Citation: BAI Yu, ZENG De-Bin, LIU Ren-Yue, LI Shao-Yu, YANG Kai, HUANG Wei-Ya, YU Chang-Lin. Three-Dimensional Dendritic C/PbWO₄ Catalysts: Preparation and Photocatalytic Performance in Degrading Different Dyes[J]. Chinese Journal of Inorganic Chemistry, ;2018, 34(4): 669-675. doi: 10.11862/CJIC.2018.089 shu

Three-Dimensional Dendritic C/PbWO₄ Catalysts: Preparation and Photocatalytic Performance in Degrading Different Dyes

BAI Yu ¹ ,
ZENG De-Bin ¹ ,
LIU Ren-Yue ¹ ,
LI Shao-Yu ¹ ,
YANG Kai ¹ ,
HUANG Wei-Ya ¹ ,
YU Chang-Lin ^1,2,,

1.
School of Metallurgy and Chemical Engineering, Jiangxi University of Science and Technology, Ganzhou, Jiangxi 341000, China
2.
State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou 350002, China

Corresponding author: YU Chang-Lin, yuchanglinjx@163.com
Received Date: 3 November 2017
Revised Date: 22 January 2018

Figures(8)

Three-dimensional dendritic C/PbWO₄ composite photocatalyst with different C content (Mass fraction=0.13%, 0.26%, 0.52%, 0.78%) was synthesized by a hydrothermal method. The photocatalysts were characterized by X-ray diffraction, N₂ sorption measurements, scanning electron microscopy, transmission electron microscopy, energy dispersive X-ray spectroscopy, ultraviolet-visible diffuse reflectance spectroscopies, photoluminescence, and photoelectrochemical measurement. The results showed that the dendritic C/PbWO₄ composite photocatalyst with 0.52% C exhibits the best photocatalytic performance in degrading orange Ⅱ, methyl orange and rhodamine B. Under the light irradiation for 100 min, the degradation rate of the acid orange Ⅱ (20 mg·L^-1) over 0.52% C/PbWO₄ reached 97% which was about 2.48 times as that of bare PbWO₄. The main reason for the increase of activity is that carbon attached to the surface of the catalyst becomes the electron trapping center, and it can effectively capture the photogenerated electrons. Therefore, the photo-generated electron-hole pairs were effectively separated to produce more active species (·OH, h⁺) to participate in the degradation of organic dye molecules.
- dendritic-like,
- PbWO₄,
- carbon-doping,
- organic dyes,
- composite photocatalyst
1. [1]
  Li K, Peng B S, Peng T Y. ACS Catal., 2016, 6:7485-7527 doi: 10.1021/acscatal.6b02089
2. [2]
  DONG Wei-Xia, BAO Qi-Fu, GU Xin-Yong, et al. Chinese J. Inorg. Chem., 2017, 33(2):292-298
3. [3]
  HE Hong-Bo, XUE Shuang-Shuang, YU Chang-Lin, et al. Chinese J. Inorg. Chem., 2016, 32(4):625-632
4. [4]
  LIU Ren-Yue, WU Zhen, BAI Yu, et al. Chinese J. Inorg. Chem., 2017, 33(3):519-527
5. [5]
  He H B, Xue S S, Wu Z, et al. Chin. J. Catal., 2016, 37(11):1841-1580 doi: 10.1016/S1872-2067(16)62515-9
6. [6]
  Yu C L, Zhou W Q, Yu J C, et al. Chin. J. Catal., 2014, 35(10):1609-1618 doi: 10.1016/S1872-2067(14)60170-4
7. [7]
  Barth J V, Costantini G, Kern K. Nanoscience and Technology: A Collection of Reviews from Nature Journals. Rodgers P. Ed., Singapore: World Scientific Publishing Company, 2014: 67-75
8. [8]
  Yue D, Chen D, Lu W, et al. RSC Adv., 2016, 6:81447-81453 doi: 10.1039/C6RA15045D
9. [9]
  ČErnýP, JelNková H, Zverev P G, et al. Prog. Quantum Electron., 2004, 28(2):113-143 doi: 10.1016/j.pquantelec.2003.09.003
10. [10]
  Angloher G, Bruckmayer M, Bucci C, et al. Astropart. Phys., 2002, 18(1):43-55 doi: 10.1016/S0927-6505(02)00111-1
11. [11]
  Sundaram R, Nagaraja K S. Mater. Res. Bull., 2004, 39(4):581-590
12. [12]
  Yu C L, Bai Y, He H B, et al. Chin. J. Catal., 2015, 36(12):2178-2185 doi: 10.1016/S1872-2067(15)61009-9
13. [13]
  Liu B, Yu S H, Li L, et al. Angew. Chem. Int. Ed., 2004, 43(36):4745-4750 doi: 10.1002/(ISSN)1521-3773
14. [14]
  Wang W, Lee S, Piao H, et al. CrystEngComm, 2015, 17(34):6548-6554 doi: 10.1039/C5CE00749F
15. [15]
  Zhang C M, Zhang J Y, Li Y S, et al. J. Alloys Compd., 2017, 698:33-38 doi: 10.1016/j.jallcom.2016.12.132
16. [16]
  Bailón-García E, Elmouwahidi A, Carrasco-Marín F, et al. Appl. Catal. B, 2017, 217:540-550 doi: 10.1016/j.apcatb.2017.05.090
17. [17]
  Chen Q C, Wu Q S. Catal. Commun., 2012, 24(26):85-89
18. [18]
  Liu C L, Cai Q, Zhang L, et al. Catal. Commun., 2017, 99:71-74 doi: 10.1016/j.catcom.2017.04.040
19. [19]
  Yu C L, Zhou W Q, Yang K, et al. J. Mater. Sci., 2010, 45(21):5756-5761 doi: 10.1007/s10853-010-4646-6
20. [20]
  Long J L, Wang S C, Chang H J, et al. Small, 2014, 10(14):2791-2795 doi: 10.1002/smll.201302950
21. [21]
  Meng H, Li X X, Zhang X, et al. Dalton Trans., 2015, 44(46):19948-19955 doi: 10.1039/C5DT03869C
22. [22]
  Kwolek P, Pilarczyk K, Tokarski T, et al. J. Mater. Chem. C, 2015, 3(11):2614-2623 doi: 10.1039/C4TC02750G
23. [23]
  Hao S Y, Ma X G, Cui G H. Ultrason. Sonochem., 2017, 37:414-423 doi: 10.1016/j.ultsonch.2017.01.027
1. [1]
  Wei Zhong , Dan Zheng , Yuanxin Ou , Aiyun Meng , Yaorong Su . K原子掺杂高度面间结晶的g-C₃N₄光催化剂及其高效H₂O₂光合成. Acta Physico-Chimica Sinica, 2024, 40(11): 2406005-. doi: 10.3866/PKU.WHXB202406005
2. [2]
  Yi YANG , Shuang WANG , Wendan WANG , Limiao CHEN . Photocatalytic CO₂ reduction performance of Z-scheme Ag-Cu₂O/BiVO₄ photocatalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 895-906. doi: 10.11862/CJIC.20230434
3. [3]
  Jingzhao Cheng , Shiyu Gao , Bei Cheng , Kai Yang , Wang Wang , Shaowen Cao . 4-氨基-1H-咪唑-5-甲腈修饰供体-受体型氮化碳光催化剂的构建及其高效光催化产氢研究. Acta Physico-Chimica Sinica, 2024, 40(11): 2406026-. doi: 10.3866/PKU.WHXB202406026
4. [4]
  Kai CHEN , Fengshun WU , Shun XIAO , Jinbao ZHANG , Lihua ZHU . PtRu/nitrogen-doped carbon for electrocatalytic methanol oxidation and hydrogen evolution by water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1357-1367. doi: 10.11862/CJIC.20230350
5. [5]
  Ke Li , Chuang Liu , Jingping Li , Guohong Wang , Kai Wang . 钛酸铋/氮化碳无机有机复合S型异质结纯水光催化产过氧化氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2403009-. doi: 10.3866/PKU.WHXB202403009
6. [6]
  Hailang JIA , Hongcheng LI , Pengcheng JI , Yang TENG , Mingyun GUAN . Preparation and performance of N-doped carbon nanotubes composite Co₃O₄ as oxygen reduction reaction electrocatalysts. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 693-700. doi: 10.11862/CJIC.20230402
7. [7]
  Wenxiu Yang , Jinfeng Zhang , Quanlong Xu , Yun Yang , Lijie Zhang . Bimetallic AuCu Alloy Decorated Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312014-. doi: 10.3866/PKU.WHXB202312014
8. [8]
  Jinyi Sun , Lin Ma , Yanjie Xi , Jing Wang . Preparation and Electrocatalytic Nitrogen Reduction Performance Study of Vanadium Nitride@Nitrogen-Doped Carbon Composite Nanomaterials: A Recommended Comprehensive Chemistry Experiment. University Chemistry, 2024, 39(4): 184-191. doi: 10.3866/PKU.DXHX202310094
9. [9]
  Kaihui Huang , Dejun Chen , Xin Zhang , Rongchen Shen , Peng Zhang , Difa Xu , Xin Li . Constructing Covalent Triazine Frameworks/N-Doped Carbon-Coated Cu₂O S-Scheme Heterojunctions for Boosting Photocatalytic Hydrogen Production. Acta Physico-Chimica Sinica, 2024, 40(12): 2407020-. doi: 10.3866/PKU.WHXB202407020
10. [10]
  Juntao Yan , Liang Wei . 2D S-Scheme Heterojunction Photocatalyst. Acta Physico-Chimica Sinica, 2024, 40(10): 2312024-. doi: 10.3866/PKU.WHXB202312024
11. [11]
  Yuanyin Cui , Jinfeng Zhang , Hailiang Chu , Lixian Sun , Kai Dai . Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion. Acta Physico-Chimica Sinica, 2024, 40(12): 2405016-. doi: 10.3866/PKU.WHXB202405016
12. [12]
  Wenlong LI , Xinyu JIA , Jie LING , Mengdan MA , Anning ZHOU . Photothermal catalytic CO₂ hydrogenation over a Mg-doped In₂O_3-x catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 919-929. doi: 10.11862/CJIC.20230421
13. [13]
  Yuanpei ZHANG , Jiahong WANG , Jinming HUANG , Zhi HU . Preparation of magnetic mesoporous carbon loaded nano zero-valent iron for removal of Cr(Ⅲ) organic complexes from high-salt wastewater. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1731-1742. doi: 10.11862/CJIC.20240077
14. [14]
  Asif Hassan Raza , Shumail Farhan , Zhixian Yu , Yan Wu . 用于高效制氢的双S型ZnS/ZnO/CdS异质结构光催化剂. Acta Physico-Chimica Sinica, 2024, 40(11): 2406020-. doi: 10.3866/PKU.WHXB202406020
15. [15]
  Zhiquan Zhang , Baker Rhimi , Zheyang Liu , Min Zhou , Guowei Deng , Wei Wei , Liang Mao , Huaming Li , Zhifeng Jiang . Insights into the Development of Copper-based Photocatalysts for CO₂ Conversion. Acta Physico-Chimica Sinica, 2024, 40(12): 2406029-. doi: 10.3866/PKU.WHXB202406029
16. [16]
  Ruolin CHENG , Haoran WANG , Jing REN , Yingying MA , Huagen LIANG . Efficient photocatalytic CO₂ cycloaddition over W₁₈O₄₉/NH₂-UiO-66 composite catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 523-532. doi: 10.11862/CJIC.20230349
17. [17]
  Qiangqiang SUN , Pengcheng ZHAO , Ruoyu WU , Baoyue CAO . Multistage microporous bifunctional catalyst constructed by P-doped nickel-based sulfide ultra-thin nanosheets for energy-efficient hydrogen production from water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1151-1161. doi: 10.11862/CJIC.20230454
18. [18]
  Kun WANG , Wenrui LIU , Peng JIANG , Yuhang SONG , Lihua CHEN , Zhao DENG . Hierarchical hollow structured BiOBr-Pt catalysts for photocatalytic CO₂ reduction. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1270-1278. doi: 10.11862/CJIC.20240037
19. [19]
  Qingqing SHEN , Xiangbowen DU , Kaicheng QIAN , Zhikang JIN , Zheng FANG , Tong WEI , Renhong LI . Self-supporting Cu/α-FeOOH/foam nickel composite catalyst for efficient hydrogen production by coupling methanol oxidation and water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1953-1964. doi: 10.11862/CJIC.20240028
20. [20]
  Zhaomei LIU , Wenshi ZHONG , Jiaxin LI , Gengshen HU . Preparation of nitrogen-doped porous carbons with ultra-high surface areas for high-performance supercapacitors. Chinese Journal of Inorganic Chemistry, 2024, 40(4): 677-685. doi: 10.11862/CJIC.20230404

Get Citation

PDF

XML

Metrics

PDF Downloads(6)
Abstract views(1292)
HTML views(260)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

Three-Dimensional Dendritic C/PbWO4 Catalysts: Preparation and Photocatalytic Performance in Degrading Different Dyes

Metrics

通讯作者: 陈斌, bchen63@163.com

Three-Dimensional Dendritic C/PbWO₄ Catalysts: Preparation and Photocatalytic Performance in Degrading Different Dyes