Citation: Lihang LAN, Yanyong SHA, Lina YANG, Wentao DAI, Daozhen SHEN, Wenlong LIU, Hongjiang LIU, Qi LIU. A one-dimensional cadmium-based coordination polymer as cathode material of lithium-ion battery[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(8): 1751-1762. doi: 10.11862/CJIC.20260039 shu

A one-dimensional cadmium-based coordination polymer as cathode material of lithium-ion battery

Lihang LAN ^{1, #} ,
Yanyong SHA ^{1, #} ,
Lina YANG ² ,
Wentao DAI ¹ ,
Daozhen SHEN ¹ ,
Wenlong LIU ³ ,
Hongjiang LIU ^2,, ,
Qi LIU ^1,,

1.
School of Petrochemical Engineering and Jiangsu Key Laboratory of Advanced Catalytic Materials Technology, Changzhou University, Changzhou, Jiangsu 213164, China
2.
Department of Chemistry, College of Science, Shanghai University, Shanghai 200444, China
3.
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, Jiangsu 225009, China

Corresponding author: Hongjiang LIU, liuhj@shu.edu.cn Qi LIU, liuqi62@163.com; liuqi@cczu.edu.cn
Received Date: 5 February 2026
Revised Date: 12 May 2026

Figures(8)

A new cadmium-based coordination polymer (CP) with 1D structure, [Cd(4-DTBPT)(DMF)₂(H₂O)₂](C₁₀H₄O₈)·4-DTBPT·3H₂O (Cd-CP), where 4-DTBPT=2,7-di(4H-1,2,4-triazol-4yl)benzo[lmn][3,8]phenanthroline-1,3,6,8-(2H, 7H)-tetraone, DMF=N,N-dimethylformamide, C₁₀H₄O₈^2-=2,5-dicarboxyterephthalate, which originates from the decomposition of N,N′-bis(glycinyl)pyromellitic diimide (BGPD), was firstly synthesized via the interaction of 4-DTBPT, BGPD, and Cd(NO₃)₂·4H₂O, and characterized by IR spectrum, thermogravimetric analysis and single-crystal X-ray diffraction. In Cd-CP, 4-DTBPT ligands linked adjacent Cd(Ⅱ) ions to produce a 1D chain structure. The C₁₀H₄O₈^2- anion and the free 4-DTBPT ligands are respectively embedded between 1D chains through electrostatic force and hydrogen bonds, forming a 3D network structure. When Cd-CP was employed as the cathode material of lithium-ion batteries (LIBs), it delivered the first discharge specific capacity of 78.3 mAh·g^-1 at 0.05 A·g^-1 along with the Coulombic efficiency of close to 100%, and a higher cycle stability with the capacity retention of 85.7% after 100 cycles.
- cadmium(Ⅱ) compound,
- lithium-ion batteries,
- coordination polymer,
- crystal structure,
- cathode material
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沈阳化工大学材料科学与工程学院沈阳 110142