Citation: ZHANG Hong-Liang, LONG Hong-Ming, LI Jia-Xin, DONG Lin. Research Progress in Iron-Based Catalysts for the Selective Catalytic Reduction of NO_x by NH₃[J]. Chinese Journal of Inorganic Chemistry, ;2019, 35(5): 753-768. doi: 10.11862/CJIC.2019.099 shu

Research Progress in Iron-Based Catalysts for the Selective Catalytic Reduction of NO_x by NH₃

ZHANG Hong-Liang ^1,2,3 ,
LONG Hong-Ming ^2,3,, ,
LI Jia-Xin ^2,3,, ,
DONG Lin ⁴

1.
Analysis and Testing Central Facility, Anhui University of Technology, Ma'anshan, Anhui 243002, China
2.
School of Metallurgical Engineering, Anhui University of Technology, Ma'anshan, Anhui 243032, China
3.
Key Laboratory of Metallurgical Emission Reduction & Resources Recycling(Anhui University of Technology), Ministry of Education, Ma'anshan, Anhui 243002, China
4.
Jiangsu Key Laboratory of Vehicle Emissions Control, Nanjing University, Nanjing 210093, China

Corresponding author: LONG Hong-Ming, yaflhm@126.com LI Jia-Xin, lijx@ahut.edu.cn
Received Date: 25 December 2018
Revised Date: 26 February 2019

Figures(12)

Selective catalytic reduction of NO_x with NH₃ is a powerful technique for the abatement of NO_x. The operating temperature window of commercial V₂O₅-WO₃(MoO₃)/TiO₂ denitration catalysts is too high to satisfy the requirements of low temperature and wide operating temperature window, and therefore the development of low-temperature denitration catalysts with wide operating temperature window becomes a hot spot of this research field in recent years. Iron-based catalysts are widely used in the low-temperature NH₃-selective catalytic reduction (NH₃-SCR) of NO_x because of their good redox ability, rich resource reserves, low-cost, non-toxic and harmlessness, etc.. Based on the different roles of Fe₂O₃ in NH₃-SCR catalysts, we have performed a systematic review of the latest research progress of iron-based catalysts in the NH₃-SCR reaction for the following aspects:Fe₂O₃ used as support, promoter, active species, and iron-based catalysts with new structures. In addition, the NH₃-SCR reaction mechanism and H₂O/SO₂ tolerance over iron-based catalysts are emphasized. Finally, the perspectives on the opportunities and challenges of iron-based catalysts for NH₃-SCR in future research are presented.
- iron,
- selective catalytic reduction,
- nitrogen oxides,
- flue gas denitration,
- structure-activity relationships
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沈阳化工大学材料科学与工程学院沈阳 110142

Research Progress in Iron-Based Catalysts for the Selective Catalytic Reduction of NOx by NH3

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通讯作者: 陈斌, bchen63@163.com

Research Progress in Iron-Based Catalysts for the Selective Catalytic Reduction of NO_x by NH₃