Citation: HAO Liang, WU Dapeng, GUAN Yafeng. Sample preparation methods for chromatographic analysis of organic components in atmospheric particulate matter[J]. Chinese Journal of Chromatography, ;2014, 32(9): 906-912. doi: 10.3724/SP.J.1123.2014.07045 shu

Sample preparation methods for chromatographic analysis of organic components in atmospheric particulate matter

HAO Liang ^1,2 ,
WU Dapeng ¹ ,
GUAN Yafeng ^1,,

1.
1. Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China;

Corresponding author: GUAN Yafeng,
Received Date: 25 July 2014
Available Online: 6 August 2014
Fund Project: 科技部“863计划”项目(2011AA060602). (2011AA060602)

The determination of organic composition in atmospheric particulate matter (PM) is of great importance in understanding how PM affects human health, environment, climate, and ecosystem. Organic components are also the scientific basis for emission source tracking, PM regulation and risk management. Therefore, the molecular characterization of the organic fraction of PM has become one of the priority research issues in the field of environmental analysis. Due to the extreme complexity of PM samples, chromatographic methods have been the chief selection. The common procedure for the analysis of organic components in PM includes several steps: sample collection on the fiber filters, sample preparation (transform the sample into a form suitable for chromatographic analysis), analysis by chromatographic methods. Among these steps, the sample preparation methods will largely determine the throughput and the data quality. Solvent extraction methods followed by sample pretreatment (e. g. pre-separation, derivatization, pre-concentration) have long been used for PM sample analysis, and thermal desorption methods have also mainly focused on the non-polar organic component analysis in PM. In this paper, the sample preparation methods prior to chromatographic analysis of organic components in PM are reviewed comprehensively, and the corresponding merits and limitations of each method are also briefly discussed.
- atmospheric particulate matter,
- organic components,
- sample preparation,
- chromatographic analysis
1. [1]
  [1] McMurry P H. Atmos Environ, 2000, 34(12/13/14): 1959
2. [2]
  [2] Cassee F R, Roux M E H, Gerlofs N M E, et al. Inhal Toxicol, 2013, 25(14): 802
3. [3]
  [3] Turpin B J, Saxena P, Andrews E. Atmos Environ, 2000, 34(18): 2983
4. [4]
  [4] Saxena P, Hildemann L. J Atmos Chem, 1996, 24: 57
5. [5]
  [5] Hays M D, Lavrich R J. TrAC-Trends Anal Chem, 2007, 26(2): 88
6. [6]
  [6] Cochran R E, Dongari N, Jeong H, et al. Anal Chim Acta, 2012, 740: 93
7. [7]
  [7] Pietrogrande M C, Bacco D, Chiereghin S. Anal Bio Chem, 2013, 405(2/3): 1095
8. [8]
  [8] Jimenez J R, Parshintsev J, Laitinen T, et al. Anal Meth, 2011, 3(11): 2501
9. [9]
  [9] Coscollà C, Castillo M, Pastor A, et al. Anal Chim Acta, 2011, 693(9): 72
10. [10]
  [10] Hart E, Coscolla C, Pastor A, et al. Atmos Environ, 2012, 62: 118
11. [11]
  [11] Schantz M M, McGaw E, Wise S A. Anal Chem, 2012, 84(19): 8222
12. [12]
  [12] Piazza R, Gambaro A, Argiriadis E, et al. Anal Bioanal Chem, 2013, 405(2/3): 917
13. [13]
  [13] Zhou Y S, Wang H W, Guan Y F. Chinese Journal of Analytical Chemistry (周延生, 王涵文, 关亚风. 分析化学), 2004, 32(8): 983
14. [14]
  [14] Zhou Y S, Liu W M, Zhao J H, et al. Chinese Journal of Analytical Chemistry (周延生, 刘文民, 赵景红, 等. 分析化学), 2005, 33(9): 1231
15. [15]
  [15] Shimmo M, Hyotylainen T, Hartonen K, et al. J Microcolumn Sep, 2001, 13(5): 202
16. [16]
  [16] Castells P, Santos F J, Gaiceran M T. J Chromatogr A, 2003, 1010(2): 141
17. [17]
  [17] Kotianová P, Matisová E, Puxbaum H, et al. Chem Anal, 2004, 49: 833
18. [18]
  [18] van Pinxteren D, Teich M, Herrmann H. J Chromatogr A, 2012, 1267: 178
19. [19]
  [19] Menezes H C, Cardeal Z D L. J Chromatogr A, 2011, 1218(21): 3300
20. [20]
  [20] Alvarez A O, Cuadra R L, Gonzalez I F, et al. Anal Chim Acta, 2007, 597(2): 273
21. [21]
  [21] Chow J C, Yu J Z, Watson J G, et al. J Environ Sci Health Part A, 2007, 42(11): 1521
22. [22]
  [22] Greaves R C, Barkley R M, Sievers R E. Anal Chem, 1985, 57: 2807
23. [23]
  [23] Hays M D, Smith N D, Kinsey J, et al. J Aerosol Sci, 2003, 34(8): 1061
24. [24]
  [24] Hays M D, Smith N D, Dong Y J. J Geophy Res Atmos, 2004, 109(D16): 1
25. [25]
  [25] Meng H, Zhao J H, Duan C F, et al. Chinese Journal of Analytical Chemistry (孟虎, 赵景红, 段春凤, 等. 分析化学), 2014, 42(7): 931
26. [26]
  [26] Waterman D, Horsfield B, Leistner F, et al. Anal Chem, 2000, 72: 3563
27. [27]
  [27] Gil-Molto J, Varea M, Galindo N, et al. J Chromatogr A, 2009, 1216(9): 1285
28. [28]
  [28] Ding L C, Ke F, Wang D K W, et al. Atmos Environ, 2009, 43(32): 4894
29. [29]
  [29] Yadav S, Tandon A, Attri A K. J Hazard Mater, 2013, 252/253: 29
30. [30]
  [30] Grandesso E, Ballesta P P, Kowalewski K. Talanta, 2013, 105: 101
31. [31]
  [31] Falkovich A H, Rudich Y. Environ Sci Tech, 2001, 35(11): 2326
32. [32]
  [32] Yu J Z, Huang X H H, Ho S S H, et al. Anal Bioanal Chem, 2011, 401(10): 3125
33. [33]
  [33] Ho S S H, Yu J Z, Chow J C, et al. J Chromatogr A, 2008, 1200(2): 217
34. [34]
  [34] Ho S S H, Yu J Z. J Chromatogr A, 2004, 1059(1/2): 121
35. [35]
  [35] Williams B J, Goldstein A H, Kreisberg N M, et al. Aerosol Sci Tech, 2006, 40(8): 627
36. [36]
  [36] Beiner K, Plewka A, Haferkorn S, et al. J Chromatogr A, 2009, 1216(38): 6642
37. [37]
  [37] Sheesley R J, Deminter J T, Meiritz M, et al. Environ Sci Tech, 2010, 44(24): 9398
38. [38]
  [38] Orasche J, Schnelle K J, Abbaszade G, et al. Atmos Chem Phys, 2011, 11(17): 8977
39. [39]
  [39] Jeon S J, Meuzelaar H L C, Sheya S A N, et al. J Air Waste Manage Assoc, 2001, 51(5): 766
40. [40]
  [40] Hansen K J, Nansen B N, Cravens E, et al. Anal Chem, 1995, 67(19): 3541
41. [41]
  [41] Neususs C, Pelzing M P A, Herrmann H. J Geophys Res, 2000, 105(D4): 4513
1. [1]
  Fan Wu , Wenchang Tian , Jin Liu , Qiuting Zhang , YanHui Zhong , Zian Lin . Core-Shell Structured Covalent Organic Framework-Coated Silica Microspheres as Mixed-Mode Stationary Phase for High Performance Liquid Chromatography. University Chemistry, 2024, 39(11): 319-326. doi: 10.12461/PKU.DXHX202403031
2. [2]
  Bao Jia , Yunzhe Ke , Shiyue Sun , Dongxue Yu , Ying Liu , Shuaishuai Ding . Innovative Experimental Teaching for the Preparation and Modification of Conductive Organic Polymer Thin Films in Undergraduate Courses. University Chemistry, 2024, 39(10): 271-282. doi: 10.12461/PKU.DXHX202404121
3. [3]
  Zunxiang Zeng , Yuling Hu , Yufei Hu , Hua Xiao . Analysis of Plant Essential Oils by Supercritical CO₂Extraction with Gas Chromatography-Mass Spectrometry: An Instrumental Analysis Comprehensive Experiment Teaching Reform. University Chemistry, 2024, 39(3): 274-282. doi: 10.3866/PKU.DXHX202309069
4. [4]
  Yuanpei ZHANG , Jiahong WANG , Jinming HUANG , Zhi HU . Preparation of magnetic mesoporous carbon loaded nano zero-valent iron for removal of Cr(Ⅲ) organic complexes from high-salt wastewater. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1731-1742. doi: 10.11862/CJIC.20240077
5. [5]
  Feng Han , Fuxian Wan , Ying Li , Congcong Zhang , Yuanhong Zhang , Chengxia Miao . Comprehensive Organic Chemistry Experiment: Phosphotungstic Acid-Catalyzed Direct Conversion of Triphenylmethanol for the Synthesis of Oxime Ethers. University Chemistry, 2025, 40(3): 342-348. doi: 10.12461/PKU.DXHX202405181
6. [6]
  Ran HUO , Zhaohui ZHANG , Xi SU , Long CHEN . Research progress on multivariate two dimensional conjugated metal organic frameworks. Chinese Journal of Inorganic Chemistry, 2024, 40(11): 2063-2074. doi: 10.11862/CJIC.20240195
7. [7]
  Bin HE , Hao ZHANG , Lin XU , Yanghe LIU , Feifan LANG , Jiandong PANG . Recent progress in multicomponent zirconium?based metal-organic frameworks. Chinese Journal of Inorganic Chemistry, 2024, 40(11): 2041-2062. doi: 10.11862/CJIC.20240161
8. [8]
  Yanhui Zhong , Ran Wang , Zian Lin . Analysis of Halogenated Quinone Compounds in Environmental Water by Dispersive Solid-Phase Extraction with Liquid Chromatography-Triple Quadrupole Mass Spectrometry. University Chemistry, 2024, 39(11): 296-303. doi: 10.12461/PKU.DXHX202402017
9. [9]
  Wendian XIE , Yuehua LONG , Jianyang XIE , Liqun XING , Shixiong SHE , Yan YANG , Zhihao HUANG . Preparation and ion separation performance of oligoether chains enriched covalent organic framework membrane. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1528-1536. doi: 10.11862/CJIC.20240050
10. [10]
  Tianyun Chen , Ruilin Xiao , Xinsheng Gu , Yunyi Shao , Qiujun Lu . Synthesis, Crystal Structure, and Mechanoluminescence Properties of Lanthanide-Based Organometallic Complexes. University Chemistry, 2024, 39(5): 363-370. doi: 10.3866/PKU.DXHX202312017
11. [11]
  Zelong LIANG , Shijia QIN , Pengfei GUO , Hang XU , Bin ZHAO . Synthesis and electrocatalytic CO₂ reduction performance of metal-organic framework catalysts loaded with silver particles. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 165-173. doi: 10.11862/CJIC.20240409
12. [12]
  Jingjing QING , Fan HE , Zhihui LIU , Shuaipeng HOU , Ya LIU , Yifan JIANG , Mengting TAN , Lifang HE , Fuxing ZHANG , Xiaoming ZHU . Synthesis, structure, and anticancer activity of two complexes of dimethylglyoxime organotin. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1301-1308. doi: 10.11862/CJIC.20240003
13. [13]
  Liang TANG , Jingfei NI , Kang XIAO , Xiangmei LIU . Synthesis and X-ray imaging application of lanthanide-organic complex-based scintillators. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1892-1902. doi: 10.11862/CJIC.20240139
14. [14]
  Jiaming Xu , Yu Xiang , Weisheng Lin , Zhiwei Miao . Research Progress in the Synthesis of Cyclic Organic Compounds Using Bimetallic Relay Catalytic Strategies. University Chemistry, 2024, 39(3): 239-257. doi: 10.3866/PKU.DXHX202309093
15. [15]
  Aidang Lu , Yunting Liu , Yanjun Jiang . Comprehensive Organic Chemistry Experiment: Synthesis and Characterization of Triazolopyrimidine Compounds. University Chemistry, 2024, 39(8): 241-246. doi: 10.3866/PKU.DXHX202401029
16. [16]
  .
  CCS Chemistry 综述推荐│绿色氧化新思路：光/电催化助力有机物高效升级
  . CCS Chemistry, 2025, 7(10.31635/ccschem.024.202405369): -.
17. [17]
  Qiuyang LUO , Xiaoning TANG , Shu XIA , Junnan LIU , Xingfu YANG , Jie LEI . Application of a densely hydrophobic copper metal layer in-situ prepared with organic solvents for protecting zinc anodes. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1243-1253. doi: 10.11862/CJIC.20240110
18. [18]
  Ling Zhang , Jing Kang . Turn Waste into Valuable: Preparation of High-Strength Water-Based Adhesives from Polymethylmethacrylate Wastes: a Comprehensive Chemical Experiments. University Chemistry, 2024, 39(2): 221-226. doi: 10.3866/PKU.DXHX202306075
19. [19]
  Yukun Chang , Haoqin Huang , Baolei Wang . Preparation of Trans-Cinnamic Acid via “One-Pot” Protocol of Aldol Condensation-Hydrolysis Reaction: Recommending an Improved Organic Synthesis Experiment. University Chemistry, 2024, 39(4): 322-328. doi: 10.3866/PKU.DXHX202309095
20. [20]
  Guodong Xu , Chengcai Sheng , Xiaomeng Zhao , Tuojiang Zhang , Zongtang Liu , Jun Dong . Reform of Comprehensive Organic Chemistry Experiments in the Context of Emerging Engineering Education: A Case Study on the Improved Preparation of Benzocaine. University Chemistry, 2024, 39(11): 286-295. doi: 10.12461/PKU.DXHX202403094

Get Citation

PDF

XML

Metrics

PDF Downloads(0)
Abstract views(533)
HTML views(80)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142