Advanced Search

Citation: ZHAO Di, ZHANG Bo, DUAN Zhao-Juan, LI Ai-Chang. Ag2S/Ag3PO4/Ni Thin Films: Preparation and Photocatalytic Activity for Rhodamine B[J]. Chinese Journal of Inorganic Chemistry, ;2016, 32(12): 2158-2164. doi: 10.11862/CJIC.2016.276 shu

Ag2S/Ag3PO4/Ni Thin Films: Preparation and Photocatalytic Activity for Rhodamine B

  • 1.

    Faculty of Chemistry and Material Science, Langfang Teachers College, Langfang, Hebei 065000, China

  • Corresponding author: LI Ai-Chang, 
  • Received Date: 28 July 2016
    Available Online: 8 October 2016

    Fund Project:

  • Ag2S/Ag3PO4/Ni composite thin films were prepared by electrochemical method. The surface morphology, phase structure, optical characteristics and band structure of the thin film were characterized by scanning electron microscopy (SEM), X-ray diffraction (XRD) and ultraviolet-visible diffuse reflectance spectroscopy (UV-Vis DRS), respectively. Its photocatalytic properties and stability were evaluated with rhodamine B (RhB) as a model compound. Using a method of adding active species scavenger to the solution, mechanism of photocatalytic degradation of the film was explored. The results show that the Ag2S/Ag3PO4/Ni thin film is composed of uniform spherical nanoparticles. The photocatalytic activity of the as-prepared Ag2S/Ag3PO4/Ni thin film was higher than those of pure Ag3PO4/Ni thin film and Ag2S/Ni thin film respectively. The film maintains nearly 100% of their corresponding initial photocatalytic activity after 6 cycles. Furthermore, the photodegradation mechanism of the composite films for RhB under the visible light was preliminary proposed.
  • 加载中
    1. [1]

      [1] Hoffmann M R, Martin S T, Choi W Y, et al. Chem. Rev., 1995,95(1):69-96

    2. [2]

      [2] Szabo-Bardos E, Zsilak Z, Horvath O. Prog. Colloid Polym. Sci., 2008,135:21-28

    3. [3]

      [3] Asahi R, Morikawa T, Ohwaki T, et al. Science, 2001,293:269-271

    4. [4]

      [4] Addamo M, Augugliaro V, Garc E, et al. Catal. Today, 2005, 107/108:612-618

    5. [5]

      [5] JIN Chao(金超), QIN Yao(秦瑶), YANG Jin-Hu(杨金虎). Prog. Chem.(化学进展), 2014,26(2/3):225-233

    6. [6]

      [6] YAN Xue-Hua(严学华), GAO Qing-Xia(高庆侠), YANG Xiao-Fei(杨小飞), et al. J. Chin. Ceram. Soc.(硅酸盐学报), 2013,10(41):1354-1365

    7. [7]

      [7] Martin D J, Liu G G, Moniz S J A, et al. Chem. Soc. Rev., 2015,44(50):7808-7828

    8. [8]

      [8] Zhang L L, Zhang H C, Liu Y, et al. New J. Chem., 2012,36(8):1541-1544

    9. [9]

      [9] Shen K, Gondal M A, Siddique R G, et al. Chin. J. Catal., 2014,5(1):78-84

    10. [10]

      [10] Yi Z G, Ye J H, Kikugawa N, et al. Nat. Mater., 2010,9(7):559-564

    11. [11]

      [11] Bi Y P, Hu H Y, Ye J H, et al. Chem. Commun., 2012,48(31):3748-3750

    12. [12]

      [12] Bi Y P, Ouyang S, Ye J H, et al. Phys. Chem. Chem. Phys., 2011,13(21):10071-10075

    13. [13]

      [13] ZHU Sui-Yi(朱遂一), XU Dong-Fang(徐东方), FANG Shuai (方帅), et al. Chem. J. Chinese Universities(高等学校化学学报), 2014,35(6):1286-1292

    14. [14]

      [14] Cao J, Luo B D, Lin H L, et al. J. Hazard. Mater., 2012,4(217/218):107-115

    15. [15]

      [15] Ma P Y, Yu H J, Yu Y, et al. Phys. Chem. Chem. Phys., 2016,18(5):3638-3643

    16. [16]

      [16] LI Ai-Chang(李爱昌), ZHAO Di(赵娣), LIU Pan-Pan(刘盼盼), et al. Chinese J. Nonferrous Met.(中国有色金属学报), 2015,25(8):2196-2204

    17. [17]

      [17] ZHAO Kai-Yuan(赵凯元), WANG Qing(王清). Phys. Test. Chem. Anal. Part B:Chem. Anal.(理化检验:化学分册), 2007,43(1):45-50

    18. [18]

      [18] LI Ai-Chang(李爱昌), ZHU Ning-Ning(朱拧拧),LI Jing-Hong(李京红), et al. Chinese J. Inorg. Chem.(无机化学学报), 2015,31(4):681-688

    19. [19]

      [19] Jiang D L, Chen L L, Xie J M, et al. Dalton Trans., 2014, 43:4878-4885

    20. [20]

      [20] LIU Jian-Xin(刘建新), WANG Yun-Fang(王韵芳), WANG Ya-Wen(王雅文), et al. Acta Phys.-Chim. Sin.(物理化学学报), 2014,30(4):729-737

    21. [21]

      [21] Tang J T, Gong W, Cai T J, et al. RSC Adv., 2013,3(8):2543-2547

  • 加载中
    1. [1]

      Ronghao Zhao ,  Yifan Liang ,  Mengyao Shi ,  Rongxiu Zhu ,  Dongju Zhang . Investigation into the Mechanism and Migratory Aptitude of Typical Pinacol Rearrangement Reactions: A Research-Oriented Computational Chemistry Experiment. University Chemistry, 2024, 39(4): 305-313. doi: 10.3866/PKU.DXHX202309101

    2. [2]

      Zhuo WANG , Junshan ZHANG , Shaoyan YANG , Lingyan ZHOU , Yedi LI , Yuanpei LAN . Preparation and photocatalytic performance of CeO2-reduced graphene oxide by thermal decomposition. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1708-1718. doi: 10.11862/CJIC.20240067

    3. [3]

      Ling Fan ,  Meili Pang ,  Yeyun Zhang ,  Yanmei Wang ,  Zhenfeng Shang . Quantum Chemistry Calculation Research on the Diels-Alder Reaction of Anthracene and Maleic Anhydride: Introduction to a Computational Chemistry Experiment. University Chemistry, 2024, 39(4): 133-139. doi: 10.3866/PKU.DXHX202309024

    4. [4]

      Xin Zhou ,  Zhi Zhang ,  Yun Yang ,  Shuijin Yang . A Study on the Enhancement of Photocatalytic Performance in C/Bi/Bi2MoO6 Composites by Ferroelectric Polarization: A Recommended Comprehensive Chemical Experiment. University Chemistry, 2024, 39(4): 296-304. doi: 10.3866/PKU.DXHX202310008

    5. [5]

      Heng Chen ,  Longhui Nie ,  Kai Xu ,  Yiqiong Yang ,  Caihong Fang . 两步焙烧法制备大比表面积和结晶性增强超薄g-C3N4纳米片及其高效光催化产H2O2. Acta Physico-Chimica Sinica, 2024, 40(11): 2406019-. doi: 10.3866/PKU.WHXB202406019

    6. [6]

      Kun WANG , Wenrui LIU , Peng JIANG , Yuhang SONG , Lihua CHEN , Zhao DENG . Hierarchical hollow structured BiOBr-Pt catalysts for photocatalytic CO2 reduction. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1270-1278. doi: 10.11862/CJIC.20240037

    7. [7]

      Jianyin He ,  Liuyun Chen ,  Xinling Xie ,  Zuzeng Qin ,  Hongbing Ji ,  Tongming Su . ZnCoP/CdLa2S4肖特基异质结的构建促进光催化产氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2404030-. doi: 10.3866/PKU.WHXB202404030

    8. [8]

      Xuejiao Wang ,  Suiying Dong ,  Kezhen Qi ,  Vadim Popkov ,  Xianglin Xiang . Photocatalytic CO2 Reduction by Modified g-C3N4. Acta Physico-Chimica Sinica, 2024, 40(12): 2408005-. doi: 10.3866/PKU.WHXB202408005

    9. [9]

      Zijian Jiang ,  Yuang Liu ,  Yijian Zong ,  Yong Fan ,  Wanchun Zhu ,  Yupeng Guo . Preparation of Nano Zinc Oxide by Microemulsion Method and Study on Its Photocatalytic Activity. University Chemistry, 2024, 39(5): 266-273. doi: 10.3866/PKU.DXHX202311101

    10. [10]

      Ruolin CHENG , Haoran WANG , Jing REN , Yingying MA , Huagen LIANG . Efficient photocatalytic CO2 cycloaddition over W18O49/NH2-UiO-66 composite catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 523-532. doi: 10.11862/CJIC.20230349

    11. [11]

      Jingyu Cai ,  Xiaoyu Miao ,  Yulai Zhao ,  Longqiang Xiao . Exploratory Teaching Experiment Design of FeOOH-RGO Aerogel for Photocatalytic Benzene to Phenol. University Chemistry, 2024, 39(4): 169-177. doi: 10.3866/PKU.DXHX202311028

    12. [12]

      Tong Zhou ,  Xue Liu ,  Liang Zhao ,  Mingtao Qiao ,  Wanying Lei . Efficient Photocatalytic H2O2 Production and Cr(VI) Reduction over a Hierarchical Ti3C2/In4SnS8 Schottky Junction. Acta Physico-Chimica Sinica, 2024, 40(10): 2309020-. doi: 10.3866/PKU.WHXB202309020

    13. [13]

      Guoqiang Chen ,  Zixuan Zheng ,  Wei Zhong ,  Guohong Wang ,  Xinhe Wu . 熔融中间体运输导向合成富氨基g-C3N4纳米片用于高效光催化产H2O2. Acta Physico-Chimica Sinica, 2024, 40(11): 2406021-. doi: 10.3866/PKU.WHXB202406021

    14. [14]

      Ke Li ,  Chuang Liu ,  Jingping Li ,  Guohong Wang ,  Kai Wang . 钛酸铋/氮化碳无机有机复合S型异质结纯水光催化产过氧化氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2403009-. doi: 10.3866/PKU.WHXB202403009

    15. [15]

      Qin Hu ,  Liuyun Chen ,  Xinling Xie ,  Zuzeng Qin ,  Hongbing Ji ,  Tongming Su . Ni掺杂构建电子桥及激活MoS2惰性基面增强光催化分解水产氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2406024-. doi: 10.3866/PKU.WHXB202406024

    16. [16]

      Shijie Li ,  Ke Rong ,  Xiaoqin Wang ,  Chuqi Shen ,  Fang Yang ,  Qinghong Zhang . Design of Carbon Quantum Dots/CdS/Ta3N5 S-Scheme Heterojunction Nanofibers for Efficient Photocatalytic Antibiotic Removal. Acta Physico-Chimica Sinica, 2024, 40(12): 2403005-. doi: 10.3866/PKU.WHXB202403005

    17. [17]

      Chenye An ,  Abiduweili Sikandaier ,  Xue Guo ,  Yukun Zhu ,  Hua Tang ,  Dongjiang Yang . 红磷纳米颗粒嵌入花状CeO2分级S型异质结高效光催化产氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2405019-. doi: 10.3866/PKU.WHXB202405019

    18. [18]

      Yong Wang ,  Yingying Zhao ,  Boshun Wan . Analysis of Organic Questions in the 37th Chinese Chemistry Olympiad (Preliminary). University Chemistry, 2024, 39(11): 406-416. doi: 10.12461/PKU.DXHX202403009

    19. [19]

      Yang Xia ,  Kangyan Zhang ,  Heng Yang ,  Lijuan Shi ,  Qun Yi . 构建双通道路径增强iCOF/Bi2O3 S型异质结在纯水体系中光催化合成H2O2性能. Acta Physico-Chimica Sinica, 2024, 40(11): 2407012-. doi: 10.3866/PKU.WHXB202407012

    20. [20]

      Xinyu Yin ,  Haiyang Shi ,  Yu Wang ,  Xuefei Wang ,  Ping Wang ,  Huogen Yu . Spontaneously Improved Adsorption of H2O and Its Intermediates on Electron-Deficient Mn(3+δ)+ for Efficient Photocatalytic H2O2 Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312007-. doi: 10.3866/PKU.WHXB202312007

Get Citation
PDF
XML
Metrics
  • PDF Downloads(0)
  • Abstract views(315)
  • HTML views(34)

通讯作者: 陈斌, bchen63@163.com
  • 1. 

    沈阳化工大学材料科学与工程学院 沈阳 110142

  1. 本站搜索
  2. 百度学术搜索
  3. 万方数据库搜索
  4. CNKI搜索
Address：Zhongguancun North First Street 2,100190 Beijing, PR China Tel: +86-010-82449177-888
Powered By info@rhhz.net

/

DownLoad:  Full-Size Img  PowerPoint
Return