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Citation: Rui GAO, Zhen-Yu WANG, Lu WANG, Peng CHEN, Sheng LIU, Zhi-Peng MA, Guang-Jie SHAO. Ni2P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries[J]. Chinese Journal of Inorganic Chemistry, ;2022, 38(4): 685-694. doi: 10.11862/CJIC.2022.070 shu

Ni2P Nanosheets on Graphene as Sulfur-Based Composite Cathode Material for Lithium-Sulfur Batteries

  • 1.

    College of Environmental and Chemical Engineering, Yanshan University, Qinhuangdao, Hebei 066004, China

  • 2.

    School of Materials Science and Engineering, Nankai University, Tianjin 300350, China

Figures(5)

  • In this work, nickel phosphide (Ni2P) nanosheets were dispersed uniformly on graphene (G) to fabricate the Ni2P/G composite. Furthermore, the S/Ni2P/G sulfur-based composite was prepared further for lithium-sulfur batteries. Due to the strong chemical absorbability and high electrocatalytic activity of Ni2P nanosheets towards soluble polysulfides, S/Ni2P/G composite showed superior electrochemical performance. In particular, under the condition of high sulfur content (80.3%) and low electrolyte usage (15 μL·mg-1), S/Ni2P/G composite delivered a high initial specific discharge capacity of 1 164.7 mAh·g-1 and good cycling stability. In addition, due to the high tap density of 1.02 g·cm-3, S/Ni2P/G composite showed a high volumetric capacity of 954.0 mAh·cm-3, almost 1.6 times of that for S/G composite.
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