press: Beijing, 2008; pp 93-94. [曹楚南.腐蚀电化学原理. 第三版. 北京: 化学工业出版社, 2008:93-94.]
  (28) Cao, C. N. Principles of Electrochemistry of Corrosion, 3rd ed.;Chemical Industry Press: Beijing, 2008; pp 93-94. [曹楚南.腐蚀电化学原理. 第三版. 北京: 化学工业出版社, 2008:93-94.]

扫一扫看文章

计量

PDF下载量: 813
文章访问数: 2622
HTML全文浏览量: 136

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

尿素对土壤中碳钢微生物腐蚀的影响

English

Effect of Urea on Microbiologically Induced Corrosion of Carbon Steel in Soil

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

尿素对土壤中碳钢微生物腐蚀的影响

English

Effect of Urea on Microbiologically Induced Corrosion of Carbon Steel in Soil

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

文章相关

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs