Citation: Yuanyin Cui, Jinfeng Zhang, Hailiang Chu, Lixian Sun, Kai Dai. Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion[J]. Acta Physico-Chimica Sinica, ;2024, 40(12): 240501. doi: 10.3866/PKU.WHXB202405016 shu

Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion

Yuanyin Cui ^1,2 ,
Jinfeng Zhang ² ,
Hailiang Chu ^1,, ,
Lixian Sun ^1,, ,
Kai Dai ^2,,

1.
Guangxi Key Laboratory of Information Materials, Guangxi Collaborative Innovation Centre of Structure and Property for New Energy Materials, School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004, Guangxi Zhuang Autonomous Region, China;
2.
Anhui Province Key Laboratory of Pollutant Sensitive Materials and Environmental Remediation, School of Physics and Electronic Information, Huaibei Normal University, Huaibei 235000, Anhui Province, China

Corresponding author: Hailiang Chu, Lixian Sun, Kai Dai,
Received Date: 20 May 2024
Revised Date: 7 July 2024
Accepted Date: 8 July 2024

Fund Project: This work was supported by the National Natural Science Foundation of China (22278169, 51973078, 22179026), the Excellent Scientific Research and Innovation Team of Education Department of Anhui Province (2022AH010028), the Major Projects of Education Department of Anhui Province (2022AH040068), and Anhui Provincial Quality Engineering Project (2022sx134), the Innovation Platform and Talent Program Project of Guilin (20210102-4), the Guilin Lijiang Scholar Foundation and the Guangxi Bagui Scholar Foundation.

Semiconductor photocatalysis makes full use of solar energy, serving as a potent tactic to solve the worldwide energy deficit and safeguard the environment. Bismuth-based photocatalysts stand out among various photocatalysts as a significant area, due to their unique crystal structure, favorable mixed electron band structure, diverse composition, and huge potential for solar catalytic conversion. This document reviews the rational design of Bi-based photocatalysts for solar energy. Recent advancements in diverse Bi-based photocatalysts such as Layered Bi, Bismuth element, BiVO₄, Bi₂S₂, and Bi₂O₃ are highlighted. Secondly, the synthesis strategies of Bi-based catalysts, including hydrothermal/solvothermal, chemical precipitation, and solid-state reaction, are summarized. Third, various structural regulation methods to improve the photocatalytic performance, including defect regulation, heteroatom doping, morphology, SPR effect utilization, and heterojunction construction, are systematically introduced. Additionally, a focus is given to the exclusive applications of Bi-based photocatalysts, including CO₂ reduction, water decomposition, N₂ fixation, NO_x removal, H₂O₂ production, and selective organic synthesis, followed by an introduction of advanced in situ characterization techniques of the Bi-based photocatalysts. Ultimately, the forthcoming obstacles are underscored, and a future outlook for Bi-based photocatalysts is anticipated. This review aims to offer detailed instructions for comprehensively understanding and logically crafting effective bismuth-based photocatalysts, while also encouraging novel ideas and advances in energy and environmental fields, contributing to the goals of green chemistry and sustainable development.
- Photocatalysis,
- Bi,
- Heterojunction,
- Charge separation,
- Application
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