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Citation: Xiaoqi LAN, Wei LI, Deyi YANG, Hao WANG, Zheng LIU, Rongting GUO, Qizhi CHEN. Preparation and electrochemical performance of “sandwich structured” MXene Ti3C2Tx/hollow ZIF-67 sulfur host composites[J]. Chinese Journal of Inorganic Chemistry, ;2026, 42(4): 760-772. doi: 10.11862/CJIC.20250273 shu

Preparation and electrochemical performance of “sandwich structured” MXene Ti3C2Tx/hollow ZIF-67 sulfur host composites

  • 1.

    Guangxi Key Laboratory of Electrochemical and Magneto-Chemical Functional Materials, College of Chemical and Biological Engineering, Guilin University of Technology, Guilin, Guangxi 541004, China

  • 2.

    School of Energy and Chemical Engineering, Luoyang Institute of Science and Technology, Luoyang, Henan 471023, China

  • 3.

    Guangxi Huiyuan Manganese Industry Co., Ltd., Laibin, Guangxi 546100, China

Figures(9)

  • MXene Ti3C2Tx/ hollow ZIF-67 (HMZ) host capable of loading the cathode active material sulfur in lithium-sulfur batteries was constructed by in-situ electrostatic self-assembly method and etching with tannic acid solution. Hollow ZIF-67 can effectively mitigate the irreversible stacking trend of MXene Ti3C2Tx, and suppress the shuttle effect through the joint chemical adsorption of lithium polysulfides by Ti and Co elements. while also physically confining lithium polysulfides and alleviating the volume expansion. HMZ-5 formed by etching with tannic acid solution for 5 min could provide a specific capacity of 615.1 mAh·g-1 at 1C after being loaded with sulfur, with a low capacity decay rate of 0.055% per cycle after 700 cycles.
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