Citation: Guo CHENG, Yuxin SHI, Gang YANG, Huan PANG. Research progress on applications of Prussian blue analogues in aqueous multivalent metal-ion batteries[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(9): 1793-1806. doi: 10.11862/CJIC.20260035 shu

Research progress on applications of Prussian blue analogues in aqueous multivalent metal-ion batteries

Guo CHENG ¹ ,
Yuxin SHI ^2,, ,
Gang YANG ² ,
Huan PANG ^1,,

1.
School of Chemistry & Materials, Yangzhou University, Yangzhou, Jiangsu 225000, China
2.
School of Materials Science and Engineering, Suzhou University of Technology, Suzhou, Jiangsu 215500, China

Corresponding author: Yuxin SHI, yuxinnano@hotmail.com Huan PANG, panghuan@yzu.edu.cn
Received Date: 2 February 2026
Revised Date: 23 April 2026

Figures(5)

Aqueous multivalent metal-ion batteries are a new type of energy storage device that operate on aqueous electrolytes and rely on the intercalation/deintercalation of multivalent metal ions in electrode materials. This type of battery offers significant advantages, including high safety, high conductivity, and high theoretical capacity, and has garnered widespread attention in recent years. However, multivalent metal ions possess a high charge density, leading to a high desolvation energy barrier in aqueous electrolytes. Additionally, solid-phase diffusion in cathode materials encounters kinetic barriers, severely limiting their electrochemical performance and further development. To address these critical challenges, it is crucial to develop cathode materials with fast ion transport channels. Among numerous candidate materials, Prussian blue analogues (PBAs) have been widely investigated as cathodes for aqueous multivalent metal-ion batteries due to their open three-dimensional framework, tunable redox-active sites, and facile synthesis suitable for scale-up. Nevertheless, PBAs are still faced with challenges such as poor conductivity and insufficient structural stability in practical applications. To overcome these limitations, current research strategies primarily focus on constructing multi-metal active sites and designing composites with highly conductive materials, aiming to optimize both charge transfer kinetics and structural integrity. This review systematically summarizes the rational design strategies of PBA-based composites and their applications as cathodes in aqueous multivalent metal-ion batteries, offering valuable insights for the development of high-performance electrode materials in next-generation energy storage systems.
- aqueous batteries,
- Prussian blue analogues,
- composites,
- regulation of structure and component
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沈阳化工大学材料科学与工程学院沈阳 110142