Citation: Shuai He, Chao Gong, Mengru Li, Jiahang Wu, Qingjie Xi, Xiaoyu Geng, Xinchao Li, Haijun Nie, Xiaoyan Zhu, Zhenlian Han, Dingsheng Wang, Ligang Wang, Pei Liu. Atomic precision of cobalt single-atom nanozymes in environmental remediation and energy sustainability[J]. Chinese Chemical Letters, ;2026, 37(12): 111906. doi: 10.1016/j.cclet.2025.111906 shu

Atomic precision of cobalt single-atom nanozymes in environmental remediation and energy sustainability

Shuai He ^{a, b} ,
Chao Gong ^b ,
Mengru Li ^b ,
Jiahang Wu ^b ,
Qingjie Xi ^c ,
Xiaoyu Geng ^b ,
Xinchao Li ^b ,
Haijun Nie ^d ,
Xiaoyan Zhu ^b ,
Zhenlian Han ^e ,
Dingsheng Wang ^{f, *,} ,
Ligang Wang ^{c, g, h, *,} ,
Pei Liu ^{a, *,}

a.
College of Biological Engineering, Qingdao University of Science and Technology, Qingdao 266042, China
b.
Faculty of Life Science and Food Engineering, Huaiyin Institute of Technology, Huaian 223003, China
c.
Institute of Molecular Plus, Tianjin University, Tianjin 300072, China
d.
Sino Science and Technology Co., Ltd., Dongying 257000, China
e.
Jiangsu Key Laboratory for Eco-Agricultural Biotechnology around Hongze Lake, School of Life Science, Huaiyin Normal University, Huaian 223300, China
f.
Department of Chemistry, Tsinghua University, Beijing 100084, China
g.
National Industry-Education Platform for Energy Storage, Tianjin University, Tianjin 300350, China
h.
Haihe Laboratory of Sustainable Chemical Transformations, Tianjin 300192, China

wangdingsheng@mail.tsinghua.edu.cn

lgwang_246@tju.edu.cn

liupeiouc@126.com

Received Date: 25 July 2025
Revised Date: 18 September 2025
Accepted Date: 27 September 2025
Available Online: 29 September 2025

Figures(16)

Cobalt single-atom nanozymes (Co-SANs) have emerged as a class of high-performance catalysts with atomic-level precision, offering promising solutions for environmental remediation and energy sustainability. This review systematically elaborates on the rational design principles of Co-SANs, focusing on coordination environment engineering (e.g., N/C coordination, defect engineering) and their structure-activity relationships. Specifically, we highlight their catalytic mechanisms in environmental remediation, encompassing efficient activation of oxidants (peroxymonosulfate, persulfate) for aqueous pollutant degradation (e.g., 4-nitrophenol, bisphenol A, pesticides) and catalytic oxidation of gaseous pollutants (formaldehyde, CO₂). In energy storage and conversion, we discuss applications in advanced energy storage and conversion systems, including Li-S batteries, Zn-air batteries, green hydrogen production, and sustainable H₂O₂ synthesis, emphasizing how atomic-level sites optimize redox kinetics. Finally, we address key challenges, such as synthesis scalability, stability under harsh reaction conditions, and mechanistic ambiguities at the atomic scale, and propose future directions such as machine learning-guided design and hybrid system integration for industrial deployment. This review establishes a comprehensive framework to leverage Co-SANs as catalytic bridges between environmental remediation and energy sustainability.
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