Citation: Yuqi Zhu, Suhua Chen, Jianping Zou, Bo Li, Wei Ren, Gaoxia Zhang, Jiajie Wang, Xinyu Liu, Qianhui Li, Huiying Zhang, Fanying Xia. Single-atom catalysts partner with defects to open a new chapter in catalysis: Synthesis, performances, and mechanisms[J]. Chinese Chemical Letters, ;2026, 37(7): 112192. doi: 10.1016/j.cclet.2025.112192 shu

Single-atom catalysts partner with defects to open a new chapter in catalysis: Synthesis, performances, and mechanisms

Yuqi Zhu ^a ,
Suhua Chen ^{a, *,} ,
Jianping Zou ^{a, *,} ,
Bo Li ^{b, *,} ,
Wei Ren ^a ,
Gaoxia Zhang ^c ,
Jiajie Wang ^a ,
Xinyu Liu ^a ,
Qianhui Li ^a ,
Huiying Zhang ^a ,
Fanying Xia ^a

a.
Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resource Reuse, School of Environmental and Chemical Engineering, Nanchang Hangkong University, Nanchang 330063, China
b.
School of Environment and Energy, South China University of Technology, Guangzhou Higher Education Mega Centre, Guangzhou 510006, China
c.
Carbon Neutrality Research Institute of Power China Jiangxi Electric Power Construction Co. Ltd., Nanchang 330001, China

s-hchen@nchu.edu.cn

zjp_112@126.com

bondboli@163.com

Received Date: 26 May 2025
Revised Date: 7 November 2025
Accepted Date: 26 November 2025
Available Online: 1 December 2025

Figures(4)

Single-atom catalysts (SACs), especially defective-SACs, have been developed into low-cost, high-selectivity and high-performance advanced catalysts due to their unique synergistic effects, and have occupied a place in the energy and environmental fields. However, there is a lack of comprehensive and comprehensive summaries and discussions on the structure-property relationships. Therefore, an exhaustive review on the topic of the synergistic interaction of SACs with defective catalysts is imminent. Firstly, this review offers an overview of the most recent generation pathways of defective-SACs based on SACs and defect formation time differences, with a focus on the important influencing factors in the different synthesis processes. Immediately thereafter, the different roles of defects in the constructed defective-SACs are comprehensively analyzed to unravel the mystery of the high stability and performance of defective-SACs. Subsequently, this article systematically analyzes the synergistic interaction mechanism between defects and SACs from the perspective of reaction mechanisms and explains how this mechanism drives significant performance improvements in various catalytic reactions. The article concludes with limitations of current research and future directions to guide the design of more perfect catalysts for defective-SACs.
- SACs,
- Defects,
- Energy and environmental,
- Mechanisms,
- Interactions
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