Citation: Yuhao Ma, Yufei Zhou, Hongli Li, Cheng Fang, Mingchuan Yu, Shaoxia Yang, Junfeng Niu. Photoelectrocatalytic degradation of refractory organic pollutants in water: Mechanism of active species generation by modulating the photoanode micro-interface[J]. Chinese Chemical Letters, ;2026, 37(1): 111249. doi: 10.1016/j.cclet.2025.111249 shu

Photoelectrocatalytic degradation of refractory organic pollutants in water: Mechanism of active species generation by modulating the photoanode micro-interface

Yuhao Ma ^{a, b} ,
Yufei Zhou ^{a, *,} ,
Hongli Li ^c ,
Cheng Fang ^d ,
Mingchuan Yu ^a ,
Shaoxia Yang ^b ,
Junfeng Niu ^a

a.
College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, China
b.
College of Water Conservancy and Hydropower Engineering, North China Electric Power University, Beijing 102206, China
c.
PetroChina Lanzhou Petrochemical Company, Lanzhou 730060, China
d.
Global Centre for Environmental Remediation (GCER), University of Newcastle, Callaghan, NSW 2308, Australia

zhouyf@ncepu.edu.cn

Received Date: 27 November 2024
Revised Date: 9 February 2025
Accepted Date: 21 April 2025
Available Online: 22 April 2025

Figures(5)

The escalating global issues of water scarcity and pollution emphasize the critical need for the rapid development of efficient and eco-friendly water treatment technologies. Photoelectrocatalytic technology has emerged as a promising solution for effectively degrading refractory organic pollutants in water under light conditions. This review delves into the advancements made in the field, focusing on strategies to enhance the generation of active species by modulating the micro-interface of the photoanode. Strategies, such as morphological control, element doping, introduction of surface oxygen vacancies, and construction of heterostructures, significantly improve the separation efficiency of photogenerated charges and the generation of active species, thereby boosting the efficiency of photoelectrocatalytic performance. Furthermore, the review explores the potential applications of photoelectrocatalytic technology in organic pollutant degradation in solutions. It also outlines the current challenges and future development directions. Despite its remarkable laboratory success, practical implementation of photoelectrocatalytic technology encounters obstacles related to stability, cost-effectiveness, and operational efficiency. Future investigations need to focus on optimizing the performance of photoelectrocatalytic materials and exploring strategies for upscaling their application in real water treatment scenarios.
- Photoelectrocatalytic degradation,
- Photoanode,
- Interface modulation,
- Active species,
- Mechanism
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沈阳化工大学材料科学与工程学院沈阳 110142