Citation: Lingyi Wang, Zhitao Xu, Shuyan Gong, Yang Tian, Sihui Zhan. Photoelectrocatalytic upgrading conversion of biomass-derived alcohols/aldehydes: Regulating the oxidation pathway by designing photoanode materials[J]. Chinese Chemical Letters, ;2026, 37(12): 112722. doi: 10.1016/j.cclet.2026.112722 shu

Photoelectrocatalytic upgrading conversion of biomass-derived alcohols/aldehydes: Regulating the oxidation pathway by designing photoanode materials

Lingyi Wang ^a ,
Zhitao Xu ^a ,
Shuyan Gong ^a ,
Yang Tian ^{a, *,} ,
Sihui Zhan ^{b, *,}

a.
Department of Chemistry, Capital Normal University, Beijing 100048, China
b.
School of Environmental Science and Engineering, Tianjin University, Tianjin 300072, China

tianyang@cnu.edu.cn

shzhan@tju.edu.cn

Received Date: 7 September 2025
Revised Date: 22 December 2025
Accepted Date: 2 April 2026
Available Online: 3 April 2026

Figures(11)

The efficient utilization of biomass energy serves as an effective approach to replace fossil fuels and advance sustainable social development. Among these, alcohols and aldehydes derived from biomass represent crucial basic raw materials in industrial synthesis. Photoelectrocatalysis (PEC) technology has opened a highly competitive pathway for producing high-value-added chemicals, comprehensively meeting requirements for controllable selectivity, green processes, and synergistic systems. These advantages are unparalleled by other methods. However, insufficient product selectivity remains the primary bottleneck before industrialization. This review summarizes the fundamental mechanisms of PEC upgrading of biomass-derived alcohols/aldehydes, along with the selection and design of photoanode materials. It focuses on the role of photoanodes in regulating oxidation pathways: Regulating oxidized depth, selecting oxidized functional group at different positions, controlling oxidized quantity of functional groups, and the C-C bond breakage. Finally, the future development and potential challenges in this field are envisioned on the basis of existing technologies.
- Photoelectrocatalytic,
- Alcohol oxidation,
- Aldehyde oxidation,
- Photoanode,
- Biomass
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沈阳化工大学材料科学与工程学院沈阳 110142