Citation: MAO Jun-Xian, JIANG Jiao, WANG Hua-Kai, YANG Li-Jun, WANG Yang-Nian, GENG Jiao, WANG Xi-Zhang, HU Zheng. Immobilizing Ruthenium Nanoparticles onto Nitrogen-Doped Carbon Nanotubes for Aerobic Oxidation of Benzyl Alcohol under Ambient Pressure[J]. Chinese Journal of Inorganic Chemistry, ;2012, 28(12): 2508-2512.
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Ruthenium nanoparticles were conveniently immobilized on nitrogen-doped carbon nanotubes (NCNTs) via microwave-assisted ethylene glycol reduction. Ru/NCNTs catalysts presented the excellent catalytic performance and cyclical stability for the aerobic oxidation of benzyl alcohol under atmospheric condition, compared with the catalysts supported on carbon nanotubes (CNTs) and activated carbon (AC). The conversion of benzyl alcohol could rearch 93% and the selectivity of benzaldehyde was higher than 99% at 90 ℃. The doped nitrogen atoms embedded in the NCNTs wall are responsible for the improved catalytic performance.
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