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Citation: Ting YANG, Jia AN, Jinyu ZHANG, Ruonan FAN, Rong YAN, Xiaoxia JING, Panpan CHANG, Wei YAN. Synergistic enhancement of ion migration and sulfur conversion kinetics in lithium-sulfur batteries by CeO2/g-C3N4[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(3): 519-530. doi: 10.11862/CJIC.20250274 shu

Synergistic enhancement of ion migration and sulfur conversion kinetics in lithium-sulfur batteries by CeO2/g-C3N4

  • 1.

    Department of Applied Chemistry, Yuncheng University, Yuncheng, Shanxi 044000, China

  • 2.

    School of Biological and Chemical Engineering, Guangxi University of Science and Technology, Liuzhou, Guangxi 545006, China

  • 3.

    Shanxi Guoxin Logistics Co., Ltd., Yuncheng Branch, Yuncheng, Shanxi 044000, China

Figures(5)

  • To simultaneously accelerate ion transport and catalyze polysulfide conversion in lithium-sulfur (Li-S) batteries, a CeO2/g-C3N4 composite with both lithium affinity and catalytic activity was designed. The abundant nitrogen units within the g-C3N4 nanosheets serve as lithium-affinity sites, reducing the lithium-ion (Li+) migration energy barrier and accelerating Li+ transport via Lewis acid-base interactions. Meanwhile, the Ce4+/Ce3+ redox couple is the key catalytically active sites that drive the generation of thiosulfate and establish a reversible thiosulfate-mediated polysulfide conversion pathway. Such a thiosulfate-mediated pathway promotes the bidirectional conversion of polysulfide. Therefore, modifying the commercial PP separator with CeO2/g-C3N4 composites can effectively enhance the kinetics of polysulfide conversion, reduce charge transfer resistance, and significantly improve the rate performance and cycling performance (1 000 cycles at 1.0C, with a capacity decay rate of only 0.049% per cycle).
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