Citation: Jun Wang, Ting Liu, Juping Xu, Guanjie Zhang, Yan Zhao, Huaican Chen, Jinxiang Fan, Sijie Guo, Sidong Zhang, Wen Yin, An-Min Cao. Multi-scale coupled failure mechanisms and stabilization strategies of high-nickel cathodes for next-generation high-energy lithium-ion batteries[J]. Chinese Chemical Letters, ;2026, 37(12): 113100. doi: 10.1016/j.cclet.2026.113100 shu

Multi-scale coupled failure mechanisms and stabilization strategies of high-nickel cathodes for next-generation high-energy lithium-ion batteries

Jun Wang ^{a, b, 1} ,
Ting Liu ^{a, b, 1} ,
Juping Xu ^{a, b} ,
Guanjie Zhang ^{a, b} ,
Yan Zhao ^{a, b} ,
Huaican Chen ^{a, b, *,} ,
Jinxiang Fan ^{c, d} ,
Sijie Guo ^c ,
Sidong Zhang ^{d, *,} ,
Wen Yin ^{a, b, e, *,} ,
An-Min Cao ^{c, d, *,}

a.
Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China
b.
Spallation Neutron Source Science Center, Dongguan 523803, China
c.
CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, and Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, China
d.
School of Chemical Science, University of Chinese Academy of Sciences, Beijing 100049, China
e.
School of Nuclear Science and Technology, University of Chinese Academy of Sciences, Beijing 100049, China

chenhuaican@ihep.ac.cn

zhangsidong@ucas.ac.cn

yinwen@ihep.ac.cn

anmincao@iccas.ac.cn

Received Date: 16 April 2026
Revised Date: 12 June 2026
Accepted Date: 18 June 2026
Available Online: 20 June 2026

Figures(8)

Lithium-ion batteries (LIBs), featuring high energy density and long cycle life, have evolved into a critical technological pillar for global energy transition and dual-carbon target achievement, with fast-growing demand in electric transportation and grid-scale energy storage. High-nickel layered oxides (HNLOs) are widely recognized as one of the most promising cathode candidates for next-generation high-energy-density LIBs, owing to their superior reversible capacity, moderate operating voltage and low material cost. Nevertheless, the continuous increase in nickel content and cutting-off voltage triggers severe chemical, structural and mechanical instability, creating an inherent contradiction between high specific energy and long-term durability, which has become the core bottleneck for their large-scale commercialization. In this review, we systematically elaborate the multi-scale coupled failure mechanisms of HNLOs from a chemical-structural-mechanical perspective, including interfacial parasitic side reactions, irreversible lattice oxygen release, cation mixing-induced phase transformation, and chemo-mechanical failure. We comprehensively summarize state-of-the-art modification strategies, clarify their regulatory mechanisms and evolution from empirical optimization to rational design, identify critical gaps between lab-scale research and industrial application, and propose a holistic design philosophy for high-performance HNLOs. This review provides systematic theoretical and practical guidance for developing durable high-energy-density LIB cathodes.
- Lithium-ion batteries,
- High-nickel layered oxides,
- High energy density,
- Multi-scale coupled failure mechanisms,
- Stabilization strategies
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沈阳化工大学材料科学与工程学院沈阳 110142