Citation: Meiyu Zhang, Yuanzhe Li, Rakesh Kumar Gupta, Mengjun Lou, Yushan Jiang, Zhen Li, Yalin Zhang, Jiayi Zhang, Xianqiang Huang, Qingde Zhang, Qinggang Sun, Di Sun. Recent advances in polyoxometalates-based photocatalysts for sustainable selective organic transformation[J]. Chinese Chemical Letters, ;2026, 37(12): 111897. doi: 10.1016/j.cclet.2025.111897 shu

Recent advances in polyoxometalates-based photocatalysts for sustainable selective organic transformation

Meiyu Zhang ^{a, 1} ,
Yuanzhe Li ^{a, 1} ,
Rakesh Kumar Gupta ^b ,
Mengjun Lou ^a ,
Yushan Jiang ^a ,
Zhen Li ^a ,
Yalin Zhang ^a ,
Jiayi Zhang ^a ,
Xianqiang Huang ^{a, *,} ,
Qingde Zhang ^c ,
Qinggang Sun ^d ,
Di Sun ^{b, *,}

a.
Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology, School of Chemistry & Chemical Engineering, Liaocheng University, Liaocheng 252059, China
b.
Key Lab of Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong University, Ji’nan 250100, China
c.
State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China
d.
National Rubber Additive Engineering Technology Center, Liaocheng 252059, China

hxq@lcu.edu.cn

dsun@sdu.edu.cn

Received Date: 4 July 2025
Revised Date: 23 September 2025
Accepted Date: 24 September 2025
Available Online: 30 September 2025

Figures(27)

Photocatalytic organic synthesis offers a green, sustainable approach for manufacturing high-value chemicals, addressing critical energy and environmental challenges. Polyoxometalates (POMs)-based photocatalysts, known for their structural tunability, robust redox properties, and thermal stability, have emerged as key players in selective oxidation and coupling reactions. This review highlights recent advances in POMs-based photocatalysts, focusing on strategic modifications such as transition metal doping, hybridization with metal-organic frameworks (MOFs), and integration with semiconductor materials to enhance light absorption, charge separation, and electron transfer efficiency. Applications in controlled oxidation of aromatic alcohols, toluene, and amines are explored, along with discussions on stability and recyclability challenges. Emerging perspectives on optimizing POMs-based photocatalysts for scalable, cost-effective, and durable use in sustainable chemical synthesis are also presented.
- Polyoxometalates,
- Redox properties,
- Photocatalytic,
- Coupling reactions,
- Organic transformation
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沈阳化工大学材料科学与工程学院沈阳 110142