Citation: Yuao WANG, Kai ZHU. Research progress of electrolyte additives for aqueous zinc-ion batteries[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(10): 2063-2076. doi: 10.11862/CJIC.20260194 shu

Research progress of electrolyte additives for aqueous zinc-ion batteries

Yuao WANG ,
Kai ZHU ^,

Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin 150001, China

Corresponding author: Kai ZHU, kzhu@hrbeu.edu.cn
Received Date: 17 June 2026
Revised Date: 2 September 2026

Figures(6)

Aqueous zinc-ion batteries have attracted increasing attention for large-scale energy storage because of their intrinsic safety, low cost, high ionic conductivity, and environmental friendliness. However, the practical application of aqueous zinc-ion batteries is still limited by unstable Zn anodes and complex electrode/electrolyte interfacial reactions, including dendrite growth, hydrogen evolution, corrosion, interfacial by-product accumulation, and cathode dissolution. Electrolyte additives provide an efficient and readily implementable strategy to regulate these issues at the molecular and interfacial levels. In this review, recent progress in electrolyte additives for aqueous zinc-ion batteries is summarized with emphasis on their roles in modulating Zn²⁺ solvation structures, reconstructing the electric double layer and electrode/electrolyte interface, regulating Zn deposition texture, suppressing cathode dissolution and buffering interfacial pH fluctuations. The structure-function relationships of representative additives are discussed, and the remaining challenges associated with mechanistic understanding, additive consumption, long-term stability, multicomponent synergy, harsh-condition adaptability, and practical engineering are further highlighted. This review aims to provide guidance for the rational design of electrolyte additives toward highly reversible, durable, and scalable aqueous zinc-ion batteries.
- aqueous zinc-ion batteries,
- electrolyte additives,
- zinc anode,
- interface regulation
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沈阳化工大学材料科学与工程学院沈阳 110142