Citation: DAI Gao-Peng, LIU Su-Qin, PENG Rong, LUO Tian-Xiong. Fabrication of Bi₂O₃/Bi₂O₃ Nanotube Arrays with High Visible-Light Photocatalytic Activity by Impregnation-Decomposition Method[J]. Acta Physico-Chimica Sinica doi: 10.3866/PKU.WHXB201207041 shu

Fabrication of Bi₂O₃/Bi₂O₃ Nanotube Arrays with High Visible-Light Photocatalytic Activity by Impregnation-Decomposition Method

1.
School of Chemical Engineering and Food Science, Hubei University of Arts and Science, Xiangyang 441053, Hubei Province, P. R. China

Received Date: 28 May 2012
Available Online: 4 July 2012
Fund Project: 湖北省教育厅项目(T201215, Q20122507)资助 (T201215, Q20122507)

Bi₂O₃/TiO₂ nanotube arrays (NTs) were prepared by depositing Bi₂O₃ nanoparticles (NPs) onto the tube wall of self-organized TiO₂ NTs using an impregnation-decomposition method. Chemical composition of the resulting Bi₂O₃/TiO₂ NTs was determined by inductively coupled plasma atomic emission spectrometry (ICP-AES). The prepared samples were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), and UV-visible (UV-Vis) diffuse reflectance spectroscopy. Photocatalytic activity was evaluated by degradation of aqueous methyl orange (MO) solution under visible-light irradiation (λ>400 nm). The Bi₂O₃ nanoparticles were found to be uniformly deposited into the nanotubes. Bi₂O₃/TiO₂ NTs exhibited much higher visible-light activity than pure Bi₂O₃ films and N-TiO₂ NTs, which was attributed to synergistic effects of the strong visible-light absorption of Bi₂O₃/TiO₂ NTs and the heterojunction formed between Bi₂O₃ and TiO₂.
- Bi₂O₃/TiO₂ nanotube array,
- Visible light,
- Photocatalysis,
- Heterojunction,
- Synergetic effect
1. [1]
  
  (1) Tu, Y. F.; Huang, S. Y.; Sang, J. P.; Zou, X.W. Mater. Res. Bull.2010, 45, 224. doi: 10.1016/j.materresbull.2009.08.020
2. [2]
  (2) Yu, J. G.; Dai, G. P.; Cheng, B. J. Phys. Chem. C 2010, 114,19378. doi: 10.1021/jp106324x
3. [3]
  (3) Wu, Q.; Su, Y. F.; Sun, L.;Wang, M. Y.;Wang, Y. Y.; Lin, C. J.Acta Phys. -Chim. Sin. 2012, 28, 635. [吴奇, 苏钰丰,孙岚, 王梦晔, 王莹莹, 林昌健. 物理化学学报, 2012, 28,635.] doi: 10.3866/PKU.WHXB201112231
4. [4]
  (4) Liu, Z. Y.; Pesic, B.; Raja, K. S.; Rangaraju, R. R.; Misra, M.Int. J. Hydrog. Energy 2009, 34, 3250. doi: 10.1016/j.ijhydene.2009.02.044
5. [5]
  (5) Mohapatra, S. K.; Misra, M.; Mahajan, V. K.; Raja, K. S.J. Catal. 2007, 246, 362. doi: 10.1016/j.jcat.2006.12.020
6. [6]
  (6) Park, J. H.; Kim, S.; Bard, A. J. Nano Lett. 2006, 6, 24. doi: 10.1021/nl051807y
7. [7]
  (7) Varghese, O. K.; Paulose, M.; Grimes, C. A. Nat. Nanotechnol.2009, 4, 592.
8. [8]
  (8) Li, H. H.; Chen, R. F.; Ma, C.; Zhang, S. L.; An, Z. F.; Huang,W. Acta Phys. -Chim. Sin. 2011, 27, 1017. [李欢欢, 陈润锋,马琮, 张胜兰, 安众福, 黄维. 物理化学学报, 2011, 27,1017.] doi: 10.3866/PKU.WHXB20110514
9. [9]
  (9) Kuang, D.; Brillet, J.; Chen, P.; Takata, M.; Uchida, S.; Miura,H.; Sumioka, K.; Zakeeruddin, S. M.; Grätzel, M. ACS Nano2008, 2, 1113. doi: 10.1021/nn800174y
10. [10]
  (10) Zheng, Q.; Zhou, B. X.; Bai, J.; Li, L. H.; Jin, Z. J.; Zhang, J.L.; Li, J. H.; Liu, Y. B.; Cai,W. M.; Zhu, X. Y. Adv. Mater.2008, 20, 1044. doi: 10.1002/adma.200701619
11. [11]
  (11) Paulose, M.; Varghese, O. K.; Mor, G. K.; Grimes, C. A.; Ong,K. G. Nanotechnology 2006, 17, 398. doi: 10.1088/0957-4484/17/2/009
12. [12]
  (12) Hoffmann, M. R.; Martin, S. T.; Choi,W. Y.; Bahnemann, D.W.Chem. Rev. 1995, 95, 69. doi: 10.1021/cr00033a004
13. [13]
  (13) Berger, T.; Sterrer, M.; Diwald, O.; Knozinger, E.; Panayotov,D.; Thompson, T. L.; Yates, J. T. J. Phys. Chem. B 2005, 109,6061. doi: 10.1021/jp0404293
14. [14]
  (14) Kumar, S.; Fedorov, A. G.; le, J. L. Appl. Catal. B 2005, 57,93. doi: 10.1016/j.apcatb.2004.10.012
15. [15]
  (15) Sun,W. T.; Yu, Y.; Pan, H. Y.; Gao, X. F.; Chen, Q.; Peng, L. M.J. Am. Chem. Soc. 2008, 130, 1124. doi: 10.1021/ja0777741
16. [16]
  (16) Chen, S. G.; Paulose, M.; Ruan, C. M.; Mor, G. K.; Varghese, O.K.;Kouzoudis,D.;Grimes, C.A. J. Photochem. Photobiol. 2006,177, 177. doi: 10.1016/j.jphotochem.2005.05.023
17. [17]
  (17) Zhang, H.; Quan, X.; Chen, S.; Yu, H. T.; Ma, N. Chem. Mater.2009, 21, 3090. doi: 10.1021/cm900100k
18. [18]
  (18) Shin, K.; Seok, S. I.; Im, S. H.; Park, J. H. Chem. Commun.2010, 46, 2385. doi: 10.1039/b923022j
19. [19]
  (19) Seabold, J. A.; Shankar, K.;Wilke, R. H. T.; Paulose, M.;Varghese, O. K.; Grimes, C. A. Chem. Mater. 2008, 20, 5266.doi: 10.1021/cm8010666
20. [20]
  (20) Gao, X. F.; Li, H. B.; Sun,W. T.; Chen, Q.; Tang, F. Q.; Peng, L.M. J. Phys. Chem. C 2009, 113, 7531. doi: 10.1021/jp810727n
21. [21]
  (21) Hou, Y.; Li, X. Y.; Zou, X. J.; Quan, X.; Chen, G. H. Environ. Sci. Technol. 2009, 43, 858. doi: 10.1021/es802420u
22. [22]
  (22) Lee, M. K.; Shih, T. H. J. Electrochem. Soc. 2007, 154, 49.
23. [23]
  (23) Bessekhouad, Y.; Robert, D.;Weber, J. V. Catal. Today 2005,101, 315. doi: 10.1016/j.cattod.2005.03.038
24. [24]
  (24) Zhang, L. S.;Wang,W. Z.; Yang, J.; Chen, Z. G.; Zhang,W. Q.;Zhou, L.; Liu, S.W. Appl. Catal. A 2006, 308, 105. doi: 10.1016/j.apcata.2006.04.016
25. [25]
  (25) Zhou, L.;Wang,W. Z.; Xu, H. L.; Sun, S. M.; Shang, M. Chem. Eur. J. 2009, 15, 1776. doi: 10.1002/chem.200801234
26. [26]
  (26) Hameed, A.; mbac, V.; Montini, T.; Felisri, L.; Fornasiero, P.Chem. Phys. Lett. 2009, 483, 254. doi: 10.1016/j.cplett.2009.10.087
27. [27]
  (27) Bian, Z. F.; Zhu, J.;Wang, S. H.; Cao, Y.; Qian, X. F.; Li, H. X.J. Phys. Chem. C 2008, 112, 6258. doi: 10.1021/jp800324t
28. [28]
  (28) Shamaila, S.; Sajjad, A. K. L.; Chen, F.; Zhang, J. L. Appl. Catal. B 2010, 94, 272. doi: 10.1016/j.apcatb.2009.12.001
29. [29]
  (29) Prakasam, H. E.; Shankar, K.; Paulose, M.; Varghese, O. K.;Grimes, C. A. J. Phys. Chem. C 2007, 111, 7235. doi: 10.1021/jp070273h
30. [30]
  (30) Lai, Y. K.; Huang, J. Y.; Zhang, H. F.; Subramaniam, V. P.; Tang,Y. X.; ng, D. G.; Sundar, L.; Sun, L.; Chen, Z.; Lin, C. J.J. Hazard. Mater. 2010, 184, 855. doi: 10.1016/j.jhazmat.2010.08.121
31. [31]
  (31) Yu, J. G.; Yu, H. G.; Cheng, B.; Zhao, X. J.; Yu, J. C.; Ho,W. K.J. Phys. Chem. B 2003, 107, 13871. doi: 10.1021/jp036158y
32. [32]
  (32) Zhu, H. M.; Yang, B. F.; Xu, J.; Fu, Z. P.;Wen, M.W.; Guo, T.;Fu, S. Q.; Zuo, J.; Zhang, S. Y. Appl. Catal. B 2009, 90, 463.doi: 10.1016/j.apcatb.2009.04.006
33. [33]
  (33) Linsebigler, A. L.; Lu, G. Q.; Yates, J. T. Chem. Rev. 1995, 95,735. doi: 10.1021/cr00035a013
34. [34]
  (34) Kim, Y. I.; Atherton, S. J.; Brigham, E. S.; Mallouk, T. E.J. Phys. Chem. 1993, 97, 11802. doi: 10.1021/j100147a038
35. [35]
  (35) Butler, M. A.; Ginley, D. S. J. Electrochem. Soc. 1978, 125, 228.doi: 10.1149/1.2131419
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Fabrication of Bi2O3/Bi2O3 Nanotube Arrays with High Visible-Light Photocatalytic Activity by Impregnation-Decomposition Method

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通讯作者: 陈斌, bchen63@163.com

Fabrication of Bi₂O₃/Bi₂O₃ Nanotube Arrays with High Visible-Light Photocatalytic Activity by Impregnation-Decomposition Method