Citation: Yue-Jiao ZHANG, Petar M RADJENOVIC, Jian-Feng LI. Shell-isolated Nanoparticle-enhanced Raman Spectroscopy towards In-Situ Investigating of Interfacial Structure[J]. Chinese Journal of Structural Chemistry, ;2020, 39(8): 1372-1376. doi: 10.14102/j.cnki.0254–5861.2011–2918 shu

Shell-isolated Nanoparticle-enhanced Raman Spectroscopy towards In-Situ Investigating of Interfacial Structure

College of Energy, State Key Laboratory for Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China

Corresponding author: Jian-Feng LI, li@xmu.edu.cn
Received Date: 23 June 2020
Accepted Date: 15 July 2020

Fund Project: the National Natural Science Foundation of China 21925404the National Natural Science Foundation of China 21775127Science and Technology Planning Project of Fujian Province 2019Y4001

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Since the discovery of surface-enhanced Raman spectroscopy (SERS), it has been rapidly applied to the in situ study of electrochemical interfaces. Shell-isolated nanoparticle-enhanced Raman spectroscopy (SHINERS) stands out as one of the most powerful tools for the in situ study of interfacial structures, especially on well-defined single crystal surface. This perspective paper focuses on the study of interfacial structures with the SHINERS technique, including the electronic structure of heterogeneous metal surfaces, and the detection of molecules absorbed on the surface, as well as intermediate species, during electrochemical reactions. Finally, we present an outlook on future research and development of SHINERS for studying interfacial structures.
- SHINERS,
- single-crystal electrode,
- spectroelectrochemistry,
- interface structure,
- in-situ
1. [1]
  Hoshi, N.; Suzuki, T.; Hori, Y. Step density dependence of CO₂ reduction rate on Pt(S)-[n(111) × (111)] single crystal electrodes. Electrochim. Acta 1996, 41, 1647–1653. doi: 10.1016/0013-4686(95)00418-1
2. [2]
  Maciá, M. D.; Campiña, J. M.; Herrero, E.; Feliu, J. M. On the kinetics of oxygen reduction on platinum stepped surfaces in acidic media. J. Electroanal. Chem. 2004, 564, 141–150. doi: 10.1016/j.jelechem.2003.09.035
3. [3]
  Schouten, K. J. P.; Qin, Z.; Pérez Gallent, E.; Koper, M. T. M. Two pathways for the formation of ethylene in CO reduction on single-crystal copper electrodes. J. Am. Chem. Soc. 2012, 134, 9864–9867. doi: 10.1021/ja302668n
4. [4]
  Gong, J.; Bao, X. Fundamental insights into interfacial catalysis. Chem. Soc. Rev. 2017, 46, 1770–1771. doi: 10.1039/C7CS90022H
5. [5]
  Fleischmann, M.; Hendra, P. J.; McQuillan, A. J. Raman spectra of pyridine adsorbed at a silver electrode. Chem. Phys. Lett. 1974, 26, 163–166. doi: 10.1016/0009-2614(74)85388-1
6. [6]
  Jeanmaire, D. L.; Van Duyne, R. P. Surface Raman spectroelectrochemistry. J. Electroanal. Chem. 1977, 84, 1–20. doi: 10.1016/S0022-0728(77)80224-6
7. [7]
  Li, J. F.; Zhang, Y. J.; Ding, S. Y.; Panneerselvam, R.; Tian, Z. Q. Core-shell nanoparticle-enhanced Raman spectroscopy. Chem. Rev. 2017, 117, 5002–5069. doi: 10.1021/acs.chemrev.6b00596
8. [8]
  Wu, D. Y.; Li, J. F.; Ren, B.; Tian, Z. Q. Electrochemical surface-enhanced Raman spectroscopy of nanostructures. Chem. Soc. Rev. 2008, 37, 1025–1041. doi: 10.1039/b707872m
9. [9]
  Lal, S.; Grady, N. K.; Kundu, J.; Levin, C. S.; Lassiter, J. B.; Halas, N. J. Tailoring plasmonic substrates for surface enhanced spectroscopies. Chem. Soc. Rev. 2008, 37, 898–911. doi: 10.1039/b705969h
10. [10]
  Lei, J.; Ju, H. Signal amplification using functional nanomaterials for biosensing. Chem. Soc. Rev. 2012, 41, 2122–2134. doi: 10.1039/c1cs15274b
11. [11]
  Wang, Y.; Yan, B.; Chen, L. Tags: novel optical nanoprobes for bioanalysis. Chem. Rev. 2013, 113, 1391–1428. doi: 10.1021/cr300120g
12. [12]
  Lane, L. A.; Qian, X. M.; Nie, S. M. SERS nanoparticles in medicine: from label-free detection to spectroscopic tagging. Chem. Rev. 2015, 115, 10489–10529. doi: 10.1021/acs.chemrev.5b00265
13. [13]
  Tian, Z. Q.; Ren, B.; Li, J. F.; Yang, Z. L. Expanding generality of surface-enhanced Raman spectroscopy with borrowing SERS activity strategy. Chem. Commun. 2007, 3514–3534.
14. [14]
  Li, J. F.; Huang, Y. F.; Ding, Y.; Yang, Z. L.; Li, S. B.; Zhou, X. S.; Fan, F. R.; Zhang, W.; Zhou, Z. Y.; Wu, D. Y.; Ren, B.; Wang, Z. L.; Tian, Z. Q. Shell-isolated nanoparticle-enhanced Raman spectroscopy. Nature 2010, 464, 392–395. doi: 10.1038/nature08907
15. [15]
  Zhang, H.; Duan, S.; Radjenovic, P. M.; Tian, Z. Q.; Li, J. F. Core-shell nanostructure-enhanced Raman spectroscopy for surface catalysis. Acc. Chem. Res. 2020, 53, 729–739. doi: 10.1021/acs.accounts.9b00545
16. [16]
  Fang, P. P.; Lu, X. H.; Liu, H.; Tong, Y. X. Applications of shell-isolated nanoparticles in surface-enhanced Raman spectroscopy and fluorescence. Trac-Trend. Anal. Chem. 2015, 66, 103–117. doi: 10.1016/j.trac.2014.11.015
17. [17]
  Greeley, J.; Jaramillo, T. F.; Bonde, J.; Chorkendorff, I.; Nørskov, J. K. Computational high-throughput screening of electrocatalytic materials for hydrogen evolution. Nat. Mater. 2006, 5, 909–913. doi: 10.1038/nmat1752
18. [18]
  Housmans, T. H. M.; Wonders, A. H.; Koper, M. T. M. Structure sensitivity of methanol electrooxidation pathways on platinum: an on-line electrochemical mass spectrometry study. J. Phys. Chem. B 2006, 110, 10021–10031. doi: 10.1021/jp055949s
19. [19]
  Christensen, C. H.; Nørskov, J. K. A molecular view of heterogeneous catalysis. J. Chem. Phys. 2008, 128, 182503. doi: 10.1063/1.2839299
20. [20]
  Zhang, Y. J.; Li, S. B.; Duan, S.; Lu, B. A.; Yang, J.; Panneerselvam, R.; Li, C. Y.; Fang, P. P.; Zhou, Z. Y.; Phillips, D. L.; Li, J. F.; Tian, Z. Q. Probing the electronic structure of heterogeneous metal interfaces by transition metal shelled gold nanoparticle-enhanced Raman spectroscopy. J. Phys. Chem. C 2016, 120, 20684–20691. doi: 10.1021/acs.jpcc.6b01879
21. [21]
  Stamenkovic, V. R.; Fowler, B.; Mun, B. S.; Wang, G.; Ross, P. N.; Lucas, C. A.; Marković, N. M. Improved oxygen reduction activity on Pt₃Ni(111) via increased surface site availability. Science 2007, 315, 493–497. doi: 10.1126/science.1135941
22. [22]
  Li, J. F.; Zhang, Y. J.; Rudnev, A. V.; Anema, J. R.; Li, S. B.; Hong, W. J.; Rajapandiyan, P.; Lipkowski, J.; Wandlowski, T.; Tian, Z. Q. Electrochemical shell-isolated nanoparticle-enhanced Raman spectroscopy: correlating structural information and adsorption processes of pyridine at the Au(hkl) single crystal/solution interface. J. Am. Chem. Soc. 2015, 137, 2400–2408. doi: 10.1021/ja513263j
23. [23]
  Wen, B. Y.; Jin, X.; Li, Y.; Wang, Y. H.; Li, C. Y.; Liang, M. M.; Panneerselvam, R.; Xu, Q. C.; Wu, D. Y.; Yang, Z. L.; Li, J. F.; Tian, Z. Q. Shell-isolated nanoparticle-enhanced Raman spectroscopy study of the adsorption behaviour of DNA bases on Au(111) electrode surfaces. Analyst 2016, 141, 3731–3736. doi: 10.1039/C6AN00180G
24. [24]
  Zhang, S. P.; Lin, J. S.; Lin, R. K.; Radjenovic, P. M.; Yang, W. M.; Xu, J.; Dong, J. C.; Yang, Z. L.; Hang, W.; Tian, Z. Q.; Li, J. F. In situ Raman study of the photoinduced behavior of dye molecules on TiO₂(hkl) single crystal surfaces. Chem. Sci. 2020, 11, 6431–6435. doi: 10.1039/D0SC00588F
25. [25]
  Nørskov, J. K.; Rossmeisl, J.; Logadottir, A.; Lindqvist, L.; Kitchin, J. R.; Bligaard, T.; Jónsson, H. Origin of the overpotential for oxygen reduction at a fuel-cell cathode. J. Phys. Chem. B 2004, 108, 17886–17892. doi: 10.1021/jp047349j
26. [26]
  Ledezma-Yanez, I.; Wallace, W. D. Z.; Sebastián-Pascual, P.; Climent, V.; Feliu, J. M.; Koper, M. T. M. Interfacial water reorganization as a pH-dependent descriptor of the hydrogen evolution rate on platinum electrodes. Nat. Energy 2017, 2, 17031. doi: 10.1038/nenergy.2017.31
27. [27]
  Li, C. Y.; Le, J. B.; Wang, Y. H.; Chen, S.; Yang, Z. L.; Li, J. F.; Cheng, J.; Tian, Z. Q. In situ probing electrified interfacial water structures at atomically flat surfaces. Nat. Mater. 2019, 18, 697–701. doi: 10.1038/s41563-019-0356-x
28. [28]
  Wang, J.; Dong, J. C.; Yang, J.; Wang, Y.; Zhang, C. J.; Xu, M. M.; Mao, B. W.; Yao, J. L.; Li, J. F.; Tian, Z. Q. In situ SERS and SHINERS study of electrochemical hydrogenation of p-ethynylaniline in nonaqueous solvents. Electrochem. Commun. 2017, 78, 16–20. doi: 10.1016/j.elecom.2017.03.015
29. [29]
  Dong, J. C.; Zhang, X. G.; Briega-Martos, V.; Jin, X.; Yang, J.; Chen, S.; Yang, Z. L.; Wu, D. Y.; Feliu, J. M.; Williams, C. T.; Tian, Z. Q.; Li, J. F. In situ Raman spectroscopic evidence for oxygen reduction reaction intermediates at platinum single-crystal surfaces. Nat. Energy 2018, 4, 60–67. doi: 10.1038/s41560-018-0292-z
30. [30]
  Bodappa, N.; Su, M.; Zhao, Y.; Le, J. B.; Yang, W. M.; Radjenovic, P.; Dong, J. C.; Cheng, J.; Tian, Z. Q.; Li, J. F. Early stages of electrochemical oxidation of Cu(111) and polycrystalline Cu surfaces revealed by in situ Raman spectroscopy. J. Am. Chem. Soc. 2019, 141, 12192–12196. doi: 10.1021/jacs.9b04638
31. [31]
  Wang, Y. H.; Wei, J.; Radjenovic, P.; Tian, Z. Q.; Li, J. F. In situ analysis of surface catalytic reactions using shell-isolated nanoparticle-enhanced Raman spectroscopy. Anal. Chem. 2019, 91, 1675–1685. doi: 10.1021/acs.analchem.8b05499
32. [32]
  Dong, J. C.; Su, M.; Briega-Martos, V.; Li, L.; Le, J. B.; Radjenovic, P.; Zhou, X. S.; Feliu, J. M.; Tian, Z. Q.; Li, J. F. Direct in situ Raman spectroscopic evidence of oxygen reduction reaction intermediates at high-index Pt(hkl) surfaces. J. Am. Chem. Soc. 2020, 142, 715–719. doi: 10.1021/jacs.9b12803
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