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Citation: Linfeng Xiao,  Wanlu Ren,  Shishi Shen,  Mengshan Chen,  Runhua Liao,  Yingtang Zhou,  Xibao Li. 调控ZnIn2S4/Bi2O3 S型异质结的电子结构和润湿性增强光催化析氢[J]. Acta Physico-Chimica Sinica, ;2024, 40(8): 230803. doi: 10.3866/PKU.WHXB202308036 shu

调控ZnIn2S4/Bi2O3 S型异质结的电子结构和润湿性增强光催化析氢

  • 1.

    School of Materials Science and Engineering, Jingdezhen Ceramic University, Jingdezhen 333403, Jiangxi Province, China;

  • 2.

    Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control, National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan 316022, Zhejiang Province, China;

  • 3.

    School of Materials Science and Engineering, Nanchang Hangkong University, Nanchang 330063, China

  • Corresponding author: Runhua Liao,  Yingtang Zhou,  Xibao Li, 
  • Received Date: 21 August 2023
    Revised Date: 28 September 2023
    Accepted Date: 28 September 2023

    Fund Project: The project was supported by the Zhejiang Province Key Research and Development Project (2023 C01191), National Natural Science Foundation of China (22262024, 51962023, 51468024), Jiangxi Academic and Technical Leader of Major Disciplines (20232BCJ22008), Natural Science Foundation of Jiangxi Province (20232ACB204007, 20202BABL203037), Jingdezhen Science and Technology Bureau Project (20192GYZD008-33).

  • 通过光催化水裂解制氢来生产可再生燃料具有巨大的潜力。然而，缓慢的析氢动力学和较差的水吸附对光催化剂构成了重大挑战。在这项研究中，我们开发了一种简单的水热法，用于从金属有机框架(MOF)中合成Bi2O3 (BO)，并将其负载到花状ZnIn2S4 (ZIS)上。该方法显著增强了水吸附和表面催化反应，从而显著提高了光催化活性。以三乙醇胺(TEOA)作为牺牲剂，在BO上负载15% (质量分数) ZIS时，析氢速率达到了1610 μmol∙h−1∙g−1，是纯BO的6.34倍。此外，利用密度泛函理论(DFT)和从头算分子动力学(AIMD)计算，我们确定了ZIS/BO S型异质结界面上的反应，包括水吸附和催化反应的活性位点。这项工作将为开发具有特定电子性能和润湿性的高性能复合光催化材料提供有价值的见解。
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