Citation: Jiancheng LAN, Xiaolan FU, Meiling FAN, Naibo ZHAO, Yu'nan ZHOU. High-performance Ta-based halide electrolytes via co-sintering method[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(10): 2162-2168. doi: 10.11862/CJIC.20260071 shu

High-performance Ta-based halide electrolytes via co-sintering method

Jiancheng LAN ^{1, 2} ,
Xiaolan FU ^{1, 2} ,
Meiling FAN ^{1, 2} ,
Naibo ZHAO ^{1, 2} ,
Yu'nan ZHOU ^{1, 2,,}

1.
Zhejiang Green Intelligent Transportation Technology Innovation Co., Ltd., Ningbo, Zhejiang 315300, China
2.
Zhejiang Geely Holding Group Co., Ltd., Hangzhou 310052, China

Corresponding author: Yu'nan ZHOU, Yunan.Zhou@geely.com
Received Date: 6 March 2026
Revised Date: 15 July 2026

Figures(4)

A high-performance Ta-based halide electrolyte material (denoted Cs-LTOC) and an efficient preparation method were developed. Structural analysis revealed that the Cs-LTOC electrolyte primarily comprises three crystalline phases: LiTaCl₆, LiTaOCl₄, and Ta₂O₅. After process optimization, the as-prepared electrolyte material achieved a high ionic conductivity of 9.02 mS·cm^-1 by simply co-sintering at 250 ℃ for 3 h. All-solid-state batteries assembled with this electrolyte and the high-nickel cathode material LiNi_0.83Co_0.12Mn_0.05O₂ (NCM83) exhibited excellent electrochemical performance. Specifically, at charge/discharge rates of 0.1C (1.0C=200 mA·g^-1), 0.3C, 0.5C, 1.0C, 2.0C, 3.0C, and 5.0C, the NCM83 cathode delivered specific discharge capacities of 221.7, 212.1, 205.9, 195.2, 183.1, 174.8, and 160.8 mAh·g^-1, respectively. Furthermore, it maintained an 81.2% capacity retention after 1 900 cycles at 5.0C.
- Ta-based halide electrolyte,
- co-sintering,
- scalable fabrication
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