Citation: LIU Hui-Min, LAN Yong-Bo, ZHAO Chao-Yue, BAI Tian-Hou, LIU Ji-Feng. Preparation of Cellulose/Iron Metal Organic Framework Loaded Peptide Composites and Their Adsorption Performances for Perfluorooctanoic Acid from Aqueous Environment[J]. Chinese Journal of Analytical Chemistry, ;2023, 51(5): 860-873. doi: 10.19756/j.issn.0253-3820.231006 shu

Preparation of Cellulose/Iron Metal Organic Framework Loaded Peptide Composites and Their Adsorption Performances for Perfluorooctanoic Acid from Aqueous Environment

Tianjin Key Laboratory of Food Quality and Health, State Key Laboratory of Food Nutrition and Safety, Tianjin University of Science and Technology, Tianjin 300457, China

Corresponding author: LIU Ji-Feng,
Received Date: 5 January 2023
Revised Date: 28 February 2023

Fund Project: Supported by the National Key Research and Development Project of China (No. 2020YFF0305002).

A composite material for selective enrichment of perfluorooctanoic acid (PFOA) in aqueous environment was prepared by using the carboxymethyl cellulose/Fe metal organic framework composite aerogel (CMC/MOF) immobilized with andpolypeptide (PEP) as the matrix. The physical and chemical properties of the composite were characterized by scanning electron microscopy, infrared spectroscopy, X-ray diffraction and thermogravimetry. The results showed that the combination of MOF and CMC aerogel material was stable, and the polypeptide selectively combined PFOA on the surface of MOF material through covalent bond. The material had porous structure, uniform morphology and stable crystalline structure. In addition, the adsorption performance of the composite for PFOA was studied by kinetic adsorption and thermodynamic adsorption. The results showed that the adsorption capacity of PFOA was 27.2 mg/g, the adsorption behavior conformed to the Pseudo second-order model and Langmuir isotherm adsorption model, and the adsorption rate tended to single-layer chemical adsorption. The adsorption efficiency of the composite material for PFOA was more than 80% within the concentration range of 50 mg/L, showing that the composite material could be used for the pretreatment of PFOA in real samples.
- Composite aerogel,
- Polypeptide,
- Perfluorooctanoic acid,
- Adsorption capacity,
- Pretreatment material
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