Citation: Jie YANG, Zhen-Hua LI, Wei FENG, Fu-You LI. Checking of Non-radiative Energy Transfer Process in Nanocrystal Self-Assembly Structure[J]. Chinese Journal of Inorganic Chemistry, ;2021, 37(12): 2158-2166. doi: 10.11862/CJIC.2021.252 shu

Checking of Non-radiative Energy Transfer Process in Nanocrystal Self-Assembly Structure

Department of Chemistry, Fudan University, Shanghai 200433, China

Corresponding author: Wei FENG, fengweifd@fudan.edu.cn Fu-You LI, fyli@fudan.edu.cn
Received Date: 14 May 2021
Revised Date: 28 September 2021

Figures(6)

Upconversion nanoparticles NaYF₄: 20%Yb, 2%Er@NaYF₄ (marked as UCNP) and gold nanoparticles (AuNP) were used as donors and acceptors to study non-radiative energy transfer in an assembly structure with a defined position relationship. Using UCNP and AuNP as basic building units, two-dimensional UCNP monolayer with large area and regular arrangement were self-assembled by solvent evaporation method at liquid-air interface. UCNP+AuNP bilayer and UCNP+NaYF₄+AuNP trilayer structures were prepared by layer-by-layer assembly. Then the luminescent properties of self-assembled films were characterized by the spectral imager system which was designed by our group. The spectrum of three kinds of films were compared. It was found that the luminescence attenuation of UCNP+AuNP bilayer structure and UCNP+NaYF₄+AuNP trilayer structure were similar, compared with UCNP monolayer. That is, there is no obvious non-radiative energy transfer between UCNP and AuNP in our research system. In the research, a well-geometric assembly model was provided, and the luminescence test equipment was set up, and it was verified that there was no non-radiative energy transfer between UCNP and AuNP in our self-assembly models.
- upconversion nanoparticle,
- nanocrystal self-assembly structure,
- energy transfer
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