Citation: SHI Wei-Long, YANG Shuang, WANG Jing-Bo, LIN Xue, GUO Feng, SHI Jun-You. Construction of MoS₂/Tubular-like g-C₃N₄ Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater[J]. Chinese Journal of Inorganic Chemistry, ;2020, 36(8): 1582-1592. doi: 10.11862/CJIC.2020.168 shu

Construction of MoS₂/Tubular-like g-C₃N₄ Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater

SHI Wei-Long ^1,2,# ,
YANG Shuang ^1,# ,
WANG Jing-Bo ¹ ,
LIN Xue ^1,, ,
GUO Feng ^3,, ,
SHI Jun-You ^1,,

1.
School of Material Science and Engineering, Beihua University, Jilin, Jilin 132013, China
2.
School of Material Science and Engineering, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212003, China
3.
School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang, Jiangsu 212013, China

Corresponding author: LIN Xue, jlsdlinxue@126.com GUO Feng, gfeng0105@126.com SHI Jun-You, bhsjy64@163.com
Received Date: 24 March 2020
Revised Date: 14 May 2020

Figures(9)

In this work, the development of efficient and stable photocatalyst has been the central topic of scientific research. Herein, MoS₂ nanosheets/tubular-like g-C₃N₄ (MS/TCN) composite photocatalysts with two dimension/one dimension (2D/1D) nanostructure were fabricated through a facile solvothermal method for photocatalytic hydrogen production from seawater under visible light irradiation, exhibiting enhanced photocatalytic performance in comparison of single MS or TCN. Among of them, MS/TCN-0.5 sample (0.5%(w/w) MoS₂) showed optimum H₂ evolution rate of 85.1 μmol·h^-1 and possessed outstanding stability (no significant decrease after 4 cycles). The enhanced photocatalytic activity of MS/TCN composite photocatalyst can be attributed to the fact that the loading of 2D MS, as a cocatalyst, promotes the transfer of photo-induced electron and improves the separation efficiency of electron-hole pairs of 1D TCN.
- photocatalysis,
- hydrogen production,
- carbon nitride,
- molybdenum disulfide
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通讯作者: 陈斌, bchen63@163.com

Construction of MoS₂/Tubular-like g-C₃N₄ Composite Photocatalyst for Improved Visible-Light Photocatalytic Hydrogen Production from Seawater