Citation: Shouhao WAN, Yihang SHEN, Xiang GAO, Yang CHEN, Jiaqi LI, Cuie ZHAO. Two-dimensional MOFs/MXene composite for high-performance transparent zinc-ion hybrid supercapacitors[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(8): 1582-1592. doi: 10.11862/CJIC.20260077 shu

Two-dimensional MOFs/MXene composite for high-performance transparent zinc-ion hybrid supercapacitors

School of Materials Science and Engineering, State Key Laboratory of Flexible Electronics (LoFE), Nanjing University of Posts and Telecommunications, Nanjing 210023, China

Corresponding author: Cuie ZHAO, iamcezhao@njupt.edu.cn
Received Date: 9 March 2026
Revised Date: 9 June 2026

Figures(6)

A facile electrostatic self-assembly strategy for the construction of a two-dimensional Cu-TCPP/MXene composite (Cu-TCPP=tetracarboxyphenyl porphyrin copper) was proposed, featuring a well-integrated heterogeneous interface with highly conductive networks and porous ion transport channels. This unique architecture effectively accelerates electrolyte ion diffusion and charge transfer. Under optimized ratio, the Cu-TCPP/MXene electrode exhibited high optical transmittance exceeding 60%, and the assembled transparent supercapacitor delivered an outstanding areal capacitance of 7.48 mF·cm^-2. Furthermore, an asymmetric zinc-ion hybrid supercapacitor (ZIHSC) was constructed by employing the Cu-TCPP/MXene as the cathode and electrochemically deposited zinc as the anode. The ZIHSC device achieved a wide voltage window of 0-1.2 V, a high transmittance of 58.9%, an outstanding areal capacitance of 10.5 mF·cm^-2, and an energy density of 2.1 μWh·cm^-2.
- asymmetric device,
- transparent electrode,
- ion transport,
- electrostatic self-assembly,
- heterogeneous interface
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