Citation: Feng Boxu, Zhuang Xiaodong. Carbon-Enriched meso-Entropy Materials: from Theory to Cases[J]. Acta Chimica Sinica, ;2020, 78(9): 833-847. doi: 10.6023/A20050167 shu

Carbon-Enriched meso-Entropy Materials: from Theory to Cases

Feng Boxu ,
Zhuang Xiaodong ^,

The meso-Entropy Matter Lab, Frontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China

Corresponding author: Zhuang Xiaodong, zhuang@sjtu.edu.cn
Received Date: 15 May 2020
Available Online: 28 June 2020
Fund Project: National Key Research and Development Program of China 2017YFE9134000Shanghai Pujiang Talent Program 18PJ1406100the National Natural Science Foundation of China 21720102002the National Natural Science Foundation of China 51811530013the National Natural Science Foundation of China Excellent Young Scientists Fund 51722304Project supported by the National Natural Science Foundation of China Excellent Young Scientists Fund (No. 51722304), National Key Research and Development Program of China (No. 2017YFE9134000), the National Natural Science Foundation of China (Nos. 51973114, 21720102002, 51811530013), Shanghai Pujiang Talent Program (No. 18PJ1406100), Science and Technology Commission of Shanghai Municipality (No. 19JC412600).the National Natural Science Foundation of China 51973114Technology Commission of Shanghai Municipality 19JC412600

Figures(19)

Carbon-enriched materials, including carbon allotropes, polycyclic aromatic hydrocarbons, polymers, frameworks, etc., are rising as stars in functional materials field. Large amount of reported work focused on development of new structures with typical features for novel applications, and has long ignored the intrinsic relationship between similar structures. The superficial relationships of those carbon-enriched materials in textbook, e.g., isomers, allotropes and topological defects, are no longer enough for fundamental understanding the structure-property relationship study due to more and more carbon-enriched materials have been developed. Such disadvantage has long hindered development of new materials based on well-established material systems. In this work, meso-entropy concept is proposed for understanding and development of different kinds of carbon-enriched materials by comparing their relative entropy values. Based on theoretical models and case-to-case discussion, meso-entropy concept has been found compatible with the concept of isomers, allotropes and topological defects in carbon-enriched materials. From now on, hopefully, the meso-entropy defined relationship for carbon-enriched materials will be no longer staying at the geometric level, and provide new thinking development of new carbon-enriched materials and other meso-entropy materials.
- meso-entropy,
- carbon,
- polymer,
- structure-property relationship,
- preparation
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