Citation: TAN Jie, LI Zhi-Feng, YANG Xiao-Fei, LI Jie, ZHANG Ting-Ting. Effect of Dry and Wet Environment of Ball Milling on Visible Light Catalytic Performance of Sulfur-Doped Carbon Nitride[J]. Chinese Journal of Inorganic Chemistry, ;2020, 36(3): 475-484. doi: 10.11862/CJIC.2020.052 shu

Effect of Dry and Wet Environment of Ball Milling on Visible Light Catalytic Performance of Sulfur-Doped Carbon Nitride

TAN Jie ¹ ,
LI Zhi-Feng ¹ ,
YANG Xiao-Fei ¹ ,
LI Jie ¹ ,
ZHANG Ting-Ting ^1,2,,

1.
College of Chemical Engineering, Beijing University of Chemical Technology, Beijing 100029, China
2.
Beijing Centre for Resource and Environmental Research, Beijing 100029, China

Corresponding author: ZHANG Ting-Ting, zhangtt@mail.buct.edu.cn
Received Date: 16 October 2019
Revised Date: 24 December 2019

Figures(10)

The photocatalytic activity of in situ sulfur-doped g-C₃N₄ was improved by simple and green ball milling using thiourea as raw material. Its structure and optical properties were characterized by X-ray diffraction, scanning electron microscope, elemental analysis, X-ray photoelectron spectroscopy, UV-Vis diffuse reflectance spectroscopy and photoluminescence spectroscopy. The visible light photocatalytic performance of ball milled sulfur-doped g-C₃N₄ photocatalyst at different solvent ratios was evaluated with methylene blue as the target pollutant. The results show that the specific surface area and the number of reactive sites of the sulfur-doped g-C₃N₄ photocatalyst after wet ball milling are increased, and the band gap also increased appropriately, resulting in enhanced redox capacity. In addition, the surface defects of the sample after wet ball milling were reduced and the degree of polymerization was increased, which promoted the effective separation and transfer of photogenerated electron-holes. Therefore, the recombination rate can be lowered, and the degradation performance of the sulfur-doped g-C₃N₄ photocatalyst improved synergistically. The degradation rate of methylene blue in the wet ball milled sample was 1.5 and 3.6 times higher than that of the without ball milled sample and the dry ball milled sample, respectively.
- carbon nitride,
- sulfur doping,
- ball milling,
- visible light photocatalysis
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