Citation: WANG Shuo-Jue, AO Yin-Yong, ZHOU Han-Yang, YUAN Li-Yong, PENG Jing, ZHAI Mao-Lin. Research Progress in Radiation Effects on Ionic Liquids[J]. Acta Physico-Chimica Sinica, ;2014, 30(9): 1597-1604. doi: 10.3866/PKU.WHXB201406271 shu

Research Progress in Radiation Effects on Ionic Liquids

1.
1. Radiochemistry and Radiation Chemistry Key Laboratory of Fundamental Science, Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, P. R. China;
2. Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, P. R. China

Received Date: 4 May 2014
Available Online: 27 June 2014
Fund Project:

Ionic liquids (ILs) are regarded as a new generation of green solvents in spent nuclear fuel reprocessing, because of their fascinating properties such as negligible vapor pressure, high thermal stability, and successful use in the extraction of metal ions. However, the full realization of their potential requires a comprehensive knowledge of radiation effects on ILs, as they would be exposed to high radiation dose during extraction of high-level radioactive nuclides. This review presents research on the radiation effects on ILs, including radiation effects on the structures and properties of ILs, pulse radiolysis and laser photolysis of ILs, identification of radiolytic products of ILs and their influence on the extraction of metal ions. Our vision for the further development of this field is also proposed.
- Ionic liquid,
- Radiation effect,
- Extraction,
- Radiolytic product,
- Spent nuclear fuel reprocessing
1. [1]
  
  (1) Herrmann,W. A.; Bohm, V. P.W. J. Organomet. Chem. 1999, 572 (1), 141. doi: 10.1016/S0022-328X(98)00941-3
2. [2]
  (2) Le Boulaire, V.; Gree, R. Chem. Commun. 2000, No. 22, 2195.(3) Xiao, Y.; Malhotra, S. V. Tetrahedron Lett. 2004, 45 (45), 8339. doi: 10.1016/j.tetlet.2004.09.070
3. [3]
  (4) Boxwell, C. J.; Dyson, P. J.; Ellis, D. J.;Welton, T. J. Am. Chem. Soc. 2002, 124 (32), 9334. doi: 10.1021/ja026361r
4. [4]
  (5) Song, C. E.; Oh, C. R.; Roh, E. J.; Choo, D. J. Chem. Commun. 2000, No. 18, 1743.(6) Wasserscheid, P.;Waffenschmidt, H. J. Mol. Catal. A-Chem. 2000, 164 (1-2), 61. doi: 10.1016/S1381-1169(00)00259-4
5. [5]
  (7) Wang, P.;Wenger, B.; Humphry-Baker, R.; Moser, J. E.; Teuscher, J.; Kantlehner,W.; Mezger, J.; Stoyanov, E. V.; Zakeeruddin, S. M.; Grätzel, M. J. Am. Chem. Soc. 2005, 127 (18), 6850. doi: 10.1021/ja042232u
6. [6]
  (8) Wang, R.; Okajima, T.; Kitamura, F.; Ohsaka, T. Electroanal. 2004, 16 (1-2), 66.(9) Jiang, T. F.; Gu, Y. L.; Liang, B.; Li, J. B.; Shi, Y. P.; Ou, Q. Y. Anal. Chim. Acta 2003, 479 (2), 249. doi: 10.1016/S0003-2670(02)01537-4
7. [7]
  (10) Zhang,W. Z.; He, L. J.; Gu, Y. L.; Liu, X.; Jiang, S. X. Anal. Lett. 2003, 36 (4), 827. doi: 10.1081/AL-120018802
8. [8]
  (11) He, L. J.; Zhang,W. Z.; Zhao, L.; Liu, X.; Jiang, S. X. J. Chromatogr. A 2003, 1007 (1-2), 39. doi: 10.1016/S0021-9673(03)00987-7
9. [9]
  (12) Dai, S.; Ju, Y. H.; Barnes, C. E. J. Chem. Soc.-Dalton Trans. 1999, No. 8, 1201.(13) Sengupta, A.; Mohapatra, P. K.; Iqbal, M.; Huskens, J.; Verboom,W. Dalton Trans. 2012, 41 (23), 6970. doi: 10.1039/c2dt12364a
10. [10]
  (14) Papaiconomou, N.; Genand-Pinaz, S.; Leveque, J. M.; Guittonneau, S. Dalton Trans. 2013, 42 (6), 1979. doi: 10.1039/c2dt32631k
11. [11]
  (15) Stepinski, D. C.; Jensen, M. P.; Dzielawa, J. A.; Dietz, M. L. Green Chem. 2005, 7 (3), 151. doi: 10.1039/b414756a
12. [12]
  (16) Luo, H. M.; Dai, S.; Bonnesen, P. V.; Buchanan, A. C.; Holbrey, J. D.; Bridges, N. J.; Rogers, R. D. Anal. Chem. 2004, 76 (11), 3078. doi: 10.1021/ac049949k
13. [13]
  (17) Visser, A. E.; Rogers, R. D. J. Solid State Chem. 2003, 171 (1-2), 109. doi: 10.1016/S0022-4596(02)00193-7
14. [14]
  (18) Rao, C. J.; Venkatesan, K. A.; Tata, B. V. R.; Nagarajan, K.; Srinivasan, T. G.; Rao, P. R. V. Radiat. Phys. Chem. 2011, 80 (5), 643. doi: 10.1016/j.radphyschem.2011.01.012
15. [15]
  (19) Bhatt, A. I.; May, I.; Volkovich, V. A.; Collison, D.; Helliwell, M.; Polovov, I. B.; Lewin, R. G. Inorg. Chem. 2005, 44 (14), 4934. doi: 10.1021/ic048199u
16. [16]
  (20) Bhatt, A. I.; Duffy, N.W.; Collison, D.; May I.; Lewin, R. G. Inorg. Chem. 2006, 45 (4), 1677. doi: 10.1021/ic051750i
17. [17]
  (21) Allen, D.; Baston, G.; Bradley, A. E.; rman, T.; Haile, A.; Hamblett, I.; Hatter, J. E.; Healey, M. J. F.; Hodgson, B.; Lewin, R.; Lovell, K. V.; Newton, B.; Pitner,W. R.; Rooney, D.W.; Sanders, D.; Seddon, K. R.; Sims, H. E.; Thied, R. C. Green Chem. 2002, 4 (2), 152. doi: 10.1039/b111042j
18. [18]
  (22) Berthon, L.; Nikitenko, S. I.; Bisel, I.; Berthon, C.; Faucon, M.; Saucerotte, B.; Zorz, N.; Moisy, P. Dalton Trans. 2006, No. 21, 2526.(23) Bosse, E.; Berthon, L.; Zorz, N.; Monget, J.; Berthon, C.; Bisel, I.; Legand, S.; Moisy, P. Dalton Trans. 2008, No. 7, 924.(24) Le Rouzo, G.; Lamouroux, C.; Dauvois, V.; Dannoux, A.; Legand, S.; Durand, D.; Moisy, P.; Moutiers, G. Dalton Trans. 2009, No. 31, 6175.(25) Qi, M. Y.;Wu, G. Z.; Chen, S. M.; Liu, Y. D. Radiat. Res. 2007, 167 (5), 508. doi: 10.1667/RR0727.1
19. [19]
  (26) Qi, M. Y.;Wu, G. Z.; Li, Q. M.; Luo, Y. S. Radiat. Phys. Chem. 2008, 77 (7), 877. doi: 10.1016/j.radphyschem.2007.12.007
20. [20]
  (27) Huang,W.; Chen, S. M.; Liu, Y. S.; Fu, H. Y.;Wu, G. Z. Radiat. Phys. Chem. 2011, 80 (4), 573. doi: 10.1016/j.radphyschem.2010.12.012
21. [21]
  (28) Huang,W.; Chen, S. M.; Fu, H. Y.;Wu, G. Z. Radiat. Res. 2010, 174 (5), 650. doi: 10.1667/RR2170.1
22. [22]
  (29) Huang, L.; Huang,W.; Fu, H. Y.;Wu, G. Z.; Guo, Z. J.;Wu,W. S.; Chen, S. M. Chin. Sci. Bull. 2013, 58 (10), 1150. doi: 10.1007/s11434-012-5656-3
23. [23]
  (30) Gao, S. Y.; Dou, H.; Ding, L. S.; ng, P.; Luo, L.; Chen, D. Radiat. Prot. 2012, 32 (1), 21. [高思旖, 窦辉, 丁立生, 龚频, 罗亮, 陈达. 辐射防护, 2012, 32 (1), 21.] doi: 10.1088/0952-4746/32/1/N21
24. [24]
  (31) Howett, S. E.; Joseph, J. M.; Noel, J. J.;Wren, J. C. J. Colloid Interface Sci. 2011, 361 (1), 338. doi: 10.1016/j.jcis.2011.05.034
25. [25]
  (32) Cui, Z. P.;Wang, S. J.; Ao, Y. Y.; Peng, J.; Li, J. Q.; Zhai, M. L. Acta Phys. -Chim. Sin. 2013, 29 (3), 619. [崔振鹏, 王硕珏, 敖银勇, 彭静, 李久强, 翟茂林. 物化化学学报, 2013, 29 (3), 619.] doi: 10.3866/PKU.WHXB201212102
26. [26]
  (33) Yuan, L. Y.; Peng, J.; Xu, L.; Zhai, M. L.; Li, J. Q.;Wei, G. S. Radiat. Phys. Chem. 2009, 78 (12), 1133. doi: 10.1016/j.radphyschem.2009.07.003
27. [27]
  (34) Yuan, L. Y.; Peng, J.; Li, J. Q.; Zhai, M. L. Acta Phys. -Chim. Sin. 2010, 26 (4), 981. [袁立永, 彭静, 李久强, 翟茂林. 物化化学学报, 2010, 26 (4), 981.] doi: 10.3866/PKU.WHXB20100423
28. [28]
  (35) Paul, A.; Mandal, P. K.; Samanta, A. Chem. Phys. Lett. 2005, 402 (4-6), 375. doi: 10.1016/j.cplett.2004.12.060
29. [29]
  (36) Paul, A.; Mandal, P. K.; Samanta, A. J. Phys. Chem. B 2005, 109 (18), 9148. doi: 10.1021/jp0503967
30. [30]
  (37) Yuan, L. Y.; Peng, J.; Zhai, M. L.; Li, J. Q.;Wei, G. S. Radiat. Phys. Chem. 2009, 78 (7-8), 737. doi: 10.1016/j.radphyschem.2009.03.064
31. [31]
  (38) Shkrob, I. A.; Marin, T.W.; Chemerisov, S. D.; Hatcher, J. L.; Wishart, J. F. J. Phys. Chem. B 2011, 115 (14), 3889. doi: 10.1021/jp200305b
32. [32]
  (39) Tarabek, P.; Liu, S. Y.; Haygarth, K.; Bartels, D. M. Radiat. Phys. Chem. 2009, 78 (3), 168. doi: 10.1016/j.radphyschem.2008.11.006
33. [33]
  (40) Dhiman, S. B.; ff, G. S.; Runde,W.; LaVerne, J. A. J. Phys. Chem. B 2013, 117 (22), 6782. doi: 10.1021/jp402502d
34. [34]
  (41) Yuan, L. Y.; Peng, J.; Xu, L.; Zhai, M. L.; Li, J. Q.;Wei, G. S. Dalton Trans. 2008, No. 45, 6358.(42) Yuan, L. Y.; Peng, J.; Xu, L.; Zhai, M. L.; Li, J. Q.;Wei, G. S. J. Phys. Chem. B 2009, 113 (26), 8948. doi: 10.1021/jp9016079
35. [35]
  (43) Yuan, L. Y.; Xu, C.; Peng, J.; Xu, L.; Zhai, M. L.; Li, J. Q.;Wei, G. S.; Shen, X. H. Dalton Trans. 2009, No. 38, 7873.(44) Sun, T. X.; Shen, X. H.; Chen, Q. D.; Ma, J. Y.; Zhang, S.; Huang, Y. Y. Radiat. Phys. Chem. 2013, 83, 74.(45) Ao, Y. Y.; Peng, J.; Yuan, L. Y.; Cui, Z. P.; Li, C.; Li, J. Q.; Zhai, M. L. Dalton Trans. 2013, 42 (12), 4299. doi: 10.1039/c2dt32418k
36. [36]
  (46) Ao, Y. Y.; Zhou, H. Y.; Yuan,W. J.;Wang, S. J.; Peng, J.; Zhai, M. L.;Wang, J. Y.; Zhao, Z. Q.; Zhao, L.;Wei, Y. Z. Dalton Trans. 2014, 43 (14), 5580. doi: 10.1039/c3dt53297f
37. [37]
  (47) Behar, D.; nzalez, C.; Neta, P. J. Phys. Chem. A 2001, 105 (32), 7607. doi: 10.1021/jp011405o
38. [38]
  (48) Marcinek, A.; Zielonka, J.; Gebicki, J.; rdon, C. M.; Dunkin, I. R. J. Phys. Chem. A 2001, 105 (40), 9305. doi: 10.1021/jp0117718
39. [39]
  (49) Wishart, J. F.; Neta, P. J. Phys. Chem. B 2003, 107 (30), 7261. doi: 10.1021/jp027792z
40. [40]
  (50) Rogers, R. D.; Seddon, K. R.;Wishart, J. F. Ionic Liquids III A: Fundamentals, Progress, Challenges, and Opportunities ; American Chemical Society:Washington, DC, 2005; pp 102-116.(51) Shkrob, I. A.; Chemerisov, S. D.;Wishart, J. F. J. Phys. Chem. B 2007, 111 (40), 11786. doi: 10.1021/jp073619x
41. [41]
  (52) Shkrob, I. A.; Marin, T.W.; Chemerisov, S. D.;Wishart, J. F. J. Phys. Chem. B 2011, 115 (14), 3872. doi: 10.1021/jp2003062
42. [42]
  (53) Shkrob, I. A.; Marin, T.W.; Chemerisov, S. D.;Wishart, J. F. J. Phys. Chem. B 2011, 115 (37), 10927. doi: 10.1021/jp206579j
43. [43]
  (54) Shkrob, I. A.; Marin, T.W.; Luo, H.; Dai, S. J. Phys. Chem. B 2013, 117 (46), 14372. doi: 10.1021/jp4082432
44. [44]
  (55) Shkrob, I. A.; Marin, T.W.; Hatcher, J. L.; Cook, A. R.; Szreder, T.;Wishart, J. F. J. Phys. Chem. B 2013, 117 (46), 14385. doi: 10.1021/jp408242b
45. [45]
  (56) Shkrob, I. A.; Marin, T.W.; Bell, J. R.; Luo, H.; Dai, S. J. Phys. Chem. B 2013, 117 (46), 14400. doi: 10.1021/jp408253y
46. [46]
  (57) Shkrob, I. A.; Marin, T.W. J. Phys. Chem. B 2013, 117 (47), 14797. doi: 10.1021/jp408252n
47. [47]
  (58) Zhu, G. L.;Wu, G. Z.; Long, D.W.; Sha, M. L.; Yao, S. Nucl. Sci. Tech. 2007, 18 (1), 16. doi: 10.1016/S1001-8042(07)60011-6
48. [48]
  (59) Grodkowski, J.; Neta, P. J. Phys. Chem. A 2002, 106 (39), 9030. doi: 10.1021/jp020806g
49. [49]
  (60) Grodkowski, J.; Neta, P.;Wishart, J. F. J. Phys. Chem. A 2003, 107 (46), 9794. doi: 10.1021/jp035265p
50. [50]
  (61) Wishart, J. F.; Lall-Ramnarine, S. I.; Raju, R.; Scumpia, A.; Bellevue, S.; Ragbir, R.; Engel, R. Radiat. Phys. Chem. 2005, 72 (2-3), 99. doi: 10.1016/j.radphyschem.2004.09.005
51. [51]
  (62) Asano, A.; Yang, J. F.; Kondoh, T.; Norizawa, K.; Nagaishi, R.; Takahashi, K.; Yoshida, Y. Radiat. Phys. Chem. 2008, 77 (10-12), 1244. doi: 10.1016/j.radphyschem.2008.05.032
52. [52]
  (63) Takahashi, K.; Sato, T.; Katsumura, Y.; Yang, J. F.; Kondoh, T.; Yoshida, Y.; Katoh, R. Radiat. Phys. Chem. 2008, 77 (10-12), 1239. doi: 10.1016/j.radphyschem.2008.05.042
53. [53]
  (64) Zhu, G. L.; Xu, J. J.;Wu, G. Z.; Zhu, H. P.; Long, D.W.; Chen, S.; Yao, S. D. Int. J. Mol. Sci. 2006, 7 (12), 590. doi: 10.3390/i7120590
54. [54]
  (65) Fu, H. Y.; Xing, Z. G.;Wu, G. Z.; Yao, S. D. Res. Chem. Intermediat. 2011, 37 (1), 79. doi: 10.1007/s11164-010-0226-2
55. [55]
  (66) Shkrob, I. A.; Marin, T.W.; Chemerisov, S. D.; Hatcher, J.; Wishart, J. F. J. Phys. Chem. B 2012, 116 (30), 9043. doi: 10.1021/jp302151c
56. [56]
  (67) Xu, C.; Yuan, L. Y.; Shen, X. H.; Zhai, M. L. Dalton Trans. 2010, 39 (16), 3897. doi: 10.1039/b925594j
1. [1]
  Lihui Jiang , Wanrong Dong , Hua Yang , Yongqing Xia , Hongjian Peng , Jun Yuan , Xiaoqian Hu , Zihan Zeng , Yingping Zou , Yiming Luo . Study on Extraction of p-Hydroxyacetophenone. University Chemistry, 2024, 39(11): 259-268. doi: 10.12461/PKU.DXHX202402056
2. [2]
  Wenjun Zheng . Application in Inorganic Synthesis of Ionic Liquids. University Chemistry, 2024, 39(8): 163-168. doi: 10.3866/PKU.DXHX202401020
3. [3]
  Kexin Dong , Chuqi Shen , Ruyu Yan , Yanping Liu , Chunqiang Zhuang , Shijie Li . Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation. Acta Physico-Chimica Sinica, 2024, 40(10): 2310013-. doi: 10.3866/PKU.WHXB202310013
4. [4]
  Zunxiang Zeng , Yuling Hu , Yufei Hu , Hua Xiao . Analysis of Plant Essential Oils by Supercritical CO₂Extraction with Gas Chromatography-Mass Spectrometry: An Instrumental Analysis Comprehensive Experiment Teaching Reform. University Chemistry, 2024, 39(3): 274-282. doi: 10.3866/PKU.DXHX202309069
5. [5]
  Yanhui Zhong , Ran Wang , Zian Lin . Analysis of Halogenated Quinone Compounds in Environmental Water by Dispersive Solid-Phase Extraction with Liquid Chromatography-Triple Quadrupole Mass Spectrometry. University Chemistry, 2024, 39(11): 296-303. doi: 10.12461/PKU.DXHX202402017
6. [6]
  Yingran Liang , Fei Wang , Jiabao Sun , Hongtao Zheng , Zhenli Zhu . Construction and Application of a New Experimental Device for Determination of Alkaline Metal Elements by Plasma Atomic Emission Spectrometry Based on Solution Cathode Glow Discharge: An Alternative Approach for Fundamental Teaching Experiments in Emission Spectroscopy. University Chemistry, 2024, 39(5): 380-387. doi: 10.3866/PKU.DXHX202312024
7. [7]
  Wei Li , Guoqiang Feng , Ze Chang . Teaching Reform of X-ray Diffraction Using Synchrotron Radiation in Materials Chemistry. University Chemistry, 2024, 39(3): 29-35. doi: 10.3866/PKU.DXHX202308060
8. [8]
  Mei Yan , Rida Feng , Yerdos·Tohtarkhan , Biao Long , Li Zhou , Chongshen Guo . Expansion and Extension of Liquid Saturated Vapor Measurement Experiment. University Chemistry, 2024, 39(3): 294-301. doi: 10.3866/PKU.DXHX202308103
9. [9]
  Shipeng WANG , Shangyu XIE , Luxian LIANG , Xuehong WANG , Jie WEI , Deqiang WANG . Piezoelectric effect of Mn, Bi co-doped sodium niobate for promoting cell proliferation and bacteriostasis. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1919-1931. doi: 10.11862/CJIC.20240094
10. [10]
  Yaling Chen . Basic Theory and Competitive Exam Analysis of Dynamic Isotope Effect. University Chemistry, 2024, 39(8): 403-410. doi: 10.3866/PKU.DXHX202311093
11. [11]
  YanYuan Jia , Rong Rong , Jie Liu , Jing Guo , GuoYu Jiang , Shuo Guo . Unity is Strength, and Independence Shines: A Science Popularization Experiment on AIE and ACQ Effects. University Chemistry, 2024, 39(9): 349-358. doi: 10.12461/PKU.DXHX202402035
12. [12]
  Xuan Zhou , Yi Fan , Zhuoqi Jiang , Zhipeng Li , Guowen Yuan , Laiying Zhang , Xu Hou . Liquid Gating Mechanism and Basic Properties Characterization: a New Experimental Design for Interface and Surface Properties in the Chemistry “101 Plan”. University Chemistry, 2024, 39(10): 113-120. doi: 10.12461/PKU.DXHX202407111
13. [13]
  Yangrui Xu , Yewei Ren , Xinlin Liu , Hongping Li , Ziyang Lu . 具有高传质和亲和表面的NH₂-UIO-66基疏水多孔液体用于增强CO₂光还原. Acta Physico-Chimica Sinica, 2024, 40(11): 2403032-. doi: 10.3866/PKU.WHXB202403032
14. [14]
  Yongmin Zhang , Shuang Guo , Mingyue Zhu , Menghui Liu , Sinong Li . Design and Improvement of Physicochemical Experiments Based on Problem-Oriented Learning: a Case Study of Liquid Surface Tension Measurement. University Chemistry, 2024, 39(2): 21-27. doi: 10.3866/PKU.DXHX202307026
15. [15]
  Jiaxi Xu , Yuan Ma . Influence of Hyperconjugation on the Stability and Stable Conformation of Ethane, Hydrazine, and Hydrogen Peroxide. University Chemistry, 2024, 39(11): 374-377. doi: 10.3866/PKU.DXHX202402049
16. [16]
  Dan Li , Hui Xin , Xiaofeng Yi . Comprehensive Experimental Design on Ni-based Catalyst for Biofuel Production. University Chemistry, 2024, 39(8): 204-211. doi: 10.3866/PKU.DXHX202312046
17. [17]
  Hong LI , Xiaoying DING , Cihang LIU , Jinghan ZHANG , Yanying RAO . Detection of iron and copper ions based on gold nanorod etching colorimetry. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 953-962. doi: 10.11862/CJIC.20230370
18. [18]
  Xiaochen Zhang , Fei Yu , Jie Ma . 多角度数理模拟在电容去离子中的前沿应用. Acta Physico-Chimica Sinica, 2024, 40(11): 2311026-. doi: 10.3866/PKU.WHXB202311026
19. [19]
  Rui Li , Huan Liu , Yinan Jiao , Shengjian Qin , Jie Meng , Jiayu Song , Rongrong Yan , Hang Su , Hengbin Chen , Zixuan Shang , Jinjin Zhao . 卤化物钙钛矿的单双向离子迁移. Acta Physico-Chimica Sinica, 2024, 40(11): 2311011-. doi: 10.3866/PKU.WHXB202311011
20. [20]
  Doudou Qin , Junyang Ding , Chu Liang , Qian Liu , Ligang Feng , Yang Luo , Guangzhi Hu , Jun Luo , Xijun Liu . Addressing Challenges and Enhancing Performance of Manganese-based Cathode Materials in Aqueous Zinc-Ion Batteries. Acta Physico-Chimica Sinica, 2024, 40(10): 2310034-. doi: 10.3866/PKU.WHXB202310034

Get Citation

PDF

XML

Metrics

PDF Downloads(775)
Abstract views(727)
HTML views(19)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142