Citation: Lao-bang WANG, Ji-jiang WANG, Er-lin YUE, Long TANG, Xiao WANG, Xiang-yang HOU, Yu-qi ZHANG. Synthesis, Structure, Magnetic and Photocatalytic Properties of Nickel(Ⅱ) Coordination Polymer Based on 1-(3,5-Dicarboxybenzyl)-1H-pyrazole-3,5-dicarboxylic Acid Ligand[J]. Chinese Journal of Inorganic Chemistry, ;2021, 37(4): 744-750. doi: 10.11862/CJIC.2021.089 shu

Synthesis, Structure, Magnetic and Photocatalytic Properties of Nickel(Ⅱ) Coordination Polymer Based on 1-(3,5-Dicarboxybenzyl)-1H-pyrazole-3,5-dicarboxylic Acid Ligand

Yan′an City Key Laboratory of New Energy & New Functional Materials, Shaanxi Key Laboratory of Chemical Reaction Engineering, College of Chemistry and Chemical Engineering, Yan′an University, Yan′an, Shannxi 716000, China

Corresponding author: Ji-jiang WANG, yadxwjj@126.com Er-lin YUE, yueerlin@yau.edu.com
Received Date: 17 September 2020
Revised Date: 30 January 2021

Figures(12)

A new coordination polymer {[Ni₂(L)(bib)_1.5(H₂O)₄]·3H₂O}_n (1)(H₄L=1-(3,5-dicarboxybenzyl)-1H-pyrazole-3,5-dicarboxylic acid, bib=1,4-bis(1-imidazolyl)benzene) was synthesized by hydrothermal method and characterized by single-crystal X-ray diffraction, elemental analyses and thermogravimetric analysis. Complex 1 features a 3D network structure. The variable temperature magnetic susceptibility measurements reveal that there are antiferromagnetic interactions between the Ni(Ⅱ) ions in complex 1. In addition, photocatalytic experiments indicated that complex 1 exhibited high photocatalytic activity up to 82.7% for the degradation of methylene blue pollutant.CCDC: 2030837.
- coordination polymer,
- Ni(Ⅱ),
- 1-(3,5-dicarboxybenzyl)-3,5-pyrazole dicarboxylic acid,
- magnetic property,
- photocatalytic properties
1. [1]
  Furukawa H, Cordova K E, Yaghi O M, O'Keeffe M. Science, 2013, 341(6149): 1230444
2. [2]
  Wang C, Liu D M, Lin W B. J. Am. Chem. Soc. , 2013, 135(36): 13222-13234 doi: 10.1021/ja308229p
3. [3]
  Li J R, Kuppler R J, Zhou H C. Chem. Soc. Rev. , 2009, 38: 1477-1504
4. [4]
  Cui Y, Qian G, Chen B, Yue Y. Chem. Rev. , 2012, 112(2): 1126-1162
5. [5]
  Kreno L E, Allendorf M, Hupp J T, Leong K, Farha O K. Chem. Rev. , 2012, 112(2): 1105-1125 doi: 10.1021/cr200324t
6. [6]
  Horcajada P, Gref R, Serre C, Baati T, Allan P K, Maurin G, Couvreur P, Morris R E, Férey G. Chem. Rev. , 2012, 112(2): 1232-1268
7. [7]
  Bavykina A, Kolobov N, Gascon J, Khan I S, Bau J A. Chem. Rev. , 2020, 120(16): 8468-8535
8. [8]
  Thorarinsdottir A E, Harris T D. Chem. Rev. , 2020, 120(16): 8716-8789
9. [9]
  Wang H H, Yang H Y, Shu C H, Chen Z Y, Hou L, Wang Y Y. Cryst. Growth Des. , 2016, 16(9): 5394-5402
10. [10]
  Lim D W, Kitagawa H. Chem. Rev. , 2020, 120(16): 8416-8467
11. [11]
  Xu Z Q, Meng W, Li H J, Hou H M, Fan Y T. Inorg. Chem. , 2014, 53(7): 3260-3262
12. [12]
  Paul A, Zangrando E, Patra A, Mahish M K, Saren D, Manna S C. Cryst. Growth Des. , 2020, 20(4): 2904-2913
13. [13]
  Zhu X, Sun P P, Ding J G, Li B L, Li H Y. Cryst. Growth Des. , 2012, 12(8): 3992-3997
14. [14]
  Sun J, Shang K X, Wu Y J, Zhang Q, Yao X Q, Yang Y X, Hu D C, Liu J C. Polyhedron, 2018, 141: 223-229
15. [15]
  Zheng B, Luo J H, Wang F, Peng Y, Li G H, Huo Q S, Liu Y L. Cryst. Growth Des. , 2013, 13(3): 1033-1044
16. [16]
  Dong X Y, Si C D, Liu J C, Fan Y, Hu D C, Yao X Q, Yang Y X. Cryst. Growth Des. , 2016, 16(4): 2062-2073
17. [17]
  Liu H, Kang Y F, Fan Y P, Guo F S, Liu L, Li J L, Liu P, Wang Y Y. Cryst. Growth Des. , 2019, 19(2): 797-807
18. [18]
  WANG J J, HOU X Y, GAO L J, ZHANG M L, REN Y X, FU F. Chinese J. Inorg. Chem. , 2014, 30(2): 379-383
19. [19]
  WANG J J, HOU X Y, GAO L J, ZHANG M L, REN Y X, FU F. Chinese J. Inorg. Chem. , 2014, 30(7): 1616-1620
20. [20]
  ZHANG M L, WANG J J, REN Y X. Chinese J. Inorg. Chem. , 2014, 30(11): 2477-2483
21. [21]
  Tang L, Jing R, Wang J J, Fu F. Chin. J. Struct. Chem. , 2017, 36(7): 1179-1184
22. [22]
  TANG L, FU Y H, WANG Y T, WANG H H, WANG J J, HOU X Y, WANG X. Chinese J. Inorg. Chem. , 2020, 36(8): 1550-1556
23. [23]
  Chen X L, Cui H L, Wang J J, Yang H, Wang X, Liu L, Ren Y X. CrystEngComm, 2019, 21: 7389-7406
24. [24]
  Sheldrick G M. SADABS, a Program for Empirical Absorption Correction of Area Detector Data, University of Göttingen, Germany, 2008.
25. [25]
  Sheldrick G M. Acta Crystallogr. Sect. A, 2015, A71: 3-8
26. [26]
  Sheldrick G M. Acta Crystallogr. Sect. C, 2015, C71: 3-8
27. [27]
  Cepeda J, Rodríguez Diéguez A. CrystEngComm, 2016, 18: 8556-8573
28. [28]
  Wang L N, Fu L, Zhu J W, Xu Y, Zhang M, You Q, Wang P, Qin J. Acta Chim. Slov. , 2017, 64(1): 202-207
29. [29]
  Qiao Y, Zhou Y F, Guan W S, Liu L H, Liu B, Che G B, Liu C B, Zhu E W. Inorg. Chim. Acta, 2017, 466: 291-297
30. [30]
  Choi W, Hong S J, Chang Y S, Cho Y. Environ. Sci. Technol. , 2000, 34(22): 4810-4815
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