Citation: SUN Meng, LI Jing-Hong. Recent Progress on Palladium-Based Oxygen Reduction Reaction Electrodes for Water Treatment[J]. Acta Physico-Chimica Sinica, ;2017, 33(1): 198-210. doi: 10.3866/PKU.WHXB201609191 shu

Recent Progress on Palladium-Based Oxygen Reduction Reaction Electrodes for Water Treatment

SUN Meng ^1,3, ,
LI Jing-Hong ²

1.
Key Laboratory of Drinking Water Science and Technology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, P. R. China;
2.
Department of Chemistry, Beijing Key Laboratory for Microanalytical Methods and Instrumentation, Tsinghua University, Beijing 100084, P. R. China;
3.
University of Chinese Academy of Sciences, Beijing 100049, P. R. China

Received Date: 18 July 2016
Revised Date: 16 September 2016

Fund Project: The project was supported by the National Key Research and Development Program of China (2016YFA0203101), National Key Basic Research Program of China (2013CB934004), National Natural Science Foundation of China (51572139), and Tsinghua University Initiative Scientific Research Program, China.

Developing highly efficient electrode catalysts with the four-electron oxygen reduction pathway has remained a research hotspot in fuel cell research. However, the pursuit of novel electrode catalysts possessing the specific two-electron reduction route for water treatment is challenging. In this review, we focus on recent progress in electrocatalytic treatment of refractory pollutants in water by palladium (Pd)-based noble metal electrodes. We highlight:(i) the degradation and mineralization of organic pollutants through electrocatalytic oxidation derived from the combination of Fe²⁺ and H₂O₂, which can be in-situ synthesized by Pd based electrodes; (ii) electrocatalytic reduction transformation from toxic organic pollutants and inorganic salts to harmless products by Pd-based electrodes; and (iii) removal of heavy metals by redox conversion via Pd-based electrodes. The future opportunities and prospects of applying noble metal nanocatalysts in water treatment are discussed.
- Electrocatalysis,
- Oxygen reduction,
- Electrode material,
- Water treatment
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