Citation: WANG Qi-Chen, WANG Jing, LEI Yong-Peng, CHEN Zhi-Yan, SONG Yao, LUO Shi-Bin. Research Progress on Carbon Nanotubes in Noble-Metal-Free Electrocatalytic Oxygen Reduction Reaction[J]. Chinese Journal of Inorganic Chemistry, ;2018, 34(5): 807-822. doi: 10.11862/CJIC.2018.101 shu

Research Progress on Carbon Nanotubes in Noble-Metal-Free Electrocatalytic Oxygen Reduction Reaction

WANG Qi-Chen ^1,3,5 ,
WANG Jing ² ,
LEI Yong-Peng ^1,4,, ,
CHEN Zhi-Yan ⁶ ,
SONG Yao ⁶ ,
LUO Shi-Bin ^1,,

1.
School of Aeronautics and Astronautics, Central South University & Science and Technology on High Strength Structural Materials Laboratory, Changsha 410083, China
2.
College of Science, National University of Defense Technology, Changsha 410073, China
3.
The State Key Laboratory of Refractories and Metallurgy, Wuhan University of Science and Technology, Wuhan 430081, China
4.
College of Basic Education, National University of Defense Technology, Changsha 410073, China
5.
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China
6.
College of Materials Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, China

Corresponding author: LEI Yong-Peng, lypkd@163.com LUO Shi-Bin, luoshibin@csu.edu.cn
Received Date: 8 December 2017
Revised Date: 18 January 2018

Figures(10)

Fuel cell and metal-air batteries are green batteries which directly convert chemical energy into electricity, possessing important merits compared to the traditional energy, examples of high energy density, safety and environmental benignity. However, the low reserves, high cost, easy poisoning and deactivation of precious metal platinum (Pt) used in cathodic oxygen reduction reactions (ORR) have severely limited the development of the fuel cell in large-scale. Therefore, the research on development of cheap, efficient and stable non-precious metal catalyst has become a hotspot. Carbon nanotubes (CNTs), owning to the outstanding feature such as the intrisic sp² hybrid structure, excellent conductivity, high specific surface area, good chemical stability, etc, have received wide attentions. Firstly, the recent progress in the noble-metal-free CNTs-based ORR catalysts were summarized, mainly including non-metal element doping, transition metal-nitrogen-CNTs, CNTs supported transition metals and their derivations (oxides, carbides, nitrides, sulfides, etc), CNTs supported single atoms, composited with other carbon materials (graphene, porous carbon, carbon nanofibers) and self-standing electrodes based on CNTs. Finally, the prospect and the future research direction of CNTs-based ORR catalysts are also discussed.
- carbon nanotubes,
- fuel cell,
- oxygen reduction,
- noble-metal-free catalysts,
- composites,
- single atom
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沈阳化工大学材料科学与工程学院沈阳 110142