Citation: Mengjiao Xie, Nadeeshani Nanayakkara, Yanbiao Liu. Pulsed electrochemistry for water decontamination: Fundamental principles and environmental application[J]. Chinese Chemical Letters, ;2026, 37(4): 111669. doi: 10.1016/j.cclet.2025.111669 shu

Pulsed electrochemistry for water decontamination: Fundamental principles and environmental application

a.
College of Environmental Science and Engineering, Donghua University, Shanghai 201620, China
b.
Department of Civil Engineering, Faculty of Engineering, University of Peradeniya, Peradeniya 20400, Sri Lanka
c.
School of Environmental Science and Technology, Key Laboratory of Industrial Ecology and Environmental Engineering (Ministry of Education), Dalian University of Technology, Dalian 116024, China

yanbiaoliu@dlut.edu.cn

Received Date: 22 February 2025
Revised Date: 16 June 2025
Accepted Date: 1 August 2025
Available Online: 5 August 2025

Figures(5)

Sustainable and efficient solutions are essential to address increasingly critical environmental issues, particularly in the field of pollutant removal and resource recovery. The latest research has shown that pulsed electrochemistry significantly contributes to these goals by precisely altering the local reaction environment, accelerating the reaction kinetics and decreasing the overall energy requirements. However, knowledge gaps exist in dynamic evolution mechanism of electric double layer (EDL) in this technology, and challenges remain toward fully implementation of this promising technology. In this review, the fundamentals of pulsed electrochemistry and its connection to the theoretical models of EDL are comprehensively presented. The critical parameters (e.g., duty ratio, frequency and waveform) for boosting the performance of the system are systematically discussed and the typical electrochemical reactions that occur with pulsed electrochemistry are outlined. The proposed pulsed electrochemistry methodologies tailored for environmental applications are also reviewed in detail. Finally, future opportunities and challenges of this promising but fledgling field are discussed, with the expectation that this technology offers a route to transform conventional chemical industries into cleaner and more sustainable production.
- Pulsed electrochemistry,
- Fundamental principles,
- Electric double layer,
- Operational parameters,
- Environmental application
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沈阳化工大学材料科学与工程学院沈阳 110142