Citation:
NG Jin-Hua, WANG Chen-Hui, BIAN Zi-Jun, YANG Li, HU Jun, LIU Hong-Lai. Asymmetric Polyimide Mixed Matrix Membranes with Porous Materials-Modified Surfaces for CO2/N2 and CO2/CH4 Separations[J]. Acta Physico-Chimica Sinica,
;2015, 31(10): 1963-1970.
doi:
10.3866/PKU.WHXB201508282
-
Membranes with both od permeation and selectivity are highly desired for gas separations. We synthesized a polyimide (PI) asymmetric membrane using the phase-inversion method, and then modified the surface with a mixture of porous fillers and poly(amic acid) (PAA). The porous fillers included the metal organic framework (MOF) of Cu3(BTC)2 (copper benzene-1,3,5-tricarboxylate), the zeolite imidazole framework (ZIF) of ZIF-8, and the porous hydrotalcite of MgAl-LDH. A series of asymmetric mixed-matrix membranes (MMMs) were obtained after surface coating and thermal amidation. The MMM structure, CO2, CH4, and N2 permeance, and the ideal gas selectivity were investigated. With the surface modification, the morphology of the surface separation layers of the asymmetric PI/ZIF-8, PI/LDH, and PI/Cu3(BTC)2 MMMs significantly changed, and the gas separation performance changed accordingly. The PI/ZIF-8 asymmetric MMM with 5% (w) ZIF-8 doping exhibited both enhanced ideal gas selectivity and permeance; the CO2/N2 and CO2/CH4 selectivity were as high as 24 and 83, respectively. Thus, this surface modification provides improved MMM gas separation performance.
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Keywords:
- Gas separation,
- Surface modification,
- Polyimide,
- ZIF-8
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References
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(33) Husain, S.; Koros, W. J. J. Membr. Sci. 2007, 288, 195. doi: 10.1016/j.memsci.2006.11.016
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(34) Li, Y.; Chung, T. S.; Huang, Z.; Kulprathipanja, S. J. Membr. Sci. 2006, 277, 28. doi: 10.1016/j.memsci.2005.10.008
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-
[1]
-
-
[1]
(1) Chen, X. Y.; Vinh-Thang, H.; Ramirez, A. A.; Rodrigue, D. RSC Adv. 2015, 5 (31), 24399. doi: 10.1039/C5RA00666J
-
[2]
(2) Nunes, S. P.; Peinemann, K. V. Gas Separation with Membranes, 1st ed.; Wiley-VCH: Weinheim, 2001; pp 39-67.
-
[3]
(3) Hara, N.; Yoshimune, M.; Negishi, H.; Hara, S. J. Membr. Sci. 2014, 450, 215. doi: 10.1016/j.memsci.2013.09.012
-
[4]
(4) Cao, L. J.; Tao, K.; Huang, A. S.; Kong, C. L.; Chen, L. Chem. Commun. 2013, 49 (76), 8513. doi: 10.1039/c3cc44530e
-
[5]
(5) Nguyen, P. T.; Voss, B. A.; Wiesenauer, E. F.; Gin, D. L.; Noble, R. D. Ind. Eng. Chem. Res. 2012, 52 (26), 8812.
-
[6]
(6) Chen, H. R.; Chang, R. R.; Li, L.; Yuan, W. H. Acta Phys. -Chim. Sin. 2011, 27 (1), 241. [陈华荣, 常然然, 李莉, 袁文辉. 物理化学学报, 2011, 27 (1), 241.] doi: 10.3866/PKU.WHXB20110119
-
[7]
(7) Huang, A.; Wang, N.; Kong, C.; Caro, J. Angew. Chem. -Int. Edit. 2012, 51 (42), 10551. doi: 10.1002/anie.201204621
-
[8]
(8) Venna, S. R.; Carreon, M. A. J. Am. Chem. Soc. 2009, 132 (1), 76.
-
[9]
(9) Ni, Z. M.; Xu, Q.; Pan, G. X.; Mao, J. H. Acta Phys. -Chim. Sin. 2009, 25 (4), 792. [倪哲明, 胥倩, 潘国祥, 毛江洪. 物理化学学报, 2009, 25 (4), 792.] doi:10.3866/PKU.WHXB20090420
-
[10]
(10) Liu, Y.; Pan, J. H.; Wang, N. Y.; Steinbach, F.; Liu, X. L.; Caro, J. J. Angew. Chem. -Int. Edit. 2015, 54 (10), 3028. doi: 10.1002/anie.201411550
-
[11]
(11) Liang, Y.; Lu, Y.; Yao, W. S.; Zhang, X. T. Acta Phys. -Chim. Sin. 2015, 31 (6), 1179. [梁祎, 卢赟, 姚维尚, 张学同. 物理化学学报, 2015, 31 (6), 1179.] doi:10.3866/PKU.WHXB201504146
-
[12]
(12) Jie, X. M.; Duan, C. J.; Wang, L. A.; Jiang, C.; Zheng, H.; Liu, J. H.; Liu, D. D.; Cao, Y. M.; Yuan, Q. Ind. Eng. Chem. Res. 2014, 53 (11), 4442. doi: 10.1021/ie404198m
-
[13]
(13) Robeson, L. M. J. Membr. Sci. 1991, 62 (2), 165. doi: 10.1016/0376-7388(91)80060-J
-
[14]
(14) Robeson, L. M. J. Membr. Sci. 2008, 320 (1-2), 390. doi: 10.1016/j.memsci.2008.04.030
-
[15]
(15) Swaidan, R.; Ma, X.; Litwiller, E.; Pinnau, I. J. Membr. Sci. 2013, 447, 387. doi: 10.1016/j.memsci.2013.07.057
-
[16]
(16) Ma, Y. H.; Zhao, H. L.; Tang, S. J.; Hu, J.; Liu, H. L. Acta Phys. -Chim. Sin. 2011, 27 (3), 689. [马燕辉, 赵会玲, 唐圣杰, 胡军, 刘洪来. 物理化学学报, 2011, 27 (3), 689.] doi: 10.3866/PKU.WHXB20110335
-
[17]
(17) Defontaine, G.; Barichard, A.; Letaief, S.; Feng, C. Y.; Matsuura, T.; Detellier, C. J. Colloid Interface Sci. 2010, 343 (2), 622. doi: 10.1016/j.jcis.2009.11.048
-
[18]
(18) Ning, X.; Koros, W. J. Carbon 2014, 66, 511. doi: 10.1016/j.carbon.2013.09.028
-
[19]
(19) Rahman, M. M.; Shishatskiy, S.; Abetz, C. J. Membr. Sci. 2014, 469, 344. doi: 10.1016/j.memsci.2014.06.048
-
[20]
(20) Xu, H.; Tong, M. M.; Wu, D.; Xiao, G.; Yang, Q. Y.; Liu, D. H.; Zhong, C. L. Acta Phys. -Chim. Sin. 2015, 31 (1), 41. [许红, 童敏曼, 吴栋, 肖刚, 阳庆元, 刘大欢, 仲崇立. 物理化学学报, 2015, 31 (1), 41.] doi: 10.3866/PKU.WHXB201411132
-
[21]
(21) Bae, T. H.; Lee, J. S. Angew. Chem. -Int. Edit. 2010, 49 (51), 9863. doi: 10.1002/anie.v49.51
-
[22]
(22) Zhang, C.; Dai, Y.; Johnson, J. R. J. Membr. Sci. 2012, 389, 34. doi: 10.1016/j.memsci.2011.10.003
-
[23]
(23) Bae, T. H.; Long, J. R. Energy Environ. Sci. 2013, 6 (12), 3565. doi: 10.1039/c3ee42394h
-
[24]
(24) Lü, L.; Wu, G. Q.; Duan, X.; Li, F.; Du, Y. B. Speciality Petrochemicals 2001, 6, 9. [吕亮, 吾国强, 段雪, 李峰, 杜以波. 精细石油化工, 2001, 6, 9.]
-
[25]
(25) Zhou, S. Y.; Zou, X. Q.; Sun, F. X.; Zhang, F.; Fan, S. J.; Zhao, H. J.; Schiestel, T.; Zhu, G. S. J. Mater. Chem. 2012, 22, 10322. doi: 10.1039/c2jm16371c
-
[26]
(26) Cravillon, J.; Münzer, S.; Lohmeier, S. J.; Feldhoff, A.; Huber, K.; Wiebcke, M. Chem. Mater. 2009, 21, 1410. doi: 10.1021/cm900166h
-
[27]
(27) Bux, H.; Liang, F. Y.; Li, Y. S.; Janosch, C.; Michael, W.; Juürgen, C. J. Am. Chem. Soc. 2009, 131, 16000. doi: 10.1021/ja907359t
-
[28]
(28) Yeny, C. H.; Trevor, K. C.; Andrew, L. L.; Douglas, L. G.; Richard, D. N. J. Membr. Sci. 2011, 370, 141. doi: 10.1016/j.memsci.2011.01.012
-
[29]
(29) Ahn, J.; Chung, W. J.; In , P.; Michael, D. G. J. Membr. Sci. 2008, 314, 123. doi: 10.1016/j.memsci.2008.01.031
-
[30]
(30) Sangil, K.; Liang, C.; Johnson, J. K.; Marand, E. J. Membr. Sci. 2007, 294, 147. doi: 10.1016/j.memsci.2007.02.028
-
[31]
(31) Song, Q. L.; Nataraj, S. K.; Roussenova, M. V.; Tan, J. C.; Hughes, D. J.; Li, W.; Bour in, P.; Alam, M. A.; Cheetham, A. K.; Al-Muhtaseb, S. A.; Sivaniah, E. Energy Environ. Sci. 2012, 5 (8), 8359. doi: 10.1039/c2ee21996d
-
[32]
(32) Adams, R. T.; Lee, J. S.; Bae, T. H.; Ward, J. K.; Johnson, J. R.; Jones, C. W.; Nair, S.; Koros, W. J. J. Membr. Sci. 2011, 367, 197. doi: 10.1016/j.memsci.2010.10.059
-
[33]
(33) Husain, S.; Koros, W. J. J. Membr. Sci. 2007, 288, 195. doi: 10.1016/j.memsci.2006.11.016
-
[34]
(34) Li, Y.; Chung, T. S.; Huang, Z.; Kulprathipanja, S. J. Membr. Sci. 2006, 277, 28. doi: 10.1016/j.memsci.2005.10.008
-
[35]
(35) Tania, R.; Marion, V. D.; Elena, G. P.; Pablo, S. C.; Beatriz, Z.; Freek, K.; Jorge, G. Adv. Funct. Mater. 2014, 24, 249. doi: 10.1002/adfm.v24.2
-
[36]
(36) Khan, A. L.; Klaysom, C.; Gahlaut, A.; Li, X.; Vankelecom, I. F. J. J. Mater. Chem. 2012, 22, 20057. doi: 10.1039/c2jm34885c
-
[37]
(37) Omid, G. N.; Xiao, Y. C.; Serge, K. J. Membr. Sci. 2012, 413, 48.
-
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