Citation: Peining Zhu, Xi Guo, Qinqin Yu, Zuyong Wang, Xiangxiao Lei, Zhiwei Zhu, Juan Du, Xiaojia Zhang, Yuan-Li Ding. Design strategies of Si-based anode for solid-state batteries[J]. Chinese Chemical Letters, ;2025, 36(9): 111383. doi: 10.1016/j.cclet.2025.111383 shu

Design strategies of Si-based anode for solid-state batteries

Peining Zhu ^{a, b} ,
Xi Guo ^c ,
Qinqin Yu ^d ,
Zuyong Wang ^c ,
Xiangxiao Lei ^{a, b} ,
Zhiwei Zhu ^a ,
Juan Du ^a ,
Xiaojia Zhang ^a ,
Yuan-Li Ding ^{c, *,}

a.
School of Electronic Information Engineering, Changsha Social Work College, Changsha 410004, China
b.
Hunan Intelligent Rehabilitation Robot and Auxiliary Equipment Engineering Technology Research Center, Changsha 410004, China
c.
College of Materials Science and Engineering, Hunan University, Changsha 410082, China
d.
College of Materials and Chemical Engineering, Pingxiang University, Pingxiang 337055, China

Received Date: 27 January 2025
Revised Date: 21 May 2025
Accepted Date: 28 May 2025
Available Online: 28 May 2025

Figures(13)

Solid-state lithium-ion batteries (SSLIBs) offer significant advantages over traditional liquid-electrolyte-based batteries, including improved safety, higher energy density, and better thermal stability. Among various anode materials, silicon (Si)-based anodes have attracted significant attention due to their ultrahigh theoretical capacity (~4200 mAh/g) and abundant resources. However, widespread adoption of Si-based anodes in SSLIBs is still restricted by some critical challenges such as severe volume expansion, low electronic and ionic conductivity, high interfacial impedance, and low initial Coulombic efficiency (ICE). This review mainly focuses on the design strategies of Si-based anode for SSLIBs at the material, electrode and cell levels including nanostructuring, Si alloys, Si-carbon composites, conductive additives, advanced binder, external pressure, electrolyte infiltration, and prelithiation. The insights provided here aim to inspire future research and accelerate commercialization of high-performance Si-based anodes in next-generation SSLIBs.
- Si anode,
- Solid state battery,
- Energy density,
- Power density,
- Design strategy
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