Citation: Qingyan JIANG, Yanyong SHA, Chen CHEN, Xiaojuan CHEN, Wenlong LIU, Hao HUANG, Hongjiang LIU, Qi LIU. Constructing a one-dimensional Cu-coordination polymer-based cathode material for Li-ion batteries[J]. Chinese Journal of Inorganic Chemistry, ;2024, 40(4): 657-668. doi: 10.11862/CJIC.20240004 shu

Constructing a one-dimensional Cu-coordination polymer-based cathode material for Li-ion batteries

1.
Jiangsu Provincial Key Laboratory of Fine Petrochemicals, School of Petrochemical Engineering, Changzhou University, Changzhou, Jiangsu 213164, China
2.
Department of Chemistry, College of Science, Shanghai University, Shanghai 200444, China
3.
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, Jiangsu 225009, China

Corresponding author: Qi LIU, liuqi62@163.com
Received Date: 3 January 2024
Revised Date: 1 March 2024

Figures(9)

A novel one-dimensional (1D) polycarbonyl coordination polymer [Cu(BGPD)(DMA)(H₂O)]·DMA (named Cu-BD, H₂BGPD=N, N′-bis(glycinyl)pyromellitic diimide; DMA=dimethylacetamide) was synthesized, and evaluated as a cathode material for lithium - ion batteries (LIBs) for the first time. The electrochemical performance study revealed that the Cu-BD cathode exhibited better cycling stability and a specific capacity of 50 mAh·g^-1 after 100 cycles at a current density of 50 mA·g^-1. The study of the reaction mechanism for the Cu-BD electrode discloses that both BGPD^2- ligands and Cu(Ⅱ) ions may take part in the electron-transfer process during charging and discharging.
- Cu(Ⅱ),
- coordination polymer,
- carbonyl compound,
- lithium-ion battery,
- electrode material
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沈阳化工大学材料科学与工程学院沈阳 110142