Citation: Pengyang FAN, Shan FAN, Qinjin DAI, Xiaoying ZHENG, Wei DONG, Mengxue WANG, Xiaoxiao HUANG, Yong ZHANG. Preparation and performance of rich 1T-MoS₂ nanosheets for high-performance aqueous zinc ion battery cathode materials[J]. Chinese Journal of Inorganic Chemistry, ;2025, 41(4): 675-682. doi: 10.11862/CJIC.20240339 shu

Preparation and performance of rich 1T-MoS₂ nanosheets for high-performance aqueous zinc ion battery cathode materials

1.
School of Materials Science and Engineering, Qiqihar University, Qiqihar, Heilongjiang 106000, China
2.
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150080, China

Corresponding author: Shan FAN, fanshan@qqhru.edu.cn Yong ZHANG,
Received Date: 19 September 2024
Revised Date: 25 December 2024

Figures(7)

A cathode material rich in 1T-MoS₂ (1T′-MoS₂) for aqueous zinc ion batteries was successfully synthesized via a one-step hydrothermal method. The characterization results and density functional theory (DFT) simulation calculations indicated that the conductivity of 1T′-MoS₂ was significantly higher than that of 2H-MoS₂, and 1T′-MoS₂ contained abundant sulfur vacancies. That substantially enhances the ion diffusion and charge transfer rates, as well as the electrochemical and kinetic characteristics of the material. Therefore, the initial discharge capacity of the battery assembled with 1T′-MoS₂ was as high as 202 mAh·g^-1 at a current density of 0.1 A·g^-1. In addition, at a high current density (1 A·g^-1), the capacity retention rate was 92% after 500 cycles, showing good high capacity and long-cycle stability.
- aqueous Zn-ion battery,
- 1T-MoS₂,
- sulfur defect,
- cathode material
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Preparation and performance of rich 1T-MoS2 nanosheets for high-performance aqueous zinc ion battery cathode materials

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通讯作者: 陈斌, bchen63@163.com

Preparation and performance of rich 1T-MoS₂ nanosheets for high-performance aqueous zinc ion battery cathode materials