Citation: Feng Liu, Liaofang Shang, Yao Liu, Xinyue Zhang, Chunbo Liu, Guangbo Che, Haiyong Guo, Yaqian Lan. Environmentally friendly Bpy-COF/PThC all-organic heterojunction for efficient removing antibiotic-resistant bacteria and organic pollutants[J]. Chinese Chemical Letters, ;2026, 37(4): 111805. doi: 10.1016/j.cclet.2025.111805 shu

Environmentally friendly Bpy-COF/PThC all-organic heterojunction for efficient removing antibiotic-resistant bacteria and organic pollutants

Feng Liu ^{a, b, c} ,
Liaofang Shang ^d ,
Yao Liu ^{a, b, c} ,
Xinyue Zhang ^{a, b, c} ,
Chunbo Liu ^{a, b, c} ,
Guangbo Che ^{e, *,} ,
Haiyong Guo ^{f, *,} ,
Yaqian Lan ^{g, *,}

a.
Jilin Provincial Key Laboratory of Emerging Contaminants Identification and Control, Jilin Normal University, Siping 136000, China
b.
Key Laboratory of Environmental Materials and Pollution Control, the Education Department of Jilin Province, Jilin Normal University, Siping 136000, China
c.
College of Engineering, Jilin Normal University, Siping 136000,China
d.
College of Chemistry, Jilin Normal University, Siping 136000, China
e.
College of Chemistry, Baicheng Normal University, Baicheng 137000, China
f.
College of Life Science, Jilin Normal University, Siping 136000, China
g.
School of Chemistry, South China Normal University, Guangzhou 510006, China

guangboche@jlnu.edu.cn

guohaiyong78@jlnu.edu.cn

yqlan@m.scnu.edu.cn

Received Date: 22 February 2025
Revised Date: 29 August 2025
Accepted Date: 8 September 2025
Available Online: 9 September 2025

Figures(9)

The extensive use of various antibiotics and organic dyes has led to increasingly severe environmental issues and posed a significant threat to human health. Developing an efficient and safe dual-functional photocatalytic material for degradation and antibacterial purposes is the key to solving environmental pollution problems. Polythiophene and covalent organic frameworks (COFs) possess excellent photophysical properties, high stability, and ease of modification, offering broad application prospects and significant development potential in the removal of organic pollutants and antibiotic-resistant bacteria (ARB). A high-performance conductive polymer PTET-T-COOH (PThC) was prepared via the Stille coupling reaction, and a bipyridine (Bpy) covalent organic framework Bpy-COF was synthesized through acid-catalyzed imine condensation. By utilizing the π-π stacking and hydrogen bonding interactions between Bpy-COF and PThC, a novel Bpy-COF/PThC all-organic heterojunction was successfully fabricated. Compared to Bpy-COF and PThC, the composite exhibits a broadened spectral response range and higher carrier separation efficiency. The 30% Bpy-COF/PThC demonstrates the best photocatalytic performance, achieving a 99.96% inactivation rate of methicillin-resistant Staphylococcus aureus (MRSA) with a cell density of 7.23 log and a 95.28% bactericidal rate of Escherichia coli (E. coli) with a cell density of 7.50 log within 60 min. Under natural light, it not only exhibits good inactivation effects on both MRSA and E. coli, but also shows excellent degradation performance for rhodamine B, methylene blue, and tetracycline. The cytotoxicity experiment demonstrates that the composite exhibits good biocompatibility and potential for practical applications. The research results provide new design ideas for constructing efficient and safe organic photocatalysts, and offer a theoretical basis for the treatment of water pollution.
- Polythiophene,
- Covalent organic framework,
- Heterojunction,
- Photocatalytic antibacterial,
- Pollutant degradation
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沈阳化工大学材料科学与工程学院沈阳 110142