Citation: Luyuan Zhang, Xibao Li, Dian Bao, Yu Xie, Yingtang Zhou, Yidan Luo, Bin Liu. Research progress on the regulation of asymmetric defect electronic structure of COFs to enhance solar energy conversion[J]. Chinese Chemical Letters, ;2026, 37(12): 113340. doi: 10.1016/j.cclet.2026.113340 shu

Research progress on the regulation of asymmetric defect electronic structure of COFs to enhance solar energy conversion

Luyuan Zhang ^a ,
Xibao Li ^{a, b, *,} ,
Dian Bao ^a ,
Yu Xie ^b ,
Yingtang Zhou ^c ,
Yidan Luo ^a ,
Bin Liu ^d

a.
School of Materials Science and Engineering, Nanchang Hangkong University, Nanchang 330063, China
b.
Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China
c.
Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control, National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan 316004, China
d.
Department of Materials Science and Engineering, City University of Hong Kong, Hong Kong 999077, China

lixibao@nchu.edu.cn

Received Date: 4 June 2026
Revised Date: 10 August 2026
Accepted Date: 24 August 2026
Available Online: 24 August 2026

Figures(7)

Covalent organic frameworks (COFs) are crystalline photocatalytic materials with tunable structures, but their light-to-chemical energy conversion efficiency is limited by severe carrier recombination and inadequate light harvesting. Asymmetric defect engineering relies on lattice distortion, vacancy creation, and asymmetric grafting to induce symmetry breaking of the framework, which serves as an effective means to modulate the electronic structure. This review attempts to systematically demonstrate that this strategy can facilitate the clarification of charge-transfer dynamics through band reconstruction and internal electric field construction, and may further provide insight into energy superposition and sequential electron transfer pathways under multiphoton excitation based on existing theoretical mechanisms. We also summarize strategies for improving photocatalytic performance and discuss recent advances in COF-based materials for photocatalytic energy conversion. Existing challenges, including the precise controllability of defect structures, framework stability, and in-situ quantitative characterization, are critically analyzed, with the aim of offering theoretical guidance for the rational design of efficient COF-based photocatalytic systems.
- COFs,
- Photocatalyst,
- Asymmetric defects,
- Electronic structure control,
- Solar energy conversion efficiency
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