Citation: Qu Zhuoyan, Zhang Xiaoyin, Xiao Ru, Sun Zhenhua, Li Feng. Application of Organosulfur Compounds in Lithium-Sulfur Batteries[J]. Acta Physico-Chimica Sinica, ;2023, 39(8): 230101. doi: 10.3866/PKU.WHXB202301019 shu

Application of Organosulfur Compounds in Lithium-Sulfur Batteries

Qu Zhuoyan ^{1, 2} ,
Zhang Xiaoyin ^{1, 2} ,
Xiao Ru ^{1, 2} ,
Sun Zhenhua ^{1, 2,,} ,
Li Feng ^{1, 2,,}

1.
Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China
2.
School of Materials Science and Engineering, University of Science and Technology of China, Shenyang 110016, China

Corresponding author: Sun Zhenhua, zhsun@imr.ac.cn Li Feng, fli@imr.ac.cn
Received Date: 12 January 2023
Revised Date: 7 February 2023
Accepted Date: 8 February 2023
Available Online: 15 February 2023
Fund Project: The project was supported by the National Natural Science Foundation of China 51972313The project was supported by the National Natural Science Foundation of China 52020105010The project was supported by the National Natural Science Foundation of China 52188101the National Key R&D Program of China 2021YFB2800201the National Key R&D Program of China 2021YFB3800301the "Strategic Priority Research Program" of the Chinese Academy of Sciences XDA22010602the Youth Innovation Promotion Association of the Chinese Academy of Sciences Y201942Liaoning Revitalization Talents Program XLYC2007080Liaoning Revitalization Talents Program XLYC1908015

Lithium-sulfur batteries are one of the prospective next-generation power sources that can replace commercial lithium-ion batteries owing to their high theoretical energy density, eco-friendliness, and low cost. However, the insulating nature of the charge–discharge products, the shuttle effect of soluble lithium polysulfides, the volume expansion of the sulfur cathode, and the uncontrollable growth of lithium dendrites severely affect the actual capacity and cycling stability of lithium-sulfur batteries. Replacing the inorganic sulfur (S₈) cathode with an organosulfur-based cathode is a promising strategy for resolving the aforementioned issues. By modulating the fundamental units of the organosulfur compound, including the sulfur chain, carbon chain, and their interactions, the electrochemical reaction process can be altered, the ion/electron conductivity can be increased, and the shuttle effect can be effectively suppressed. In addition, organosulfur compounds as electrolyte additives can regulate the reaction process of the sulfur cathode and protect the lithium anode by forming a stable solid electrolyte interface, and as polymer electrolyte segments, they can accelerate the conduction of lithium ions. This review provides a detailed outline of the research progress and application of organosulfur compounds as cathodes, electrolyte additives, and solid-state electrolytes in lithium-sulfur batteries. The structure, reaction mechanism, and electrochemical properties of organosulfur compounds are correlated to provide comprehensive insights that can help address the prevailing issues of lithium-sulfur batteries. Finally, future prospects, including the challenges and potential solutions, are presented to guide the design, synthesis, and mechanistic studies of high-performance organosulfur compounds to realize a practical lithium-sulfur battery.
- Lithium-sulfur battery,
- Organosulfur compound,
- Shuttle effect,
- Electrolyte additive,
- Polymer solid-state electrolyte,
- Electrochemical energy storage
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