Citation: Wenda WANG, Jinku MA, Yuzhu WEI, Shuaishuai MA. Waste biomass-derived carbon modified porous graphite carbon nitride heterojunction for efficient photodegradation of oxytetracycline in seawater[J]. Chinese Journal of Inorganic Chemistry, ;2024, 40(4): 809-822. doi: 10.11862/CJIC.20230353 shu

Waste biomass-derived carbon modified porous graphite carbon nitride heterojunction for efficient photodegradation of oxytetracycline in seawater

1.
School of Chemistry and Chemical Engineering, Jiangsu University of Technology, Changzhou, Jiangsu 213001, China
2.
College of Resources and Environmental Engineering, Jiangsu University of Technology, Changzhou, Jiangsu 213001, China

Corresponding author: Shuaishuai MA, machem@jsut.edu.cn
Received Date: 25 September 2023
Revised Date: 24 January 2024

Figures(12)

A metal - free photocatalyst was developed and synthesized through a single - step thermal treatment process involving banana peel (BP) and urea. The close interfacial connection between biomass-derived carbon (BC) and porous graphite carbon nitride (pg - C₃N₄) resulted in an increased specific surface area, expanded photo-response range, effective migration of photo-induced electrons, and enhanced stability. The reaction rate constant of pg-C₃N₄/BC for degradation oxytetracycline (OTC) in artificial seawater was 9.4 times higher than that of pristine pg-C₃N₄ after 70 min of visible-light illumination, and pg-C₃N₄/BC also performed better photocatalytic degradation on OTC in the continuous flow reaction process owing to facilitated photogenerated charge separation and transfer. Additionally, a potential photocatalytic mechanism was proposed to explain the enhanced performance of pg-C₃N₄/BC composites.
- g-C₃N₄,
- biomass carbon,
- seawater,
- photocatalysis,
- antibiotic
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