Citation: WANG Gui-Xian, XIA Yan, WANG Xiao-Juan, FENG Yun-Long. DNA-binding Studies of Two Silver(I)-sulfonate Complexes Constructed by In Situ Reaction[J]. Chinese Journal of Structural Chemistry, ;2016, 35(2): 219-226. doi: 10.14102/j.cnki.0254-5861.2011-0841 shu

DNA-binding Studies of Two Silver(I)-sulfonate Complexes Constructed by In Situ Reaction

1.
a Department of Chemistry and Chemical Engineering, Lishui University, Lishui, Zhejiang 323000, China;
2.
b Key Laboratory of the Ministry of Education for Advanced Catalysis Material, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, Zhejiang 321004, China

Corresponding author: FENG Yun-Long,
Received Date: 10 June 2015
Available Online: 11 November 2015
Fund Project: This project was supported by the National Natural Science Foundation of China (No. 21173197) (No. 21173197)

Two silver(I)-sulfonate complexes, [Ag(NO₃)(4,4'-bipy)][Ag(HL)(4,4'-bipy)]·2H₂O (1) and [Ag(H₂O)(4,4'-bipy)][AgL(4,4'-bipy)]·2H₂O (2), have been synthesized by in situ reaction (H₂L = 2-formylbenzenesulfonic acid, 4,4'-bipy = 4,4'-bipyridine). 1 displays two parallel 1D chains expending to a 3D supramolecule by π…π interactions and O-H…O hydrogen bonds, in which the [Ag(NO₃)] or [Ag(HL)] units are joined by bridging 4,4'-bipy molecules, respectively. The interactions between the complexes and DNA were studied by means of fluorescence spectra and surface-enhanced Raman scattering (SERS) spectra. The special configuration and intercalation effects between 1 and DNA are stronger than that between 2 and DNA.
- in situ synthesis,
- Ag(I) complex,
- DNA-binding
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