Citation: Ning DING, Siyu WANG, Shihua YU, Pengcheng XU, Dandan HAN, Dexin SHI, Chao ZHANG. Crystalline and amorphous metal sulfide composite electrode materials with long cycle life: Preparation and performance of hybrid capacitors[J]. Chinese Journal of Inorganic Chemistry, ;2024, 40(9): 1784-1794. doi: 10.11862/CJIC.20240146 shu

Crystalline and amorphous metal sulfide composite electrode materials with long cycle life: Preparation and performance of hybrid capacitors

Ning DING ¹ ,
Siyu WANG ¹ ,
Shihua YU ¹ ,
Pengcheng XU ^1,, ,
Dandan HAN ^{1, 2,,} ,
Dexin SHI ³ ,
Chao ZHANG ⁴

1.
College of Chemistry and Pharmaceutical Engineering, Jilin Institute of Chemical Technology, Jilin, Jilin 132022, China
2.
College of Biology & Food Engineering, Jilin Institute of Chemical Technology, Jilin, Jilin 132022, China
3.
Connell Chemical Industry Co., Ltd., Jilin, Jilin 132002, China
4.
Jilin Zhongwang Safety Environment Technology Co., Ltd., Jilin, Jilin 132113, China

Corresponding author: Pengcheng XU, pengchengxu2006@163.com Dandan HAN, luckhan2006@163.com
Received Date: 26 April 2024
Revised Date: 13 June 2024

Figures(7)

Crystalline@amorphous NiCo₂S₄@MoS₂ (v-NCS@MS) nanostructures were designed and constructed via an ethylene glycol-induced strategy with hydrothermal synthesis and solvothermal method, which simultaneously realized the defect regulation of crystal NiCo₂S₄ in the core. Taking advantage of the flexible protection of an amor-phous shell and the high capacity of a conductive core with defects, the v-NCS@MS electrode exhibited high specific capacity (1 034 mAh·g^-1 at 1 A·g^-1) and outstanding rate capability. Moreover, a hybrid supercapacitor was assembled with v-NCS@MS as cathode and activated carbon (AC) as anode, which can achieve remarkably high specific energy of 111 Wh·kg^-1 at a specific power of 219 W·kg^-1 and outstanding capacity retention of 80.5% after 15 000 cycling at different current densities.
- crystalline@amorphous heterostructure,
- NiCo₂S₄@MoS₂,
- hybrid supercapacitor,
- defect design,
- long cycle life
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