Citation: Ting WANG, Peipei ZHANG, Shuqin LIU, Ruihong WANG, Jianjun ZHANG. A Bi-CP-based solid-state thin-film sensor: Preparation and luminescence sensing for bioamine vapors[J]. Chinese Journal of Inorganic Chemistry, ;2024, 40(8): 1615-1621. doi: 10.11862/CJIC.20240134 shu

A Bi-CP-based solid-state thin-film sensor: Preparation and luminescence sensing for bioamine vapors

1.
School of Chemistry, Dalian University of Technology, Dalian, Liaoning 116024, China
2.
School of Chemical and Biological Engineering, Guilin University of Technology, Guilin, Guangxi 541004, China

Corresponding author: Peipei ZHANG, 2421076309@qq.com Shuqin LIU, shuqinliu@163.com Jianjun ZHANG, zhangjj@dlut.edu.cn
Received Date: 17 April 2024
Revised Date: 21 June 2024

Figures(3)

A 1D coordination polymer (CP), (TBA) [Bi(bp4do)Br₄] (1), was synthesized by the assembly of 4, 4' - bipyridine -N, N'-dioxide (bp4do) and Bi³⁺ (TBA⁺=tetrabutylammonium). 1 exhibits a red luminescence with a quantum yield of up to 69%. A solid-state thin-film sensor (1/PVP) with extremely high luminescence stability was prepared by combining 1 with polyvinyl pyrrolidone (PVP). 1/PVP has a wide - range sensing capability for 11 NH₃/amine vapors with rapid response. During the sensing process, its luminescence color changed from red to blue, which was easy for naked -eye observation. The sensing mechanism is NH₃/amine-induced collapse of the framework of 1. Furthermore, 1/PVP has been successfully applied to monitoring food freshness such as meat/aquatic products.
- coordination polymer,
- solid state thin-film sensor,
- luminescence,
- bioamine,
- vapor sensing
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沈阳化工大学材料科学与工程学院沈阳 110142