Citation: Yu Jun, Yang Yusen, Wei Min. Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides[J]. Acta Chimica Sinica, ;2019, 77(11): 1129-1139. doi: 10.6023/A19070260 shu

Preparation and Catalytic Performance of Supported Catalysts Derived from Layered Double Hydroxides

State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology, Beijing 100029

Corresponding author: Yang Yusen, 2016400160@mail.buct.edu.cn Wei Min, weimin@mail.buct.edu.cn
Received Date: 11 July 2019
Available Online: 4 November 2019
Fund Project: the Fundamental Research Funds for the Central Universities XK1802-6the National Natural Science Foundation of China 21521005the National Key Research and Development Program 2017YFA0206804the National Natural Science Foundation of China 21871021Project supported by the National Natural Science Foundation of China (Nos. 21871021, 21521005), the National Key Research and Development Program (No. 2017YFA0206804), and the Fundamental Research Funds for the Central Universities (Nos. buctylkxj01, XK1802-6)the Fundamental Research Funds for the Central Universities buctylkxj01

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Supported catalysts have been widely used in a large variety of industrial processes, including ammonia synthesis, energy conversion and fine chemical synthesis. Layered double hydroxides (LDHs) are a class of two-dimensional functional anionic materials. By virtue of the unique structural characteristics (e.g., tunability of host layers, high dispersion of metal cations and structure topological transformation), LDHs have shown potential applications in heterogeneous catalysis as precursors or supports. In this review, high-performance monometallic or bimetallic supported catalysts by using LDHs as supports/precursors, or by utilizing mixed metal oxides (MMO) as supports via topotactic transformation from LDHs is highlighted. Their recent progresses in electrocatalysis, oxidative dehydrogenation, selective hydrogenation and syngas conversion reaction are reviewed. In the final section, future opportunities and challenges in the preparation of LDHs-based catalysts are discussed, and some strategies to resolve these critical problems are further proposed.
- layered double hydroxides,
- topological transformation,
- preparation method,
- high dispersion,
- supported catalyst
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沈阳化工大学材料科学与工程学院沈阳 110142