Citation: Chen Peng, Zhou Ying, Dong Fan. Advances in Regulation Strategies for Electronic Structure and Performance of Two-Dimensional Photocatalytic Materials[J]. Acta Physico-Chimica Sinica, ;2021, 37(8): 201001. doi: 10.3866/PKU.WHXB202010010 shu

Advances in Regulation Strategies for Electronic Structure and Performance of Two-Dimensional Photocatalytic Materials

Chen Peng ^1,2 ,
Zhou Ying ¹ ,
Dong Fan ^1,2,,

1.
School of New Energy and Materials, Southwest Petroleum University, Chengdu 610500, China
2.
Research Center for Environmental and Energy Catalysis, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 611731, China

Corresponding author: Dong Fan, dfctbu@126.com; dongfan@uestc.edu.cn
Received Date: 8 October 2020
Revised Date: 10 November 2020
Accepted Date: 10 November 2020
Available Online: 17 November 2020
Fund Project: the National Natural Science Foundation of China 21777011the National Natural Science Foundation of China 21822601The project was supported by the National Natural Science Foundation of China (21822601, 21777011)

Two-dimensional photocatalytic materials have potential applications in the fields of environmental purification and energy conversion owing to their rich surface active sites, unique geometric structures, adjustable electronic structures, and good photocatalytic activities. At present, the main two-dimensional photocatalytic materials include metal oxides, metal composite oxides, metal hydroxides, metal sulfides, bismuth-based materials, and non-metallic photocatalytic materials. The absorption of photons in bulk materials or nanoparticles is often limited by the transmittance and reflection at the grain boundary, while the two-dimensional structure can provide a large specific surface area and abundant surface low-coordination atoms to obtain more UV visible light. In addition, the smaller atomic thickness of two-dimensional photocatalytic materials can shorten the carrier migration distance. Thus, in two-dimensional photocatalytic materials, the carriers generated in the interior migrate to the surface faster than that in the bulk materials, which can reduce the recombination of photogenerated carriers and facilitate the photocatalytic reaction. For the surface redox reaction, the two-dimensional structure can provide more abundant surface-active sites to accelerate the reaction process. Additionally, when the thickness is reduced to the atomic scale, the escape energy of atoms is relatively small, thereby increasing the surface defects, which is helpful for the adsorption and activation of target molecules. Thus, the synthesis methods and performance enhancement strategies of two-dimensional photocatalytic materials have been developed rapidly. The former strategies mainly focus on the adjustment of morphology and geometric structure characteristics, which cannot fully meet the design requirements of efficient and stable photocatalysts. The photocatalytic performance and stability can be improved by surface design to construct abundant active sites and adjust the electronic structure. Research on the reaction mechanism of photocatalysis can help us understand the demand for photocatalytic structure characteristics in different reactions, thereby guiding the design of photocatalysts. In this paper, the advances in surface design and electronic structure regulation strategies of two-dimensional photocatalytic materials are reviewed from three aspects: light absorption; charge separation; and active sites, including element doping, heterojunction design, defect construction, single atom modification, and plasmonic metal loading. The effects on the reaction mechanism for typical air pollutant purification by regulating the electronic structure of two-dimensional photocatalytic materials are summarized. Finally, the problems and challenges associated with the development of two-dimensional photocatalytic materials are analyzed and discussed.
- Two dimensional photocatalytic materials,
- Surface design,
- Electronic structure,
- Reaction mechanism,
- Active sites
1. [1]
  Feng, J.; Zhang, Y.; Song, W.; Deng, W.; Zhu, M.; Fang, Z.; Ye, Y.; Fang, H.; Wu, Z.; Lowther, S.; et al. Environ. Pollut. 2020, 267, 115623. doi: 10.1016/j.envpol.2020.115623 doi: 10.1016/j.envpol.2020.115623
2. [2]
  An, J.; Zou, J.; Wang, J.; Lin, X.; Zhu, B. Environ. Sci. Pollut. Res. 2015, 22, 19607. doi: 10.1007/s11356-015-5177-0 doi: 10.1007/s11356-015-5177-0
3. [3]
  Glasius, M.; Goldstein, A. H. Environ. Sci. Technol. 2016, 50, 2754. doi: 10.1021/acs.est.5b05105 doi: 10.1021/acs.est.5b05105
4. [4]
  Li, J.; Dong, X. A.; Sun, Y.; Jiang, G.; Chu, Y.; Lee, S. C.; Dong, F. Appl. Catal. B-Environ. 2018, 239, 187. doi: 10.1016/j.apcatb.2018.08.019 doi: 10.1016/j.apcatb.2018.08.019
5. [5]
  Deng, Y.; Li, J.; Li, Y.; Wu, R.; Xie, S. J. Environ. Sci. 2019, 75, 334. doi: 10.1016/j.jes.2018.05.004 doi: 10.1016/j.jes.2018.05.004
6. [6]
  Muñoz, V.; Casado, C.; Suárez, S.; Sánchez, B.; Marugán, J. Catal. Today 2019, 326, 82. doi: 10.1016/j.cattod.2018.09.001 doi: 10.1016/j.cattod.2018.09.001
7. [7]
  Mo, J.; Zhang, Y.; Xu, Q.; Lamson, J. J.; Zhao, R. Atmos. Environ. 2009, 43, 2229. doi: 10.1016/j.atmosenv.2009.01.034 doi: 10.1016/j.atmosenv.2009.01.034
8. [8]
  Wang, S.; Ang, H. M.; Tade, M. O. Environ. Int. 2007, 33, 694. doi: 10.1016/j.envint.2007.02.011 doi: 10.1016/j.envint.2007.02.011
9. [9]
  Gao, X.; An, L.; Qu, D.; Jiang, W.; Chai, Y.; Sun, S.; Liu, X.; Sun, Z. Sci. Bull. 2019, 64, 918. doi: 10.1016/j.scib.2019.05.009 doi: 10.1016/j.scib.2019.05.009
10. [10]
  Li, S.; Wang, D.; Wu, X.; Chen, Y. Chin. J. Catal. 2020, 41, 550. doi: 10.1016/S1872-2067(19)63446-7 doi: 10.1016/S1872-2067(19)63446-7
11. [11]
  Luo, J.; Zhang, S.; Sun, M.; Yang, L.; Luo, S.; Crittenden, J. C. ACS Nano 2019, 13, 9811. doi: 10.1021/acsnano.9b03649 doi: 10.1021/acsnano.9b03649
12. [12]
  Wang, Q.; Hisatomi, T.; Jia, Q.; Tokudome, H.; Zhong, M.; Wang, C.; Pan, Z.; Takata, T.; Nakabayashi, M.; Shibata, N.; et al. Nat. Mater. 2016, 15, 611. doi: 10.1038/nmat4589 doi: 10.1038/nmat4589
13. [13]
  Ong, W. J.; Tan, L. L.; Ng, Y. H.; Yong, S. T.; Chai, S. P. Chem. Rev. 2016, 116, 7159. doi: 10.1021/acs.chemrev.6b00075 doi: 10.1021/acs.chemrev.6b00075
14. [14]
  Li, Y.; Zhang, D.; Fan, J.; Xiang, Q. Chin. J. Catal. 2021, 42, 627. doi: 10.1016/S1872-2067(20)63684-1 doi: 10.1016/S1872-2067(20)63684-1
15. [15]
  Cui, W.; Li, J.; Chen, L.; Dong, X. A.; Wang, H.; Sheng, J.; Sun, Y.; Zhou, Y.; Dong, F. Sci. Bull. 2020, 65, 1626. doi: 10.1016/j.scib.2020.05.024 doi: 10.1016/j.scib.2020.05.024
16. [16]
  Wang, H.; Zhang, L.; Chen, Z.; Hu, J.; Li, S.; Wang, Z.; Liu, J.; Wang, X. Chem. Soc. Rev. 2014, 43, 5234. doi: 10.1039/C4CS00126E doi: 10.1039/C4CS00126E
17. [17]
  Wu, W. Q.; Feng, H. L.; Rao, H. S.; Xu, Y. F.; Kuang, D. B.; Su, C. Y. Nat. Commun. 2014, 5, 3968. doi: 10.1038/ncomms4968 doi: 10.1038/ncomms4968
18. [18]
  Luo, B.; Liu, G.; Wang, L. Nanoscale 2016, 8, 6904. doi: 10.1039/C6NR00546B doi: 10.1039/C6NR00546B
19. [19]
  Xiong, J.; Di, J.; Xia, J.; Zhu, W.; Li, H. Adv. Funct. Mater. 2018, 28, 1801983. doi: 10.1002/adfm.201801983 doi: 10.1002/adfm.201801983
20. [20]
  Wang, L.; Zhang, Y.; Chen, L.; Xu, H.; Xiong, Y. Adv. Mater. 2018, 30, 1801955. doi: 10.1002/adma.201801955 doi: 10.1002/adma.201801955
21. [21]
  Liu, G.; Zhen, C.; Kang, Y.; Wang, L.; Cheng, H. -M. Chem. Soc. Rev. 2018, 47, 6410. doi: 10.1039/C8CS00396C doi: 10.1039/C8CS00396C
22. [22]
  Xiang, Q.; Yu, J.; Jaroniec, M. Chem. Soc. Rev. 2012, 41, 782. doi: 10.1039/C1CS15172J doi: 10.1039/C1CS15172J
23. [23]
  Gogotsi, Y. J. Phys. Chem. Lett. 2011, 2, 2509. doi: 10.1021/jz201145a doi: 10.1021/jz201145a
24. [24]
  Meng, N.; Ren, J.; Liu, Y.; Huang, Y.; Petit, T.; Zhang, B. Energy Environ. Sci. 2018, 11, 566. doi: 10.1039/C7EE03592F doi: 10.1039/C7EE03592F
25. [25]
  Safaei, J.; Mohamed, N. A.; Mohamad Noh, M. F.; Soh, M. F.; Ludin, N. A.; Ibrahim, M. A.; Roslam Wan Isahak, W. N.; Mat Teridi, M. A. J. Mater. Chem. A 2018, 6, 22346. doi: 10.1039/C8TA08001A doi: 10.1039/C8TA08001A
26. [26]
  Ding, F.; Yang, D.; Tong, Z.; Nan, Y.; Wang, Y.; Zou, X.; Jiang, Z. Environ. Sci. Nano 2017, 4, 1455. doi: 10.1039/C7EN00255F doi: 10.1039/C7EN00255F
27. [27]
  Low, J.; Cao, S.; Yu, J.; Wageh, S. Chem. Commun. 2014, 50, 10768. doi: 10.1039/C4CC02553A doi: 10.1039/C4CC02553A
28. [28]
  Li, X.; Dai, Y.; Ma, Y.; Han, S.; Huang, B. Phys. Chem. Chem. Phys. 2014, 16, 4230. doi: 10.1039/C3CP54592J doi: 10.1039/C3CP54592J
29. [29]
  Di, J.; Xiong, J.; Li, H.; Liu, Z. Adv. Mater. 2018, 30, 1704548. doi: 10.1002/adma.201704548 doi: 10.1002/adma.201704548
30. [30]
  Sun, Y.; Gao, S.; Lei, F.; Xie, Y. Chem. Soc. Rev. 2015, 44, 623. doi: 10.1039/C4CS00236A doi: 10.1039/C4CS00236A
31. [31]
  Zhang, J.; Chen, Y.; Wang, X. Energy Environ. Sci. 2015, 8, 3092. doi: 10.1039/C5EE01895A doi: 10.1039/C5EE01895A
32. [32]
  Zhao, Z.; Sun, Y.; Dong, F. Nanoscale 2015, 7, 15. doi: 10.1039/C4NR03008G doi: 10.1039/C4NR03008G
33. [33]
  Chen, P.; Liu, H.; Cui, W.; Lee, S. C.; Wang, L. A.; Dong, F. EcoMat 2020, 2, e12047. doi: 10.1002/eom2.12047 doi: 10.1002/eom2.12047
34. [34]
  Di, J.; Xiong, J.; Li, H.; Liu, Z. Adv. Mater. 2018, 30, 1704548. doi: 10.1002/adma.201704548 doi: 10.1002/adma.201704548
35. [35]
  Ong, W. J.; Tan, L. L.; Ng, Y. H.; Yong, S. T.; Chai, S. P. Chem. Rev. 2016, 116, 7159. doi: 10.1021/acs.chemrev.6b00075 doi: 10.1021/acs.chemrev.6b00075
36. [36]
  Xu, M.; Yang, J.; Sun, C.; Liu, L.; Cui, Y.; Liang, B. Chem. Eng. J. 2020, 389, 124402. doi: 10.1016/j.cej.2020.124402 doi: 10.1016/j.cej.2020.124402
37. [37]
  Li, S.; Sun, J.; Guan, J. Chin. J. Catal. 2021, 42, 511. doi: 10.1016/S1872-2067(20)63693-2 doi: 10.1016/S1872-2067(20)63693-2
38. [38]
  Ran, J.; Zhang, J.; Yu, J.; Jaroniec, M.; Qiao, S. Z. Chem. Soc. Rev. 2014, 43, 7787. doi: 10.1039/C3CS60425J doi: 10.1039/C3CS60425J
39. [39]
  Li, X.; Yu, J.; Jaroniec, M. Chem. Soc. Rev. 2016, 45, 2603. doi: 10.1039/C5CS00838G doi: 10.1039/C5CS00838G
40. [40]
  Dong, X.; Li, J.; Xing, Q.; Zhou, Y.; Huang, H.; Dong, F. Appl. Catal. B-Environ. 2018, 232, 69. doi: 10.1016/j.apcatb.2018.03.054 doi: 10.1016/j.apcatb.2018.03.054
41. [41]
  Cui, W.; Li, J.; Cen, W.; Sun, Y.; Lee, S. C.; Dong, F. J. Catal. 2017, 352, 351. doi: 10.1016/j.jcat.2017.05.017 doi: 10.1016/j.jcat.2017.05.017
42. [42]
  Chen, P.; Sun, Y.; Liu, H.; Zhou, Y.; Jiang, G.; Lee, S. C.; Zhang, Y.; Dong, F. Nanoscale 2019, 11, 2366. doi: 10.1039/c8nr09147a doi: 10.1039/c8nr09147a
43. [43]
  Li, J.; Dong, X.; Zhang, G.; Cui, W.; Cen, W.; Wu, Z.; Lee, S. C.; Dong, F. J. Mater. Chem. 2019, 7, 3366. doi: 10.1039/C8TA11627J doi: 10.1039/C8TA11627J
44. [44]
  Kabir, E.; Kumar, P.; Kumar, S.; Adelodun, A. A.; Kim, K. -H. Renew. Sust. Energ. Rev. 2018, 82, 894. doi: 10.1016/j.rser.2017.09.094 doi: 10.1016/j.rser.2017.09.094
45. [45]
  Xu, Z.; Quintanilla, M.; Vetrone, F.; Govorov, A. O.; Chaker, M.; Ma, D. Adv. Funct. Mater. 2015, 25, 2950. doi: 10.1002/adfm.201500810 doi: 10.1002/adfm.201500810
46. [46]
  Meng, X.; Liu, L.; Ouyang, S.; Xu, H.; Wang, D.; Zhao, N.; Ye, J. Adv. Mater. 2016, 28, 6781. doi: 10.1002/adma.201600305 doi: 10.1002/adma.201600305
47. [47]
  Wang, X.; Wang, F.; Sang, Y.; Liu, H. Adv. Energy Mater. 2017, 7, 1700473. doi: 10.1002/aenm.201700473 doi: 10.1002/aenm.201700473
48. [48]
  Osterloh, F. E. Chem. Soc. Rev. 2013, 42, 2294. doi: 10.1039/C2CS35266D doi: 10.1039/C2CS35266D
49. [49]
  Dong, F.; Ho, W.-K.; Lee, S. C.; Wu, Z.; Fu, M.; Zou, S.; Huang, Y. J. Mater. Chem. 2011, 21, 12428. doi: 10.1039/C1JM11840D doi: 10.1039/C1JM11840D
50. [50]
  Liu, Y.; Wang, Z.; Huang, B.; Yang, K.; Zhang, X.; Qin, X.; Dai, Y. Appl. Surf. Sci. 2010, 257, 172. doi: 10.1016/j.apsusc.2010.06.058 doi: 10.1016/j.apsusc.2010.06.058
51. [51]
  Yu, L.; Zhang, X.; Li, G.; Cao, Y.; Shao, Y.; Li, D. Appl. Catal. B: Environ. 2016, 187, 301. doi: 10.1016/j.apcatb.2016.01.045 doi: 10.1016/j.apcatb.2016.01.045
52. [52]
  Chen, L.; Yin, S. -F.; Luo, S. -L.; Huang, R.; Zhang, Q.; Hong, T.; Au, P. C. T. Ind. Eng. Chem. Res. 2012, 51, 6760. doi: 10.1021/ie300567y doi: 10.1021/ie300567y
53. [53]
  Wang, J. -J.; Zhai, X. -Y.; Zhang, G. -Y.; Zhang, J. -B.; Zhao, Y. -F. Solid State Sci. 2020, 105, 106288. doi: 10.1016/j.solidstatesciences.2020.106288 doi: 10.1016/j.solidstatesciences.2020.106288
54. [54]
  Tian, N.; Huang, H.; Guo, Y.; He, Y.; Zhang, Y. Appl. Surf. Sci. 2014, 322, 249. doi: https://doi.org/10.1016/j.apsusc.2014.10.071
55. [55]
  Hu, J.; Chen, D.; Li, N.; Xu, Q.; Li, H.; He, J.; Lu, J. Appl. Catal. B: Environ. 2017, 217, 224. doi: 10.1016/j.apcatb.2017.05.088 doi: 10.1016/j.apcatb.2017.05.088
56. [56]
  Dong, F.; Xiong, T.; Wang, R.; Sun, Y.; Jiang, Y. Dalton Trans. 2014, 43, 6631. doi:10.1039/C3DT53383B doi: 10.1039/C3DT53383B
57. [57]
  Hou, W.; Cronin, S. B. Adv. Funct. Mater. 2013, 23, 1612. doi: 10.1002/adfm.201202148 doi: 10.1002/adfm.201202148
58. [58]
  Atay, T.; Song, J.-H.; Nurmikko, A. V. Nano Letters 2004, 4, 1627. doi: 10.1021/nl049215n doi: 10.1021/nl049215n
59. [59]
  Kolwas, K.; Derkachova, A.; Shopa, M. J. Quant. Spectrosc. Radiat. Trans. 2009, 110, 1490. doi: 10.1016/j.jqsrt.2009.03.020 doi: 10.1016/j.jqsrt.2009.03.020
60. [60]
  Mock, J. J.; Barbic, M.; Smith, D. R.; Schultz, D. A.; Schultz, S. J. Chem. Phys. 2002, 116, 6755. doi: 10.1063/1.1462610 doi: 10.1063/1.1462610
61. [61]
  Kelly, K. L.; Coronado, E.; Zhao, L. L.; Schatz, G. C. J. Phys. Chem. B 2003, 107, 668. doi: 10.1021/jp026731y doi: 10.1021/jp026731y
62. [62]
  Li, Q.; Hao, X.; Guo, X.; Dong, F.; Zhang, Y. Dalton Trans. 2015, 44, 8805. doi: 10.1039/c5dt00844a doi: 10.1039/c5dt00844a
63. [63]
  Dong, F.; Li, Q.; Zhou, Y.; Sun, Y.; Zhang, H.; Wu, Z. Dalton Trans. 2014, 43, 9468. doi: 10.1039/c4dt00427b doi: 10.1039/c4dt00427b
64. [64]
  Dong, F.; Li, P.; Zhong, J.; Liu, X.; Zhang, Y.; Cen, W.; Huang, H. Appl. Catal. A-Gen. 2016, 510, 161. doi: 10.1016/j.apcata.2015.11.022 doi: 10.1016/j.apcata.2015.11.022
65. [65]
  Dong, F.; Li, Q.; Sun, Y.; Ho, W. ACS Catal. 2014, 4, 4341. doi: 10.1021/cs501038q doi: 10.1021/cs501038q
66. [66]
  Dong, X.; Zhang, W.; Cui, W.; Sun, Y.; Huang, H.; Wu, Z.; Dong, F. Catal. Sci. Technol. 2017, 7, 1324. doi: 10.1039/C6CY02444K doi: 10.1039/C6CY02444K
67. [67]
  Guo, L.; Yang, Z.; Marcus, K.; Li, Z.; Luo, B.; Zhou, L.; Wang, X.; Du, Y.; Yang, Y. Energy Environ. Sci. 2018, 11, 106. doi: 10.1039/C7EE02464A doi: 10.1039/C7EE02464A
68. [68]
  Chen, Y.; Ji, S.; Chen, C.; Peng, Q.; Wang, D.; Li, Y. Joule 2018, 2, 1242. doi: 10.1016/j.joule.2018.06.019 doi: 10.1016/j.joule.2018.06.019
69. [69]
  Zhang, J. Z. J. Phys. Chem. B 2000, 104, 7239. doi: 10.1021/jp000594s doi: 10.1021/jp000594s
70. [70]
  Kubacka, A.; Fernández-García, M.; Colón, G. Chem. Rev. 2012, 112, 1555. doi: 10.1021/cr100454n doi: 10.1021/cr100454n
71. [71]
  Shao, W.; Wang, H.; Zhang, X. Dalton Trans. 2018, 47, 12642. doi: 10.1039/C8DT02613K doi: 10.1039/C8DT02613K
72. [72]
  Wang, Y. Q.; Shen S. H. Acta Phys. -Chim. Sin. 2020, 36, 1905080. doi: 10.3866/pku.whxb201905080
73. [73]
  Park, H. S.; Kweon, K. E.; Ye, H.; Paek, E.; Hwang, G. S.; Bard, A. J. J. Phys. Chem. C 2011, 115, 17870. doi: 10.1021/jp204492r doi: 10.1021/jp204492r
74. [74]
  Zhao, Z.; Sun, Y.; Dong, F.; Zhang, Y.; Zhao, H. Rsc Adv. 2015, 5, 39549. doi: 10.1039/C5RA03433G doi: 10.1039/C5RA03433G
75. [75]
  Chen, P.; Wang, H.; Liu, H.; Ni, Z.; Li, J.; Zhou, Y.; Dong, F. Appl. Catal. B-Environ. 2019, 242, 19. doi:10.1016/j.apcatb.2018.09.078 doi: 10.1016/j.apcatb.2018.09.078
76. [76]
  Yuan, C.; Cui, W.; Sun, Y.; Wang, J.; Chen, R.; Zhang, J.; Zhang, Y.; Dong, F. Chin. Chem. Lett. 2020, 31, 751. doi: 10.1016/j.cclet.2019.09.033 doi: 10.1016/j.cclet.2019.09.033
77. [77]
  Lei, F.; Zhang, L.; Sun, Y.; Liang, L.; Liu, K.; Xu, J.; Zhang, Q.; Pan, B.; Luo, Y.; Xie, Y. Angew. Chem. Int. Edit. 2015, 54, 9266. doi: 10.1002/anie.201503410 doi: 10.1002/anie.201503410
78. [78]
  Mi, Y.; Wen, L.; Wang, Z.; Cao, D.; Xu, R.; Fang, Y.; Zhou, Y.; Lei, Y. Nano Energy 2016, 30, 109. doi: 10.1016/j.nanoen.2016.10.001 doi: 10.1016/j.nanoen.2016.10.001
79. [79]
  Xiong, T.; Cen, W.; Zhang, Y.; Dong, F. ACS Catal. 2016, 6, 2462. doi: 10.1021/acscatal.5b02922 doi: 10.1021/acscatal.5b02922
80. [80]
  Li, J.; Cui, W.; Sun, Y.; Chu, Y.; Cen, W.; Dong, F. J. Mater. Chem. A 2017, 5, 9358. doi: 10.1039/C7TA02183F doi: 10.1039/C7TA02183F
81. [81]
  Liu, G.; Niu, P.; Sun, C.; Smith, S. C.; Chen, Z.; Lu, G. Q.; Cheng, H. -M. J. Am. Chem. Soc. 2010, 132, 11642. doi: 10.1021/ja103798k doi: 10.1021/ja103798k
82. [82]
  Zai, J.; Cao, F.; Liang, N.; Yu, K.; Tian, Y.; Sun, H.; Qian, X. J. Hazard. Mater. 2017, 321, 464. doi: 10.1016/j.jhazmat.2016.09.034 doi: 10.1016/j.jhazmat.2016.09.034
83. [83]
  Wu, D.; Yue, S.; Wang, W.; An, T.; Li, G.; Yip, H. Y.; Zhao, H.; Wong, P. K. Appl. Catal. B-Environ. 2016, 192, 35. doi: 10.1016/j.apcatb.2016.03.046 doi: 10.1016/j.apcatb.2016.03.046
84. [84]
  Yang, W.; Zhang, L.; Xie, J.; Zhang, X.; Liu, Q.; Yao, T.; Wei, S.; Zhang, Q.; Xie, Y. Angew. Chem. Int. Edit. 2016, 55, 6716. doi: 10.1002/anie.201602543 doi: 10.1002/anie.201602543
85. [85]
  Huang, H.; Li, X.; Wang, J.; Dong, F.; Chu, P. K.; Zhang, T.; Zhang, Y. ACS Catal. 2015, 5, 4094. doi: 10.1021/acscatal.5b00444 doi: 10.1021/acscatal.5b00444
86. [86]
  Cui, W.; Li, J.; Sun, Y.; Wang, H.; Jiang, G.; Lee, S. C.; Dong, F. Appl. Catal. B-Environ. 2018, 237, 938. doi: 10.1016/j.apcatb.2018.06.071 doi: 10.1016/j.apcatb.2018.06.071
87. [87]
  Li, J.; Zhang, Z.; Cui, W.; Wang, H.; Cen, W.; Johnson, G.; Jiang, G.; Zhang, S.; Dong, F. ACS Catal. 2018, 8, 8376. doi: 10.1021/acscatal.8b02459 doi: 10.1021/acscatal.8b02459
88. [88]
  Marschall, R. Adv. Funct. Mater. 2014, 24, 2421. doi: 10.1002/adfm.201303214 doi: 10.1002/adfm.201303214
89. [89]
  An, X.; Wang, Y.; Lin, J.; Shen, J.; Zhang, Z.; Wang, X. Sci. Bull. 2017, 62, 599. doi: 10.1016/j.scib.2017.03.025 doi: 10.1016/j.scib.2017.03.025
90. [90]
  Zhou, H.; Qu, Y.; Zeid, T.; Duan, X. Energy Environ. Sci. 2012, 5, 6732. doi: 10.1039/C2EE03447F doi: 10.1039/C2EE03447F
91. [91]
  Wang, Y.; Wang, Q.; Zhan, X.; Wang, F.; Safdar, M.; He, J. Nanoscale 2013, 5, 8326. doi: 10.1039/C3NR01577G doi: 10.1039/C3NR01577G
92. [92]
  He, W.; Wu, X.; Li, Y.; Xiong, J.; Tang, Z.; Wei, Y.; Zhao, Z.; Zhang, X.; Liu, J. Chin. Chem. Lett. 2020, 31, 2774. doi: 10.1016/j.cclet.2020.07.019 doi: 10.1016/j.cclet.2020.07.019
93. [93]
  Ao, Y.; Wang, K.; Wang, P.; Wang, C.; Hou, J. Appl. Catal. B: Environ. 2016, 194, 157. doi: 10.1016/j.apcatb.2016.04.050 doi: 10.1016/j.apcatb.2016.04.050
94. [94]
  Tian, N.; Huang, H.; Liu, C.; Dong, F.; Zhang, T.; Du, X.; Yu, S.; Zhang, Y. J. Mater. Chem. A 2015, 3, 17120. doi: 10.1039/C5TA03669K doi: 10.1039/C5TA03669K
95. [95]
  Zhang, Y.; Wang, Q.; Liu, D.; Wang, Q.; Li, T.; Wang, Z. Appl. Surf. Sci. 2020, 521, 146434. doi: 10.1016/j.apsusc.2020.146434 doi: 10.1016/j.apsusc.2020.146434
96. [96]
  Yu, W.; Chen, J.; Shang, T.; Chen, L.; Gu, L.; Peng, T. Appl. Catal. B: Environ. 2017, 219, 693. doi:10.1016/j.apcatb.2017.08.018 doi: 10.1016/j.apcatb.2017.08.018
97. [97]
  Di, J.; Chen, C.; Yang, S. -Z.; Ji, M.; Yan, C.; Gu, K.; Xia, J.; Li, H.; Li, S.; Liu, Z. J. Mater. Chem. A 2017, 5, 14144. doi: 10.1039/C7TA03624H doi: 10.1039/C7TA03624H
98. [98]
  Zhang, N.; Li, X.; Ye, H.; Chen, S.; Ju, H.; Liu, D.; Lin, Y.; Ye, W.; Wang, C.; Xu, Q.; et al. J. Am. Chem. Soc. 2016, 138, 8928. doi: 10.1021/jacs.6b04629 doi: 10.1021/jacs.6b04629
99. [99]
  Liu, Y.; Xiao, C.; Li, Z.; Xie, Y. Adv. Energy Mater. 2016, 6, 1600436. doi: 10.1002/aenm.201600436 doi: 10.1002/aenm.201600436
100. [100]
  Wang, H.; He, W.; Dong, X. a.; Wang, H.; Dong, F. Sci. Bull. 2018, 63, 117. doi: 10.1016/j.scib.2017.12.013 doi: 10.1016/j.scib.2017.12.013
101. [101]
  Huang, J. J.; D, J. M.; Du H. W.; Xu G. S.; Yuan, Y. P.. Acta Phys. -Chim. Sin. 2020, 36, 1905056. doi: 10.3866/PKU.WHXB201905056
102. [102]
  Niu, P.; Liu, G.; Cheng, H. -M. J. Phys. Chem. C 2012, 116, 11013. doi: 10.1021/jp301026y doi: 10.1021/jp301026y
103. [103]
  Yuan, J.; Liu, X.; Tang, Y.; Zeng, Y.; Wang, L.; Zhang, S.; Cai, T.; Liu, Y.; Luo, S.; Pei, Y.; Liu, C. Appl. Catal. B-Environ. 2018, 237, 24. doi: 10.1016/j.apcatb.2018.05.064 doi: 10.1016/j.apcatb.2018.05.064
104. [104]
  Liao, J.; Cui, W.; Li, J.; Sheng, J.; Wang, H.; Dong, X. a.; Chen, P.; Jiang, G.; Wang, Z.; Dong, F. Chem. Eng. J. 2020, 379, 122282. doi: 10.1016/j.cej.2019.122282 doi: 10.1016/j.cej.2019.122282
105. [105]
  Liu, H.; Chen, P.; Yuan, X.; Zhang, Y.; Huang, H.; Wang, L. A.; Dong, F. Chin. J. Catal. 2019, 40, 620. doi: 10.1016/S1872-2067(19)63279-1 doi: 10.1016/S1872-2067(19)63279-1
106. [106]
  Dong, X. A.; Cui, W.; Wang, H.; Li, J.; Sun, Y.; Wang, H.; Zhang, Y.; Huang, H.; Dong, F. Sci. Bull. 2019, 64, 669. doi: 10.1016/j.scib.2019.04.020 doi: 10.1016/j.scib.2019.04.020
107. [107]
  Chen, P.; Liu, H.; Sun, Y.; Li, J.; Cui, W.; Wang, L. A.; Zhang, W.; Yuan, X.; Wang, Z.; Zhang, Y.; Dong, F. Appl. Catal. B-Environ. 2020, 264, 118545. doi: 10.1016/j.apcatb.2019.118545 doi: 10.1016/j.apcatb.2019.118545
108. [108]
  Wang, H.; Zhang, W.; Li, X.; Li, J.; Cen, W.; Li, Q.; Dong, F. Appl. Catal. B-Environ. 2018, 225, 218. doi: 10.1016/j.apcatb.2017.11.079 doi: 10.1016/j.apcatb.2017.11.079
109. [109]
  Dong, X. A.; Zhang, W.; Sun, Y.; Li, J.; Cen, W.; Cui, Z.; Huang, H.; Dong, F. J. Catal. 2018, 357, 41. doi: 10.1016/j.jcat.2017.10.004 doi: 10.1016/j.jcat.2017.10.004
110. [110]
  Liao, J.; Li, K.; Ma, H.; Dong, F.; Zeng, X.; Sun, Y. Chin. Chem. Lett. 2020, doi: 10.1016/j.cclet.2020.03.081 doi: 10.1016/j.cclet.2020.03.081
111. [111]
  Gao, S.; Gu, B.; Jiao, X.; Sun, Y.; Zu, X.; Yang, F.; Zhu, W.; Wang, C.; Feng, Z.; Ye, B.; Xie, Y. J. Am. Chem. Soc. 2017, 139, 3438. doi: 10.1021/jacs.6b11263 doi: 10.1021/jacs.6b11263
112. [112]
  Zhu, C.; Liu, T.; Qian, F.; Han, T. Y. -J.; Duoss, E. B.; Kuntz, J. D.; Spadaccini, C. M.; Worsley, M. A.; Li, Y. Nano Lett. 2016, 16, 3448. doi: 10.1021/acs.nanolett.5b04965 doi: 10.1021/acs.nanolett.5b04965
113. [113]
  Li, S.; Shi, M.; Yu, J.; Li, S.; Lei, S.; Lin, L.; Wang, J. Chin. Chem. Lett. 2020, doi:10.1016/j.cclet.2020.09.056 doi: 10.1016/j.cclet.2020.09.056
114. [114]
  Liu, J. ACS Catal. 2017, 7, 34. doi: 10.1021/acscatal.6b01534 doi: 10.1021/acscatal.6b01534
115. [115]
  Yang, S.; Gong, Y.; Zhang, J.; Zhan, L.; Ma, L.; Fang, Z.; Vajtai, R.; Wang, X.; Ajayan, P. M. Adv. Mater. 2013, 25, 2452. doi: 10.1002/adma.201204453 doi: 10.1002/adma.201204453
116. [116]
  Niu, P.; Zhang, L.; Liu, G.; Cheng, H. -M. Adv. Funct. Mater. 2012, 22, 4763. doi: 10.1002/adfm.201200922 doi: 10.1002/adfm.201200922
117. [117]
  Ovchinnikov, D.; Allain, A.; Huang, Y. -S.; Dumcenco, D.; Kis, A. ACS Nano 2014, 8, 8174. doi: 10.1021/nn502362b doi: 10.1021/nn502362b
118. [118]
  Parzinger, E.; Miller, B.; Blaschke, B.; Garrido, J. A.; Ager, J. W.; Holleitner, A.; Wurstbauer, U. ACS Nano 2015, 9, 11302. doi: 10.1021/acsnano.5b04979 doi: 10.1021/acsnano.5b04979
119. [119]
  Lei, F.; Sun, Y.; Liu, K.; Gao, S.; Liang, L.; Pan, B.; Xie, Y. J. Am. Chem. Soc. 2014, 136, 6826. doi: 10.1021/ja501866r doi: 10.1021/ja501866r
120. [120]
  Liu, J.; Wang, D.; Wang, M.; Kong, D.; Zhang, Y.; Chen, J.-F.; Dai, L. Chem. Eng. Technol. 2016, 39, 891. doi: 10.1002/ceat.201500542 doi: 10.1002/ceat.201500542
121. [121]
  Xie, J.; Zhang, X.; Zhang, H.; Zhang, J.; Li, S.; Wang, R.; Pan, B.; Xie, Y. Adv. Mater. 2017, 29, 1604765. doi: 10.1002/adma.201604765 doi: 10.1002/adma.201604765
122. [122]
  Li, X.; Bi, W.; Zhang, L.; Tao, S.; Chu, W.; Zhang, Q.; Luo, Y.; Wu, C.; Xie, Y. Adv. Mater. 2016, 28, 2427. doi: 10.1002/adma.201505281 doi: 10.1002/adma.201505281
123. [123]
  Chen, Z.; Mitchell, S.; Vorobyeva, E.; Leary, R. K.; Hauert, R.; Furnival, T.; Ramasse, Q. M.; Thomas, J. M.; Midgley, P. A.; Dontsova, D.; et al. Adv. Funct. Mater. 2017, 27, 1605785. doi: 10.1002/adfm.201605785 doi: 10.1002/adfm.201605785
124. [124]
  Liu, G.; Robertson, A. W.; Li, M. M.-J.; Kuo, W. C. H.; Darby, M. T.; Muhieddine, M. H.; Lin, Y. -C.; Suenaga, K.; Stamatakis, M.; Warner, J. H.; Tsang, S. C. E. Nat. Chem. 2017, 9, 810. doi: 10.1038/nchem.2740 doi: 10.1038/nchem.2740
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